Spin filtering in CrI${}_3$ tunnel junctions

Abstract

The recently discovered magnetism of two-dimensional (2D) van der Waals crystals have attracted a lot of attention. Among these materials is CrI${}_3$ - a magnetic semiconductor exhibiting transitions between antiferromagnetic and ferromagnetic orderings under the influence of an applied magnetic field. Here, using first-principles methods based on density functional theory, we explore spin-dependent transport in tunnel junctions formed of fcc Cu (111) electrodes and a CrI${}_3$ tunnel barrier. We find about 100% spin polarization of the tunneling current for a ferromagnetically-ordered four-monolayer CrI${}_3$ and tunneling magnetoresistance of about 3,000% associated with a change of magnetic ordering in CrI${}_3$. This behavior is understood in terms of the spin and wave-vector dependent evanescent states in CrI${}_3$ which control the tunneling conductance. We find a sizable charge transfer from Cu to CrI${}_3$ which adds new features to the mechanism of spin-filtering in CrI${}_3$-based tunnel junctions. Our results elucidate the mechanisms of spin filtering in CrI3 tunnel junctions and provide important insights for the design of magnetoresistive devices based on 2D magnetic crystals.

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