Discovery (theoretical prediction and experimental observation) of a large-gap topological-insulator class with spin-polarized single-Dirac-cone on the surface
arXiv:0908.3513 · doi:10.1038/nphys1274
Abstract
Recent theories and experiments have suggested that strong spin-orbit coupling effects in certain band insulators can give rise to a new phase of quantum matter, the so-called topological insulator, which can show macroscopic entanglement effects. Such systems feature two-dimensional surface states whose electrodynamic properties are described not by the conventional Maxwell equations but rather by an attached axion field, originally proposed to describe strongly interacting particles. It has been proposed that a topological insulator with a single spin-textured Dirac cone interfaced with a superconductor can form the most elementary unit for performing fault-tolerant quantum computation. Here we present an angle-resolved photoemission spectroscopy study and first-principle theoretical calculation-predictions that reveal the first observation of such a topological state of matter featuring a single-surface-Dirac-cone realized in the naturally occurring BiSe class of materials. Our results, supported by our theoretical predictions and calculations, demonstrate that undoped compound of this class of materials can serve as the parent matrix compound for the long-sought topological device where in-plane surface carrier transport would have a purely quantum topological origin. Our study further suggests that the undoped compound reached via n-to-p doping should show topological transport phenomena even at room temperature.
3 Figures, 18 pages, Submitted to NATURE PHYSICS in December 2008
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- Engineering topological phases in triple HgTe/CdTe quantum wells
- Polariton vortex Chern insulator
- Magnetic band representations, Fu-Kane-like symmetry indicators and magnetic topological materials
- Searching for two-dimensional Weyl superconductors in heterostructures
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- Quantum transport in topological insulator hybrid structures -- A combination of topological insulator and superconductor
- Time-reversal Invariant SU(2) Hofstadter Problem in Three Dimensional Lattices
- Growth of Ultrathin BiSe Films by Molecular Beam Epitaxy
- Link between \emph{Zitterbewegung} and topological phase transition
- Anomalous nuclear magnetic resonance spectra in BiSe nanowires
- Ferromagnetism and glassiness on the surface of topological insulators
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- Magnetoelectric effect of a conducting sphere near a planar topological insulator
- Spectromicroscopic measurement of surface and bulk band structure interplay in a disordered topological insulator
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- A fourth-order compact time-splitting method for the Dirac equation with time-dependent potentials
- On nonlinear classical electrodynamics with an axionic term
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- Dirac Electrons on a Sharply Edged Surface of Topological Insulators
- Competing energy scales in topological superconducting heterostructures
- Confining electrons on a topological insulator surface using potentials and a magnetic field
- Straining the Identity of Majorana Fermions
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- Probing edge state conductance in ultra-thin topological insulator films
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- Phononic drumhead surface state in distorted kagome compound RhPb
- Spatial Control of Charge Doping in n-Type Topological Insulators
- Exchange-Driven Intermixing of Bulk and Topological Surface State by Chiral Excitons in Bi2Se3
- Gapless interface states at the junction between two topological insulators
- Strain-induced topological phase transition at (111) SrTiO-based heterostructures
- Observation of anisotropic Dirac cones in the topological material Ti2Te2P
- Selective Trapping of Hexagonally Warped Topological Surface States in a Triangular Quantum Corral
- Berry-phase switch in electrostatically-confined topological surface states
- Photoemission spectra of massless Dirac fermions on the verge of exciton condensation
- Topological field-effect transistor with quantized ON/OFF conductance of helical/chiral dislocation states
- Structure of surface electronic states in strained mercury telluride
- Thin films as practical quantum materials: a status quo and beyond
- Spin Current Density Functional Theory of the Quantum Spin-Hall Phase
- Tunnel Magnetoresistance scan of a pristine three-dimensional topological insulator
- Robustness of persistent currents in two-dimensional Dirac systems with disorders
- Geometrical phase shift in Friedel oscillations
- Observability of superconductivity in Sr-doped Bi2Se3 at the surface using scanning tunneling microscope
- Effect of surface hybridization on RKKY coupling in ferromagnet/topological insulator/ferromagnet trilayer system
- La1-xBi1+xS3 (x~0.08): An n-Type Semiconductor
- Room temperature nonlocal detection of charge-spin interconversion in a topological insulator
- Signature of pressure-induced topological phase transition in ZrTe
- New polarization rotation and exact TEM wave solutions in topological insulators
- Electronic and Vibrational Excitations on the Surface of the Three-Dimensional Topological Insulator BiTeSe (x = 0, 2, 3)
- Experimental demonstration of a magnetically induced warping transition in a topological insulator mediated by rare-earth surface dopants
- Engineering Interlayer Hybridization in Energy Space via Dipolar Overlayers
- Topologically localized insulators
- Existence of dual topological phases in Sn-based ternary chalcogenides
- Coulomb drag in topological materials
- Topological electronic bands in crystalline solids
- Tailoring Kinetics on a Topological Insulator Surface by Defect-Induced Strain: Pb Mobility on Bi2Te3
- Measuring the Chern number with quantum oscillations
- An increase in under hydrostatic pressure in the superconducting doped topological insulator NbBiSe
- Ultrathin film of 3D topological insulators by vapor-phase epitaxy: Surface dominant transport in wide temperature revealed by Seebeck measurement
- Plasmon modes in the magnetically doped Single Layer and Multilayers of Helical Metals
- Dirac Fermions and Topological Phases in Magnetic Topological Insulator Films
- Linear nonsaturating magnetoresistance in the Nowotny chimney ladder compound RuSn
- Topological transitions to Weyl states in bulk BiSe: Effect of hydrostatic pressure and doping
- Experimental observation and spin texture of Dirac node arcs in tetradymite topological metals
- Generic theory of characterizing topological phases under quantum slow dynamics
- Strong magneto-optical effects due to surface states in three-dimensional topological insulators
- Bulk cyclotron resonance in the topological insulator Bi2Te3
- Ultrahigh magnetic field spectroscopy reveals the band structure of the 3D topological insulator BiSe
- Electrical modulation of the edge channel transport in topological insulators coupled to ferromagnetic leads
- Proximity induced ferromagnetism, superconductivity, and finite-size effects on the surface and edge states of topological insulator nanostructures
- Novel Majorana mode and magnetoresistance in ferromagnetic superconducting topological insulator
- The search for strong topological insulators
- Optical intersubband properties of a core-shell semiconductor-topological insulator quantum dot described by -Electrodynamics
- Hidden-symmetry-protected Z_2 topological insulator in a cubic lattice
- Full superconducting gap in the candidate topological superconductor InPbTe for x = 0.2
- Kramers-Weyl fermions in the chiral charge density wave material (TaSe)I
- Electrified magnetic catalysis in three-dimensional topological insulators
- Automated construction of maximally localized Wannier functions for bands with nontrivial topology
- Quantum spin Hall effect in two-dimensional transition-metal chalcogenides
- Observation of optical absorption correlated with surface state of topological insulator
- Anisotropic RKKY interactions mediated by quasiparticles in half-Heusler topological semimetal
- Weyl states and Fermi arcs in parabolic bands
- Universal Metallic Surface States in Electride
- Software implementation for calculating the Chern and topological invariants with WIEN2k all-electron density functional package
- Low-energy phonons and superconductivity in SnInTe
- 2D compressibility of surface states on 3D topological insulators
- Effect of chiral selective tunneling on quantum transport in magnetic topological-insulator thin films
- Quantum oscillations and nontrivial transport in (Bi0.92In0.08)2Se3
- Topological Field Theories of Three-Dimensional Rotation Symmetric Insulators: Coupling Curvature and Electromagnetism
- Stability of Topological Insulators with Non-Abelian Edge Excitations
- Modulation of Dirac electrons in epitaxial Bi2Se3 ultrathin films on van-der-Waals ferromagnet Cr2Si2Te6
- Autonomous microARPES
- In-situ topotactic chemical reaction for spectroscopies
- From classical to quantum regime of topological surface states via defect engineering
- Theory of Weyl orbital semimetals and predictions of several materials classes
- Spectroscopic signature of surface states and bunching of bulk subbands in topological insulator (BiSb)Te thin films
- Transmission in graphene-topological insulator heterostructures
- Surface states induced weak anti-localization effect in Bi0.85Sb0.15 topological single crystal
- Large Thermal Hall Effect in MnPS
- Interacting topological phases in thin films of topological mirror Kondo insulators
- Capacitive scheme to detect the topological magnetoelectric effect
- Vavilov-Cherenkov radiation for parallel motion in three-dimensional topological insulators
- Weakly interacting one-dimensional topological insulators: a bosonization approach
- Electronic Transport Studies of Ag-doped Bi2Se3 Topological Insulator
- Electron dynamics in topological insulator based semiconductor-metal interfaces (topological p-n interface based on Bi2Se3 class)
- Elementary models of 3D topological insulators with chiral symmetry
- Berry curvature, semiclassical electron dynamics, and topological materials: Lecture notes for Introduction to Solid State Physics
- Topological property of a system with a honeycomb lattice structure
- Weyl semimetallic state with antiferromagnetic order in Rashba-Hubbard model
- Refined Majorana phase diagram in topological insulator-superconductor hybrid system
- Ambipolar Electric Field Effect in Metallic Bi2Se3
- Anomalous in-gap edge states in two-dimensional pseudospin-1 Dirac insulators
- Time- and angle-resolved photoemission spectroscopy with wavelength-tunable pump and extreme ultraviolet probe enabled by twin synchronized amplifiers
- Environmental Doping-Induced Degradation of the Quantum Anomalous Hall Insulators
- Interplay between Topological States and Rashba States as Manifested on Surface Steps at Room Temperature
- Low-temperature thermal expansion of the topological material candidates -PtBi and -BiPd
- Observation of paramagnetic spin-degeneracy lifting in EuZn2Sb2
- Probing surface states exposed by crystal terminations at arbitrary orientations of three-dimensional topological insulators
- Topological surface states in the Kondo insulator YbB revealed via planar tunneling spectroscopy
- Electronic structure of 2D van der Waals crystals and heterostructures investigated by spatially- and angle-resolved photoemission
- Intrinsic Layer-Dependent Surface Energy and Exfoliation Energy of van der Waals Materials
- High-field charge transport on the surface of BiSe
- Single Crystal Growth and Transport Properties of van der Waals Materials Te ( = Ti, Zr, Hf)
- Electromagnetic coupling and transport in a topological insulator-graphene hetero-structure
- Mode-Shell correspondence, a unifying phase space theory in topological physics -- part II: Higher-dimensional spectral invariants
- Topological quantum phase transition in strongly correlated Kondo insulators in 1D
- Semiconducting Electronic Structure of the Ferromagnetic Spinel Revealed by Soft-X-Ray Angle-Resolved Photoemission Spectroscopy
- Nonlinear planar magnetotransport as a probe of the topology of surface states
- Observation of Dirac-like surface state bands on the top surface of BiSe
- Detecting winding and Chern numbers in topological matter using spectral function
- Electronic structure in a transition metal dipnictide TaAs2
- Layer dependent topological phases and transitions in TaRhTe: From monolayer and bilayer to bulk
- Ultrafast electron dynamics in a topological surface state observed in two-dimensional momentum space
- Spectroscopic Evidence on Realization of a Genuine Topological Nodal Line Semimetal in LaSbTe
- Dynamical characterization of Floquet topological phases via quantum quenches
- Collective excitations and screening in two-dimensional tilted nodal-line semimetals
- A proposal for realizing Majorana fermions without external magnetic field in strongly correlated nanowires
- Anomalous temperature dependence of optical and acoustic phonons in BiSe arising from stacking faults
- Microscopic Green's function approach for generalized Dirac Hamiltonians
- Spintronic Quantum Phase Transition in a Heterostructure with Giant Rashba Spin-Orbit Coupling
- Emergent topological states via digital (001) oxide superlattices
- SPADExp: A photoemission angular distribution simulator directly linked to first-principles calculations
- Ultra-high mechanical stretchability and controllable topological phase transitions in two-dimensional arsenic
- Non-linear hybrid surface-defect states in defective BiSe
- An ab initio investigation of BiSe topological insulator deposited on amorphous SiO
- Modification of the hybridization gap by twisted stacking of quintuple layers in a three dimensional topological insulator thin film
- One-Dimensional Spin-Polarised Surface States -- A Comparison of Bi(112) with Other Vicinal Bismuth Surfaces
- Interfacial Fermi Loops from Interfacial Symmetries
- Operator Formalism for Noncollinear Functionals in Multicollinear Approach
- Unoccupied Topological Surface State in MnBiTe
- Beta-Ag2Te: A topological insulator with strong anisotropy
- Electron-electron interactions in partially mixed helical states
- Fermi Surface Topology and Magneto-transport Properties of Superconducting PdBiSe
- Reconstructing the wavefunction of magnetic topological insulators MnBi2Te4 and MnBi4Te7 using spin-resolved photoemission
- Topological surface states hybridized with bulk states of Bi-doped PbSb2Te4 revealed in quasiparticle interference
- Interacting Crystalline Topological Insulators in two-dimensions with Time-Reversal Symmetry
- Anomalous Linear and Quadratic Nodeless Surface Dirac Cones in Three-Dimensional Dirac Semimetals
- Anomalous Shiba spectrum and superconductivity induced magnetic interactions in materials with topological band inversion
- Quantum-anomalous-Hall current patterns and interference in thin slabs of chiral topological superconductors
- Sb2Se3 and SbBiSe3 Surface Capping and Biaxial Strain Co-Engineering for Tuning the Surface Electronic Properties of Bi2Se3 Nanosheet- A Density Functional Theory based Investigation
- Berezinskii-Kosterlitz-Thouless transitions in a topological superconductor-ferromagnet-superconductor junction
- Stability of the X-Y-phase of the two-dimensional C4 point group insulator
- Ultrafast electron dynamics at the Dirac node of the topological insulator SbTe
- Diffusion at the Surface of Topological Insulators
- Inter-quintuple layer coupling and topological phase transitions in the chalcogenide topological insulators
- Quantum Transport and Magnetism of Dirac Electrons in Solids
- Quasiparticle scattering in three-dimensional topological insulators near the thickness limit
- Non-necessity of band inversion process in 2D topological insulators for bulk gapless states and topological phase transitions
- Reexamining Circular Dichroism in Photoemission From a Topological Insulator
- X-ray diffraction tools for structural modeling of epitaxic films of an intrinsic antiferromagnetic topological insulator
- Visualizing the in-gap states in domain boundaries of ultra-thin topological insulator films
- Spin-orbit torque: Moving towards two-dimensional van der Waals heterostructures
- Electron scattering in a superlattice of line defects on the surface of topological insulators
- Band structure of Bi surfaces formed on Bi2Se3 upon exposure to air
- Magnetic-flux tunable electronic transport through domain walls in a three-dimensional second-order topological insulator
- Exact modes, hybridization and polarization rotation of electromagnetic fields propagating in topological insulating slab
- Phonon Weyl points and chiral edge modes with unconventional Fermi arcs in NbSi
- Reversible Modification of Rashba States in Topological Insulators at Room Temperature by Edge Functionalization
- Nucleation and Antiphase Twin Control in BiSe via Step-Terminated AlO Substrates
- Low-energy effective Hamiltonian and end states of an inverted HgTe nanowire
- Fermions in -dimensions modified by nonminimal coupling and its applications to condensed matter physics
- Bulk and surface electron scattering in disordered BiTe probed by quasiparticle interference
- Strain-engineering quantum anomalous Hall effect in janus MnBi2SexTe4-x monolayers
- Origin of Robust Topological Phases in Stacked Hermitian Systems: Non-Hermitian Level Repulsion
- Mass fluctuations and absorption rates in Dirac materials sensors
- Interplay between strain and size quantization in a class of topological insulators based on inverted-band semiconductors
- Photonic analogue of quantum spin Hall effect
- Non-Hermitian topological wall modes in rotating Rayleigh-Benard convection
- Fermionic atoms in a spin-dependent optical lattice potential: topological insulators with broken time-reversal symmetry
- Engineering Topological Nodal Line Semimetals in Rashba Spin-Orbit Coupled Atomic Chains
- Parity anomaly with impurities and the Pauli--Villars subtraction
- Hybridization and Field Driven Phase Transitions in Hexagonally Warped Topological Insulators
- Electronic structures and stability investigation of the new class of large band gap topological insulators MTlTe (M = Cd, Hg)
- Tuning the vertical location of helical surface states in topological insulator heterostructures via dual-proximity effects
- Persistent Topological Surface State at the Interface of Bi2Se3 Film Grown on Patterned Graphene
- Discovery of the topological surface state in a noncentrosymmetric superconductor BiPd
- Scanning tunneling microscopy study of the possible topological surface states in BiTeCl
- Current Modulator based on Topological Insulator with Sliding Magnetic Superlattice
- Development of a versatile micro-focused angle-resolved photoemission spectroscopy system with Kirkpatrick-Baez mirror optics
- Emergence of Type-I and Type-II Dirac line nodes in penta-octa-graphene
- Non-unique connection between bulk topological invariants and surface physics
- Exact solutions for topological surface states of three-dimensional lattice models
- Preparation and observation of anomalous counterpropagating edge states in a periodically driven optical Raman lattice
- ToMSGKpoint: A user-friendly package for computing symmetry transformation properties of electronic eigenstates of nonmagnetic and magnetic crystalline materials
- Distinct topological excitonic insulators characterized by quantum geometry
- Multiplicative Chern insulator
- Synthetic gauge field and pseudospin-orbit interaction in a stacked two-dimensional ring-network lattice
- Electrical probe of spin-spiral order in quantum spin Hall/spin-spiral magnet van der Waals heterostructures
- Theory of Superconductivity Mediated by Topological Phonons
- Topological Surface States and Superconductivity in [Tl](TlSn)Te Perovskites
- Majorana vortex phases in time-reversal invariant higher-order topological insulators and topologically trivial insulators
- Superconductivity in spin-orbit coupled BaBi formed by in situ reduction of bismuthate films
- Intrinsic Nernst Effect from Berry Curvature in Superconductors
- Multipartite Entanglement in Crossing the Quantum Critical Point
- Electromagnetic response of the surface states of a topological insulator nanowire embedded within a resonator
- Quantum anomalous Hall effect with high Chern number in two dimensional ferromagnets Ti2TeSO
- Feynman paradox in a spherical axion insulator
- Analytical solutions of topological surface states in a series of lattice models
- To See a World in a Grain of Sand -- The Scientific Life of Shoucheng Zhang
- Induced robust topological order on an ordinary insulator hetero-structured with a strong topological insulator
- Controlling quantum spin Hall state via strain in various stacking bilayer phosphorene
- Enhanced detection of circularly polarized photons with topological materials
- Tailoring Ultrathin Magnetic Multilayers at Terraced Topologically Insulating Interfaces for Perpendicularly Magnetized Domains
- Conductance Oscillations in a Topological Insulator-Disordered Superconductor Hybrid Interface
- Sb doping effect on transport behavior in the topological insulator Bi2Se3
- Evolution from Topological Dirac Metal to Flat-band-Induced Antiferromagnet in Layered KxNi4S2 (0<=x<=1)
- A weak topological insulator state in quasi-one-dimensional superconductor TaSe
- Temperature-Dependent Collective Excitations in a Three-Dimensional Dirac System ZrTe
- Topological excitations in quasi two-dimensional quantum magnets with weak interlayer interactions
- Termination dependence of the surface states in PbPd
- Full investigation of nonadiabatic dynamical characterization in arbitrary quenching process
- Systematic study for two-dimensional topological phase transitions at high-symmetry points in all layer groups
- Symmetry-protected topological corner modes in a periodically driven interacting spin lattice
- Local density of state oscillations in laterally heterostructured topological insulator-semiconductor systems
- Procedures for assessing the stability of proposed topological materials
- Signature of topological crystalline insulating behavior in new B2X2Zn (X=Ir, Rh, Co) compound from first-principles Computation
- Robust large-gap topological insulator phase in transition-metal chalcogenide ZrTeSe