Direct characterization of photo-induced lattice dynamics in BaFe2As2

Abstract

Ultrafast light pulses can modify the electronic properties of quantum materials by perturbing the underlying, intertwined degrees of freedom. In particular, iron-based superconductors exhibit a strong coupling among electronic nematic fluctuations, spins, and the lattice, serving as a playground for ultrafast manipulation. Here we use time-resolved x-ray scattering to measure the lattice dynamics of photo-excited BaFe2As2. Upon optical excitation, no signature of an ultrafast change of the crystal symmetry is observed, but the lattice oscillates rapidly in time due to the coherent excitation of an A1g mode that modulates the Fe-As-Fe bond angle. We directly quantify the coherent lattice dynamics and show that even a small photo-induced lattice distortion can induce notable changes in the electronic and magnetic properties. Our analysis implies that transient structural modification can generally be an effective tool for manipulating the electronic properties of multi-orbital systems, where electronic instabilities are sensitive to the orbital character of bands near the Fermi level.

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• Analysis methodology of coherent oscillations in time- and angle-resolved photoemission spectroscopy
• Transient gap generation in BaFe${}_2$As${}_2$ driven by coherent lattice vibrations
• Time-Resolved Photoemission Spectroscopy of Quantum Materials Using High Harmonic Generation: Probing Electron-Phonon Interactions and Non-Equilibrium Dynamics