Time-Resolved Photoemission Spectroscopy of Quantum Materials Using High Harmonic Generation: Probing Electron-Phonon Interactions and Non-Equilibrium Dynamics

Abstract

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum materials in both time and momentum space. In this review, we present recent representative studies utilizing HHG-laser-based time- and angle-resolved photoemission spectroscopy for a variety of quantum materials. We particularly highlight electron-phonon interactions and non-equilibrium dynamics in time and frequency domain, through which rich information about non-equilibrium electron-phonon couplings and related phenomena has been clearly revealed.

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