Electrical Control of 2D Magnetism in Bilayer CrI3

Abstract

The challenge of controlling magnetism using electric fields raises fundamental questions and addresses technological needs such as low-dissipation magnetic memory. The recently reported two-dimensional (2D) magnets provide a new system for studying this problem owing to their unique magnetic properties. For instance, bilayer chromium triiodide (CrI3) behaves as a layered antiferromagnet with a magnetic field-driven metamagnetic transition. Here, we demonstrate electrostatic gate control of magnetism in CrI3 bilayers, probed by magneto-optical Kerr effect (MOKE) microscopy. At fixed magnetic fields near the metamagnetic transition, we realize voltage-controlled switching between antiferromagnetic and ferromagnetic states. At zero magnetic field, we demonstrate a time-reversal pair of layered antiferromagnetic states which exhibit spin-layer locking, leading to a remarkable linear dependence of their MOKE signals on gate voltage with opposite slopes. Our results pave the way for exploring new magnetoelectric phenomena and van der Waals spintronics based on 2D materials.

To appear in Nature Nanotechnology

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• Gate control of 2D magnetism in tri- and four-layers $\mathrm{Cr}{\mathrm{I}}_3$/graphene heterostructures
• Magnetic domain wall dynamics under external electric field in bilayer CrI${}_3$
• Tuning bulk topological magnon properties with light-induced magnons
• Noncollinearity-modulated electronic properties of the monolayer CrI${}_3$
• Interlayer superexchange in bilayer chromium trihalides
• Discovery of an ultrastable antiferromagnetic two-dimensional CrF3 phase with anisotropic quasi-one-dimensional mechanical, electronic, and thermal properties
• Dynamical response of noncollinear spin systems at constrained magnetic moments
• Pressure-driven switching of magnetism in layered CrCl3
• Linear and Nonlinear Edelstein Effects in Chiral Topological Semimetals
• Hard ferromagnetism down to the thinnest limit of iron-intercalated tantalum disulfide
• Two-Terminal Electrical Detection of the Néel Vector via Longitudinal Antiferromagnetic Nonreciprocal Transport
• Group Theory Analysis of Phonons in Monolayer Chromium Trihalides and Their Janus Structures
• Interface engineering of van der Waals heterostructures towards energy-efficient quantum devices operating at high temperatures
• Magnetic Moiré Systems: a review
• Nanoscale electronic transparency of wafer-scale hexagonal boron nitride
• Ligand Field Exciton Annihilation in Bulk CrCl3
• Spin textures in chiral magnetic monolayers with suppressed nearest-neighbor exchange
• Electronic excitations and spin interactions in chromium trihalides from embedded many-body wavefunctions
• Spin transistor built on 2D van der Waals heterostructures
• Giant spin transfer torque in atomically thin magnetic bilayers
• Electrical detection of magnetic circular dichroism: application to magnetic microscopy in ultra-thin ferromagnetic films
• Probing Hidden Symmetry and Altermagnetism with Sub-Picometer Sensitivity via Nonlinear Transport
• Exploring van der Waals cuprate superconductors using a hybrid microwave circuit
• Phonon-induced renormalization of exchange interactions in metallic two-dimensional magnets
• Magnetoelectric torque in polar magnetic bilayers
• Spin pumping effect in non-Fermi liquid metals
• Effect of spin-dependent tunneling and intervalley scattering in magnetic-semiconductor van der Waals heterostructures on exciton and trion polarization
• Moiré magnetism in a bilayer Ising model
• Space-Charge-Limited van der Waals Spin Transistor
• Moiré spintronics: Emergent phenomena, material realization and machine learning accelerating discovery
• Spin-orbit torque: Moving towards two-dimensional van der Waals heterostructures
• Light-induced ultrafast magnetization dynamics in van der Waals antiferromagnetic CrSBr
• Large ferromagnetic-like band splitting in ultrathin ${\mathrm{SmC}}_6$ films
• Laser-Irradiated CrI${}_3$: When Chiral Photons Meet Topological Magnons
• An ab initio description of the family of Cr selenides: structure, magnetism and electronic structure from bulk to the single-layer limit
• Magnetic Proximity Effect in 2D Ferromagnetic CrBr3/Graphene van der Waals Heterostructures
• Tunable Magneto-optical Kerr effect in two-dimensional non-collinear antiferromagnetic material HfFeCl6
• Tailoring high-TN interlayer antiferromagnetism in a van der Waals itinerant magnet
• All-Optical Generation of Antiferromagnetic Magnon Currents via the Magnon Circular Photogalvanic Effect
• Unprecedented Spin-Lifetime of Itinerant Electrons in Natural Graphite Crystals
• Band Splitting and Long-lived Carrier Recombination in Ferromagnetic CrSiTe3 Nanosheets
• Current-induced CrI3 surface spin-flop transition probed by proximity magnetoresistance in Pt
• Detecting and Distinguishing Majorana Zero Modes with the Scanning Tunneling Microscope
• Valley-Polarized Quantum Anomalous Hall Phase in Bilayer Graphene with Layer-Dependent Proximity Effects
• Orbital Longitudinal Magneto-electric Coupling in Multilayer Graphene
• Electrical Modulation and Probing of Antiferromagnetism in Hybrid Multiferroic Heterostructures
• Spontaneous Enhancement of Dzyaloshinskii-Moriya Interaction via Field-Cooling-Induced Interface Engineering in 2D van der Waals Ferromagnetic ternary Tellurides
• Spin scattering and Hall effects in monolayer Fe3GeTe2
• Valence Modifications in Hygroscopic VI3 Degraded Crystals via Soft X-Ray Synchrotron Radiation
• Electrostatic Control of Magneto-Optic Excitonic Resonances in the van der Waals Ferromagnetic Semiconductor Cr${}_2$Ge${}_2$Te${}_6$
• Emergent exotic chirality dependent dielectricity in magnetic twisted bilayer system
• Environmental Screening and Ligand-Field Effects to Magnetism in CrI${}_3$ Monolayer
• Energetically Favored One-Dimensional Moiré Superstructure in the Pseudo-Square Lattice GdTe3
• Skyrmion generation via Laguerre-Gaussian beam irradiation in frustrated magnets
• High Curie Temperature Ferromagnetic Semiconductor: Bimetal Transition Iodide V${}_2$Cr${}_2$I${}_9$
• Orbital mixing and strong Hund's coupling stabilize spin order in van der Waals ferromagnet CrI3