Ultrafast dynamics of photocurrents in surface states of 3D topological insulators

Abstract

This article reviews experimental work on the ultrafast electron dynamics in the topological surface state (TSS) of three-dimensional (3D) topological insulators (TIs) observed with time- and angle-resolved two-photon photoemission (2PPE). The focus is laid on the generation of ultrafast photocurrents and the time-resolved observation of their decay. 2PPE not only allow to unambiguously relate the photocurrents to the spin-polarized electronic surface states. Probing of the asymmetric momentum distribution of the electrons carrying the current makes it possible to study the microscopic scattering processes that governs the unusual electron transport in the time domain. Ultrashort mid-infrared pump pulses permit not only a direct optical excitation of the TSS in Sb${}_2$Te${}_3$ but also lead to a strong asymmetry of the TSS population in momentum space. Two-dimensional band mapping of the TSS shows that this asymmetry is in fact representative for a macroscopic photocurrent while the helicity-dependence of the photocurrent is found to be small. The time-resolved observation of the photocurrent decay reveals a huge mean free path of the electrons in the TSS.

arXiv comment15 pages, 11 figures

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• Nonthermal pathways to ultrafast control in quantum materials
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• Ultrafast transient absorption spectroscopy of 2D semiconductors: a review
• Two-photon IR pumped UV-Vis transient absorption spectroscopy of Dirac fermions in the 2D and 3D topological insulator Bi2Se3