Roton pair density wave and unconventional strong-coupling superconductivity in a topological kagome metal
arXiv:2103.09188 · doi:10.1038/s41586-021-03983-5
Abstract
The transition-metal kagome lattice materials host frustrated, correlated, and topological quantum states of matter. Recently, a new family of vanadium-based kagome metals AV3Sb5 (A=K, Rb, and Cs) with topological band structures has been discovered. These layered compounds are nonmagnetic and undergo charge density wave transitions before developing superconductivity at low temperatures. Here we report the observation of unconventional superconductivity and pair density wave (PDW) in CsV3Sb5 using scanning tunneling microscope/spectroscopy (STM/STS) and Josephson STS. We find that CsV3Sb5 exhibits a V-shaped pairing gap Δ~0.5 meV and is a strong-coupling superconductor (2Δ/kBTc~5) that coexists with 4a0 unidirectional and 2a0X2a0 charge order. Remarkably, we discover a 3Q PDW accompanied by bidirectional 4a0/3 spatial modulations of the superconducting gap, coherence peak and gap-depth in the tunneling conductance. We term this novel quantum state a roton-PDW associated with an underlying vortex-antivortex lattice that can account for the observed conductance modulations. Probing the electronic states in the vortex halo in an applied magnetic field, in strong-field that suppresses superconductivity, and in zero-field above Tc reveals that the PDW is a primary state responsible for an emergent pseudogap and intertwined electronic order. Our findings show striking analogies and distinctions to the phenomenology of high-Tc cuprate superconductors, and provide groundwork for understanding the microscopic origin of correlated electronic states and superconductivity in vanadium-based kagome metals.
Nature (2021)
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Cited by in corpus (353)
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- Charge-density wave fluctuation driven composite order in the layered Kagome Metals
- Observation of multiple flat bands and van Hove singularities in the distorted kagome metal NdTi3Bi4
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- Competing Lattice Instability and Magnetism on the Surface of Kagome Metals
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- Vortex phase diagram of kagome superconductor CsVSb
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- Switchable chiral 2x2 pair density wave in pure CsV3Sb5
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- Enhanced pair-density-wave vertices in a bilayer Hubbard model at half-filling
- Calculated Unconventional Superconductivity via Charge Fluctuations in Kagome Metal CsV3Sb5
- Strong pair-density-wave fluctuations in an exactly solvable doped Mott insulator
- Electronic structure of topological defects in the pair density wave superconductor
- Emergent dynamical Kondo coherence and competing magnetic order in a correlated kagome flat-band metal CsCr6Sb6
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- Current-induced magnetoresistance hysteresis in the kagome superconductor CsVSb
- Time-Resolved Photoemission Spectroscopy of Quantum Materials Using High Harmonic Generation: Probing Electron-Phonon Interactions and Non-Equilibrium Dynamics
- Inter-Layer Correlation of Loop Current Charge Density Wave on the Bilayer Kagomé Lattice
- Nematic correlations and nematic Berezinskii-Kosterlitz-Thouless transition in spin-1 kagome lattice antiferromagnets
- Emergent Pair Density Wave Order Across a Lifshitz Transition
- Role of On-site and Inter-site Coulomb Interactions in KVSb: A first-principles DFT++ study
- Crystal structure, properties and pressure-induced insulator-metal transition in layered kagome chalcogenides
- Kekulé order from diffuse nesting near higher-order Van Hove points
- The possible frustrated superconductivity in the kagome superconductors
- Pair-density-wave phase of strongly interacting electrons on the triangular lattice: A variational Monte Carlo study
- Incommensurate charge-stripe correlations in the kagome superconductor CsVSbSn
- Moire Engineering of Cooper-Pair Density Modulation States
- Phenomenological Ginzburg-Landau theory for triple-Q magnetic orders on a hexagonal lattice
- Nested Fermi surfaces and correlated electronic phases in hole-doped semiconductor quantum wells
- Effective Ionic Valence and Local Magnetic Moment in Kagome Superconductors
- Strain-Tuned Nodal Superconductivity in the Charge-Ordered Kagome Metal CsVSb
- Spin-triplet pair density wave superconductors
- Probing Quantum Geometric Phases via Scanning Tunneling Microscopy
- Mott-Derived Local Moments and Kondo Hybridization in a d-electron Kagome lattice
- Evidence of intertwined pair density and charge density wave orders in UTe2
- Gap fluctuations, Cooper pairs with finite center-of-mass momentum, and suppression of superconductivity in inhomogeneous systems with dopant superpuddles agglomerates
- Hexagonal-to-base-centered-orthorhombic charge density wave order in kagome metals KVSb, RbVSb, and CsVSb
- Charge-density waves in kagome-lattice extended Hubbard models at the van Hove filling
- Precompression engineering of metal-insulator transition and magnetism in designed breathing kagome systems
- Enhanced Coupling of Superconductivity and Evolution of Gap Structure in CsV3Sb5 through Ta Doping
- Coexisting electronic smectic liquid crystal and superconductivity in a Si square-net semimetal
- Kagome edge states under lattice termination, spin-orbit coupling, and magnetic order
- Novel dynamical excitations and roton-based measurement of Cooper-pair momentum in a two-dimensional Fulde-Ferrell-Larkin-Ovchinnikov superfluid on optical lattices
- Visualizing Pair-breaking Scattering Interference in Bulk FeSe
- Microscopic origin of period-four stripe charge-density-wave in kagome metal CsVSb
- Time-reversal symmetry-breaking phenomena in transport study of kagome superconductivity
- Topological pair density waves in kagome superconductors
- Magnetic fluctuations near the Van Hove singularity in the kagome-lattice Hubbard model at finite doping