Time- and angle-resolved photoemission spectroscopy with wavelength-tunable pump and extreme ultraviolet probe enabled by twin synchronized amplifiers

Abstract

We describe a setup for time- and angle-resolved photoemission spectroscopy with wavelength-tunable excitation and extreme ultraviolet probe. It is enabled by using the 10 kHz twin Ti:sapphire amplifiers seeded by the common Ti:sapphire oscillator. The typical probe energy is 21.7 eV, and the wavelength of the pump excitation is tuned between 2400 and 1200 nm by using the optical parametric amplifier. The total energy resolution of 133 meV is achieved, and the time resolution is dependent on the wavelength for the pump, typically better than 100 fs. This system enables the pump energy to be matched with a specific interband transition and to probe a wider energy-momentum space. We present the results for the prototypical materials of highly oriented pyrolytic graphite and Bi2Se3 to show the performance of our system.

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Cited by in corpus (3)

• Unveiling van Hove singularity modulation and fluctuated charge order in kagome superconductor $\mathrm{Cs}{\mathrm{V}}_3\mathrm{S}{\mathrm{b}}_5$ via time-resolved ARPES
• Time-Resolved Photoemission Spectroscopy of Quantum Materials Using High Harmonic Generation: Probing Electron-Phonon Interactions and Non-Equilibrium Dynamics
• Distinct amplitude mode dynamics upon resonant and off-resonant excitation across the charge density wave energy gap in LaTe3 investigated by time- and angle-resolved photoemission spectroscopy