Phase Diagram and High Temperature Superconductivity at 65 K in Tuning Carrier Concentration of Single-Layer FeSe Films
arXiv:1207.6823 · doi:10.1038/nmat3648
Abstract
Superconductivity in the cuprate superconductors and the Fe-based superconductors is realized by doping the parent compound with charge carriers, or by application of high pressure, to suppress the antiferromagnetic state. Such a rich phase diagram is important in understanding superconductivity mechanism and other physics in the Cu- and Fe-based high temperature superconductors. In this paper, we report a phase diagram in the single-layer FeSe films grown on SrTiO3 substrate by an annealing procedure to tune the charge carrier concentration over a wide range. A dramatic change of the band structure and Fermi surface is observed, with two distinct phases identified that are competing during the annealing process. Superconductivity with a record high transition temperature (Tc) at ~65 K is realized by optimizing the annealing process. The wide tunability of the system across different phases, and its high-Tc, make the single-layer FeSe film ideal not only to investigate the superconductivity physics and mechanism, but also to study novel quantum phenomena and for potential applications.
15 pages, 4 figures
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- Temperature dependence and limiting mechanisms of the upper critical field of FeSe thin films
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- Nodeless multigap superconductivity in organic-ion-intercalated (tetrabutyl~ammonium)FeSe
- Suppression of nematicity by tensile strain in multilayer FeSe/SrTiO films
- Inferior interfacial superconductivity in 1 UC FeSe/SrVO/SrTiO with screened interfacial electron-phonon coupling
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- Identifying a forward scattering superconductor through pump-probe spectroscopy
- Studies of superconductivity of Fe chalcogenides in films grown by PLD technique
- Study on fluctuations of interface-enhanced superconductivity in ultrathin FeSe/SrTiO3 by the Nernst effect
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- LaO as a candidate substrate for realizing superconductivity in FeSe epitaxial film
- Enhancing the hybridization of plasmons in graphene with 2D superconductor collective modes
- Time-Resolved Photoemission Spectroscopy of Quantum Materials Using High Harmonic Generation: Probing Electron-Phonon Interactions and Non-Equilibrium Dynamics
- Suppression and revival of superconducting phase coherence in monolayer FeSe/SrTiO
- Origin of the Electronic Structure in Single-Layer FeSe/SrTiO3 Films
- Fabrication of oxide/FeSe multilayer films using the PLD technique
- Fragile pressure-induced magnetism in FeSe superconductors with a thickness reduction
- Fe-vacancy ordered Fe4Se5: The insulating parent phase of FeSe superconductor
- Temperature evolution of the Fermi surface of the FeSe monolayer on SrTiO
- Disorder-induced time effect in the antiferromagnetic domain state of Fe1+yTe
- Quantum-Critical Spin-Density Waves in Iron-Selenide High-Tc Superconductors
- Dual Enhancement of Superconductivity in FeSe/SrTiO3 via Orbital and Correlation Synergy
- Coexistence of d-Wave Altermagnetism and Topological States in Janus FeSeX (X = S, Te) Monolayers
- Superconductivity in the bilayer Hubbard model: Are two Fermi surfaces better than one?