Dynamical criticality of spin-shear coupling in van der Waals antiferromagnets

Abstract

The interplay between a multitude of electronic, spin, and lattice degrees of freedom underlies the complex phase diagrams of quantum materials. Layer stacking in van der Waals (vdW) heterostructures is responsible for exotic electronic and magnetic properties, which inspires stacking control of two-dimensional magnetism. Beyond the interplay between stacking order and interlayer magnetism, we discover a spin-shear coupling mechanism in which a subtle shear of the atomic layers can have a profound effect on the intralayer magnetic order in a family of vdW antiferromagnets. Using time-resolved x-ray diffraction and optical linear dichroism measurements, interlayer shear is identified as the primary structural degree of freedom that couples with magnetic order. The recovery times of both shear and magnetic order upon optical excitation diverge at the magnetic ordering temperature with the same critical exponent. The time-dependent Ginzburg-Landau theory shows that this concurrent critical slowing down arises from a linear coupling of the interlayer shear to the magnetic order, which is dictated by the broken mirror symmetry intrinsic to the monoclinic stacking. Our results highlight the importance of interlayer shear in ultrafast control of magnetic order via spin-mechanical coupling.

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• Terahertz field-induced metastable magnetization near criticality in FePS3
• Progress and Prospects in Two-Dimensional Magnetism of van der Waals Materials
• Identifying band structure changes of FePS3 across the antiferromagnetic phase transition
• Laser-induced Demagnetization in van der Waals $XY$- and Ising-like Antiferromagnets NiPS${}_3$ and FePS${}_3$
• Dynamical decoding of the competition between charge density waves in a kagome superconductor
• Time-domain study of coupled collective excitations in quantum materials
• Terahertz Control of Linear and Nonlinear Magno-Phononics
• Pressure-induced transitions in FePS${}_3$: Structural, magnetic and electronic properties
• Ultrafast Dynamics of Spin-Orbit Entangled Excitons Coupled to Magnetic Ordering in van der Waals Antiferromagnet NiPS3