Gate-tunable Room-temperature Ferromagnetism in Two-dimensional FeGeTe
arXiv:1803.02038 · doi:10.1038/s41586-018-0626-9
Abstract
Material research has been a major driving force in the development of modern nano-electronic devices. In particular, research in magnetic thin films has revolutionized the development of spintronic devices; identifying new magnetic materials is key to better device performance and new device paradigm. The advent of two-dimensional van der Waals crystals creates new possibilities. This family of materials retain their chemical stability and structural integrity down to monolayers and, being atomically thin, are readily tuned by various kinds of gate modulation. Recent experiments have demonstrated that it is possible to obtain two-dimensional ferromagnetic order in insulating CrGeTe and CrI at low temperatures. Here, we developed a new device fabrication technique, and successfully isolated monolayers from layered metallic magnet FeGeTe for magnetotransport study. We found that the itinerant ferromagnetism persists in FeGeTe down to monolayer with an out-of-plane magnetocrystalline anisotropy. The ferromagnetic transition temperature, , is suppressed in pristine FeGeTe thin flakes. An ionic gate, however, dramatically raises the up to room temperature, significantly higher than the bulk of 205 Kelvin. The gate-tunable room-temperature ferromagnetism in two-dimensional FeGeTe opens up opportunities for potential voltage-controlled magnetoelectronics based on atomically thin van der Waals crystals.
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- Tunable large spin Nernst effect in a two-dimensional magnetic bilayer
- Enhanced - hybridization intertwined with anomalous ground state formation in van der Waals-coupled magnetic metal FeGeTe
- Two-dimensional Heisenberg models with materials-dependent superexchange interactions
- On-site and inter-site Hubbard corrections in magnetic monolayers: The case of FePS and CrI
- Ferromagnetic MnSn monolayer epitaxially grown on silicon substrate
- Imaging current control of magnetization in FeGeTe with a widefield nitrogen-vacancy microscope
- Sign-reversed anomalous Nernst effect in the ferromagnetic Weyl-semimetal FeGeTe: the role of Fe vacancies
- Tunneling-tip-induced collapse of the charge gap in the excitonic insulator TaNiSe
- Stability of the novel interorbital-hopping mechanism for ferromagnetism in multi-orbital Hubbard models
- Monolayer Magnetic Metal with Scalable Conductivity
- Layer Control of Magneto-Optical Effects and Their Quantization in Spin-Valley Splitting Antiferromagnets
- Effect of biaxial strain and hydrostatic pressure on the magnetic properties of bilayer CrI3
- Tuning the Curie temperature of a 2D magnet/topological insulator heterostructure to above room temperature by epitaxial growth
- Relating spin-polarized STM imaging and inelastic neutron scattering in the van-der-Waals ferromagnet Fe3GeTe2
- Coexistence of intrinsic piezoelectricity, ferromagnetism and nontrivial band topology in Li-decorated Janus monolayer with high Curie temperature
- Microscopic origin of the magnetic easy-axis switching in Fe3GaTe2 under pressure
- Magnetic State Control of Non-van der Waals 2D Materials by Hydrogenation
- Mechanism of magnetic phase transition in correlated magnetic metal: insight into itinerant ferromagnet FeGeTe
- Realization of Kagome Kondo lattice
- Stability of the In-Plane Room Temperature van der Waals Ferromagnet Chromium Ditelluride and Its Conversion to Chromium-Interleaved CrTe Compounds
- Above-room-temperature intrinsic ferromagnetism in ultrathin van der Waals crystal FeGaTe
- Room temperature ferromagnetic semiconductors through metal-semiconductor transition in monolayer MnSe2
- Identifying band structure changes of FePS3 across the antiferromagnetic phase transition
- Spanning Fermi arcs in a two-dimensional magnet
- Pressure evolution of electronic structure and magnetism in the layered van der Waals ferromagnet CrGeTe
- Josephson spin-valve realization in the magnetic nodal-line topological semimetal FeGeTe
- Magnetic Switching in Monolayer 2D Diluted Magnetic Semiconductors via Spin-to- Spin Conversion
- Mechanism of carrier doping induced magnetic phase transitions in two-dimensional materials
- Anisotropic magnetic properties and tunable conductivity in two-dimensional layered NaCrX2 (X=Te,Se,S) single crystals
- Magnetoelectric effect in van der Waals magnets
- Synthesis and physical properties of a new layered ferromagnet, Cr1.21Te2
- DFT+DMFT investigation of the magnetic phase transition in the itinerant ferromagnet FeGaTe
- Proposal for all-electrical skyrmion detection in van der Waals tunnel junctions
- Defect-induced -magnetism in layered platinum diselenide
- Correlation-driven topological transition in Janus VSiGeP2As2
- Monolayer C networks: A first-principles perspective
- FeGeTe -- A new exfoliable itinerant ferromagnet with high Curie temperature and large perpendicular magnetic anisotropy
- Twisted Bogoliubov quasiparticles in the superconducting NbSe monolayer on graphene
- Gate-controlled proximity effect in superconductor/ferromagnet van der Waals heterostructures
- Two-dimensional hole transport in ion-gated diamond surfaces: A brief review
- Electron transport and scattering mechanisms in ferromagnetic monolayer FeGeTe
- Frustration-induced magnetic bimerons in transition metal halide CoX2 (X = Cl, Br) monolayers
- Magnetic surface on nonmagnetic bulk of electride Hf2S
- Magnetoelectricity in two-dimensional materials
- Prediction of 2D ferromagnetism and monovalent europium ions in the EuBr/graphene heterojunctions
- Synthetic Semimetals with van der Waals Interfaces
- Acousto-magnonic spin Hall effect in honeycomb antiferromagnets
- Hidden interplay of current-induced spin and orbital torques in bulk FeGeTe
- Designing spin-textured flat bands in twisted graphene multilayers via helimagnet encapsulation
- Tunable magnetism in bilayer transition metal dichalcogenides
- Infrared study of carrier scattering mechanism in ion-gated graphene
- Enhanced Ferromagnetism in Monolayer Cr2Te3 via Topological Insulator Coupling
- First-principles study on the bulk and two-dimensional structures of AMnBi(A =K, Rb, Cs)-family materials
- Gate-tunable Exchange Bias and Voltage-controlled Magnetization Switching in a van der Waals Ferromagnet
- Spin filtering effect in intrinsic 2D magnetic semiconductor Cr2Ge2Te6
- Magnetic damping anisotropy in the two-dimensional van der Waals material FeGeTe from first principles
- High-spin orbital interactions across van der Waals gaps controlling the interlayer ferromagnetism in van der Waals ferromagnets
- Intricate magnetic interactions and topological Hall effect observed in itinerant room-temperature layered ferromagnet Cr0.83Te
- Electric-field-induced formation and annihilation of skyrmions in two-dimensional magnet
- Kubo formula for dc conductivity: generalization to systems with spin-orbit coupling
- Robust magnetic proximity induced anomalous Hall effect in a room temperature van der Waals ferromagnetic semiconductor based 2D heterostructure
- Unusual ferromagnetic band evolution and high Curie temperature in monolayer 1T-CrTe2 on bilayer graphene
- Magnon dispersion in bilayers of two-dimensional ferromagnets
- Contrasting magnetic anisotropy in CrCl3 and CrBr3: A first-principles study
- Deteriorated Interlayer Coupling in Twisted Bilayer Cobaltites
- Magnetic proximity effect in superconductor/ferromagnet van der Waals heterostructures: dependence on the number of superconducting monolayers
- Field-induced spin polarization in lightly Cr-substituted layered antiferromagnet NiPS3
- Unconventional bias-dependent tunneling magnetoresistance in van der Waals ferromagnetic/semiconductor heterojunctions
- Pressure-tunable magnetic topological phases in magnetic topological insulator MnSb4Te7
- Observation of intrinsic crystal phase in bare CrI3 ferromagnetism
- Electrical control of topological 3Q state in intercalated van der Waals antiferromagnet Cox-TaS2
- Quartic asymmetric exchange for two-dimensional ferromagnets with trigonal prismatic symmetry
- Electrical tuning of the magnetic properties of 2D magnets: the case of
- Fingerprints of Universal Spin-Stiffness Jump in Two-Dimensional Ferromagnets
- Anomalous Tunneling Magnetoresistance Oscillation and Electrically Tunable Tunneling Anisotropic Magnetoresistance in Few-layer CrPS4
- Controllable Spin Current in van der Waals Ferromagnet Fe3GeTe2
- Electrically tunable Gilbert damping in van der Waals heterostructures of two-dimensional ferromagnetic metals and ferroelectrics
- Magnetism between magnetic adatoms on monolayer NbSe
- Giant Valley-Polarized Spin Splittings in Magnetized Janus Pt Dichalcogenides
- Electric and magnetic fields tuned spin-polarized topological phases in two-dimensional ferromagnetic MnBiTe
- Writing and detecting topological charges in exfoliated FeGeTe
- Artificially creating emergent interfacial antiferromagnetism and its manipulation in a magnetic van-der-Waals heterostructure
- Angular dependence of spin-orbit torque in monolayer
- Kagome surface states and weak electronic correlation in vanadium-kagome metals
- An effective spin model on the honeycomb lattice for the description of magnetic properties in two-dimensional FeGeTe
- Dimensional crossover of charge order in IrTe with strong interlayer coupling
- Epitaxial growth of bilayer Bi(110) on two-dimensional ferromagnetic Fe3GeTe2
- Theoretical realization of rich magnon topology by symmetry-breaking in honeycomb bilayer ferromagnets
- Probing Short-Range Correlations in the van der Waals Magnet CrSBr by Small-Angle Neutron Scattering
- Flat bands and magnetism in and due to bipartite crystal lattices
- Topological magnon-polarons in honeycomb antiferromagnets with spin-flop transition
- MXene Fe2C as a promising candidate for the 2D XY ferromagnet
- Strong band-filling-dependence of the scattering lifetime in gated MoS2 nanolayers induced by the opening of intervalley scattering channels
- Defect complexes in CrSBr revealed through electron microscopy and deep learning
- Optical Switching of Moiré Chern Ferromagnet
- Anomalous valley Hall effect in monolayer chromium-based triple-Q magnets
- Spin-polarized supercurrent through the van der Waals Kondo lattice ferromagnet FeGeTe
- Stacking-induced magnetic frustration and spiral spin liquid
- Two-Dimensional Altermagnetic Iron Oxyhalides: Real Chern Topology and Valley-Spin-Lattice Coupling
- Frustrated ferromagnetic transition in AB-stacked honeycomb bilayer
- Microscopic mechanisms of Strong Electron Scattering and Giant Anomalous Hall Effect in high-Curie-temperature Fe3GaTe2 van der Waals Films
- Tunable moire spinons in magnetically encapsulated twisted van der Waals quantum spin-liquids
- Long-range anisotropic Heisenberg ferromagnets and electrically tunable ordering
- Kinetically-controlled epitaxial growth of FeGeTe van der Waals ferromagnetic films
- Gate-tunable nonlocal Josephson effect through magnetic van der Waals bilayers
- A DFT study of the structural and electronic properties of single and double acceptor dopants in MX2 monolayers
- Giant anisotropy of Gilbert damping in a Rashba honeycomb antiferromagnet
- Impact of inherent energy barrier on spin-orbit torques in magnetic-metal/semimetal heterojunctions
- Anomalous Hall and Nernst effects in the Two-Dimensional ferromagnetic metal FePd2Te2
- In-Plane Magnetic Anisotropy and Large topological Hall Effect in Self-Intercalated Ferromagnet Cr1.61Te2
- Gate-tunable Intrinsic Anomalous Hall Effect in Epitaxial MnBi2Te4 Films
- Manifestation of incoherent-coherent crossover and non-Stoner magnetism in the electronic structure of FeGeTe
- Resonant Tunneling Anisotropic Magnetoresistance Induced by Magnetic Proximity
- Graphendofullerene: a novel molecular two-dimensional ferromagnet
- Second-harmonic response as a tool to detect spin textures in magnetic nodal-line semimetal FeGeTe
- Jahn-Teller distortion driven ferromagnetism in a perovskite fluoride monolayer
- Van der Waals Layered Ferroelectric CuInP2S6: Physical Properties and Device Applications
- Unexpected large electrostatic gating by pyroelectric charge accumulation
- 2D hybrid CrCl2(N2C4H4)2 with tunable ferromagnetic half-metallicity
- Bias voltage controlled inversions of tunneling magnetoresistance in van der Waals heterostructures Fe3GaTe2/hBN/Fe3GaTe2
- The influence of Ga doping on magnetic properties, magnetocaloric effect, and electronic structure of pseudo-binary GdZn1-xGax (x = 0-0.1)
- In-situ scanning tunneling microscopy observation of thickness-dependent air-sensitive layered materials and heterodevices
- Dynamically generated spin-interactions and nutational spin inertia in normal metal-ferromagnet heterostructures
- Electrically tunable room-temperature ferromagnetism in CrBr
- Spin-orbit Torque Switching in an All-Van der Waals Heterostructure
- Enhanced ferromagnetism in artificially stretched lattice in quasi two-dimensional Cr2Ge2Te6
- Stabilization of antiferromagnetism in 1T-FeTaS
- Magnetic domain wall dynamics under external electric field in bilayer CrI
- Facilitating field-free perpendicular magnetization switching with a Berry curvature dipole in a Weyl semimetal
- Metamagnetic Transitions in Few-Layer CrOCl Controlled by Magnetic Anisotropy Flipping
- Spin and lattice dynamics of a van der Waals antiferromagnet MnPSe
- Long Range Magnetic order stabilized by acceptors
- Edge non-collinear magnetism in nanoribbons of Fe3GeTe2 and Fe3GaTe2
- Spin waves in the bilayer van der Waals magnet CrSBr
- Van der Waals Magnet based Spin-Valve Devices at Room Temperature
- Tailoring coercive fields and the Curie temperature via proximity coupling in WSe/FeGeTe van der Waals heterostructures
- Computational studies on magnetism and ferroelectricity
- Nearly-room-temperature ferromagnetism and tunable anomalous Hall effect in atomically thin Fe4CoGeTe2
- Evidence for anisotropic spin-triplet Andreev reflection at the 2D van der Waals ferromagnet/superconductor interface
- Minority magnons and mode branching in monolayer FeGeTe
- Multiferroic Metallic Monolayer Cu(CrSe2)2
- Spin mapping of intralayer antiferromagnetism and spin-flop transition in monolayer CrTe
- Scratching lithography, manipulation, and soldering of 2D materials using microneedle probes
- Rashba spin-orbit coupling enhanced magnetoresistance in junctions with one ferromagnet
- Exotic spintronic properties of transition-metal monolayers on graphyne
- Hard ferromagnetism down to the thinnest limit of iron-intercalated tantalum disulfide
- Near room-temperature ferromagnetism from double-exchange in the van der Waals material CrGeTe: evidence from optical conductivity under pressure
- Tunable magnetic anisotropy, Curie temperature and band alignment of two-dimensional ferromagnet VSiSnN4 via non-volatile ferroelectrical control
- Air Stable and Layer Dependent Ferromagnetism in Atomically Thin van der Waals CrPS
- Room temperature energy-efficient spin-orbit torque switching in wafer-scale all-vdW heterostructure
- Physical properties of the layered -electron van der Waals magnet CeTe
- Optical fingerprints of the electronic band reconstruction in van der Waals magnetic materials
- Multi-Meron Interactions and Statistics in Two-Dimensional Materials
- Electron-doped magnetic Weyl semimetal LixCo3Sn2S2 by bulk-gating
- Monolayer FeGaX (X=I, Br, Sb): high-temperature two-dimensional magnets and a novel partially ordered spin state
- Phonon-induced renormalization of exchange interactions in metallic two-dimensional magnets
- Magnetic excitations and absence of charge order in the van der Waals ferromagnet FeGeTe
- High temperature antiferromagnetism in ultrathin SrRu2O6 nanosheets
- Quantum selection of order and dynamic properties of Kitaev-Heisenberg ferromagnet on a triangular lattice
- Strongly enhanced topological quantum phases in dual-surface AlO-encapsulated MnBiTe
- Electronic structures and magnetism in van der Waals flat-band material NiGeTe
- Emergent giant topological Hall effect in twisted Fe3GeTe2 metallic system
- Nonlinear Valley and Spin Valves in Bilayer Graphene
- Electronic Landscape of Group-5 Transition Metal Ditellurides Te ( = V, Nb, Ta): Multiple Crystal Phases with Local Bonds and Flat Bands
- The atlas of ferroicity in two dimensional MGeX3 family: room-temperature ferromagnetic half metals and unexpected ferroelectricity and ferroelasticity
- Spin transistor built on 2D van der Waals heterostructures
- Giant spin transfer torque in atomically thin magnetic bilayers
- Moiré spintronics: Emergent phenomena, material realization and machine learning accelerating discovery
- Uncovering A Two-Dimensional Semiconductor with Intrinsic Ferromagnetism at Room Temperature
- Long lifetimes of nanoscale skyrmions in lithium-decorated van der Waals ferromagnet FeGeTe
- Electric-field control of two-dimensional ferromagnetic properties by chiral ionic gating
- Large ferromagnetic-like band splitting in ultrathin films
- Probing the band structure of the strongly correlated antiferromagnet NiPS3 across its phase transition
- Scanning Tunneling Microscopy Study of Epitaxial Fe3GeTe2 Monolayers on Bi2Te3
- Enhanced Itinerant Ferromagnetism in Hole-doped Transition Metal Oxides: Beyond the Canonical Double Exchange Mechanism
- Thickness Dependent Magnetic Transition in Few Layer 1T Phase CrTe2
- Enhanced Valley Zeeman Splitting in Fe-Doped Monolayer MoS2
- Importance of Paramagnetic Background Subtraction for Determining the Magnetic Moment in Epitaxially Grown Monolayer and Few-Layer van der Waals Magnets
- Magnon Damping as a Probe of Kondo Coupling in Magnetically Ordered Systems
- Nitrogen-Vacancy Magnetometry of Edge Magnetism in WS2 Flakes
- Tunable linear and nonlinear anomalous Hall transport in two-dimensional CrPS
- Chromium chalcohalide Janus monolayer ferromagnets with perpendicular magnetic anisotropy and high Curie temperature
- AMaRaNTA: Automated First-Principles Exchange Parameters In 2D Magnets
- Highly tunable Gilbert damping in two-dimensional van der Waals ferromagnet Fe3GaTe2: From bilayer to the twisted bilayer
- Spin-orbit torque: Moving towards two-dimensional van der Waals heterostructures
- CrFe2Ge2: Investigation of novel ferromagnetic material of Fe13Ge8-type crystal
- Van der Waals Antiferromagnets: From Early Discoveries to Future Directions in the 2D Limit
- Spin-Orbit Torque and Magnetization Switching in 2D Ferromagnetic Devices
- Robustness of ferromagnetism in van der Waals magnet FeGeTe to hydrostatic pressure
- Reference lattice, sound, stiffness, and magnetic transitions of Ising monolayers
- Heisenberg-like critical behavior in the quasi-two-dimensional metallic ferromagnet LaCrSb3
- Computational Frameworks for Patterned Two-Dimensional Magnetism
- Gate-Tunable Superconducting Spin Valve in a van der Waals Ferromagnet/Superconductor/Ferromagnet Trilayer
- Quantum tunneling devices incorporating two-dimensional magnetic semiconductors
- Spontaneous Enhancement of Dzyaloshinskii-Moriya Interaction via Field-Cooling-Induced Interface Engineering in 2D van der Waals Ferromagnetic ternary Tellurides
- Symmetry-forbidden intraband transitions leading to ultralow Gilbert damping in van der Waals ferromagnets
- Electrostatic Control of Magneto-Optic Excitonic Resonances in the van der Waals Ferromagnetic Semiconductor CrGeTe
- Magnetic Field Dependent Piezoelectricity in Atomically Thin CoTe
- Noncentrosymmetric Nowotny Chimney Ladder Ferromagnet Cr4Ge7 with a High Curie Temperature of ~ 207 K
- Band Splitting and Long-lived Carrier Recombination in Ferromagnetic CrSiTe3 Nanosheets
- High Curie Temperature Ferromagnetic Semiconductor: Bimetal Transition Iodide VCrI
- Topological properties of multilayer magnon insulators
- Tailoring high-TN interlayer antiferromagnetism in a van der Waals itinerant magnet
- Epitaxial Growth and Band Structure of Antiferromagnetic Mott Insulator CeOI
- Spin scattering and Hall effects in monolayer Fe3GeTe2
- Quenching the Non-Collinear Spin Order in High-Tc Layered Ferromagnet Fe5GeTe2