Realizing a lattice spin model with polar molecules
arXiv:1305.5598 · doi:10.1038/nature12483
Abstract
With the recent production of polar molecules in the quantum regime, long-range dipolar interactions are expected to facilitate the understanding of strongly interacting many-body quantum systems and to realize lattice spin models for exploring quantum magnetism. In atomic systems, where interactions require wave function overlap, effective spin interactions on a lattice can be realized via superexchange; however, the coupling is weak and limited to nearest-neighbor interactions. In contrast, dipolar interactions exist in the absence of tunneling and extend beyond nearest neighbors. This allows coherent spin dynamics to persist even at high entropy and low lattice filling. Effects of dipolar interactions in ultracold molecular gases have so far been limited to the modification of chemical reactions. We now report the observation of dipolar interactions of polar molecules pinned in a 3D optical lattice. We realize a lattice spin model with spin encoded in rotational states, prepared and probed by microwaves. This spin-exchange interaction arises from the resonant exchange of rotational angular momentum between two molecules. We observe clear oscillations in the evolution of the spin coherence in addition to an overall decay. The frequency of these oscillations, the strong dependence of the spin coherence time on the lattice filling, and the effect of a multi-pulse sequence designed to reverse dynamics due to two-body exchange interactions all provide evidence of dipolar interactions. We also demonstrate suppression of loss in weak lattices due to a quantum Zeno mechanism. Measurements of these tunneling-induced losses allow us to independently determine the lattice filling factor. These results comprise an initial exploration of the behavior of many-body spin models with direct, long-range spin interactions and lay the groundwork for future studies of many-body dynamics in spin lattices.
18 pages, 6 figures
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- Interaction-driven Lifshitz transition with dipolar fermions in optical lattices
- Efficient Pathway to NaCs Ground State Molecules
- Effective spin-spin interactions in bilayers of Rydberg atoms and polar molecules
- Superfluidity and solid orders in two-component Bose gas with dipolar interactions in an optical lattice
- Entanglement entropy of the long-range Dyson hierarchical model
- Hidden Magnetism in Periodically Modulated One Dimensional Dipolar Fermions
- Interactions of benzene, naphthalene, and azulene with alkali-metal and alkaline-earth-metal atoms for ultracold studies
- Enhanced quantum state transfer via feedforward cancellation of optical phase noise
- General classification of qubit encodings in ultracold diatomic molecules
- Disconnecting a Traversable Wormhole: Universal Quench Dynamics in Random Spin Models
- Versatile electric fields for the manipulation of ultracold NaK molecules
- Coherent optical nano-tweezers for ultra-cold atoms
- Tuneable defect interactions and supersolidity in dipolar quantum gases on a lattice potential
- A Nonequilibrium quantum phase transition in strongly coupled spin chains
- Quantum walk and Anderson localization of rotational excitations in disordered ensembles of polar molecules
- Variational approach to the dynamics of dissipative quantum impurity models
- Rotational-state dependence of interactions between polar molecules
- Multidimensional Spectroscopy of Time-Dependent Impurities in Ultracold Fermions
- Feasibility of Kitaev quantum spin liquids in ultracold polar molecules
- Fast high-fidelity multi-qubit state transfer with long-range interactions
- Quantum Atom Optics: Theory and Applications to Quantum Technology
- Prospects of forming high-spin polar molecules from ultracold atoms
- Homogeneous and domain wall topological Haldane conductors with dressed Rydberg atoms
- Characterizing the phase diagram of finite-size dipolar Bose-Hubbard systems
- String order via Floquet interactions in atomic systems
- Exactly soluble model of boundary degeneracy
- Quantum few-body bound states of dipolar particles in a helical geometry
- Few-body physics of ultracold atoms and molecules with long-range interactions
- Transverse instability and universal decay of spin spiral order in the Heisenberg model
- A general Zeeman slower for type-II transitions and polar molecules
- Universality and two-body losses: lessons from the effective non-Hermitian dynamics of two particles
- Bilayer fractional quantum Hall states with ultracold dysprosium
- Unconventional symmetries of Fermi liquid and Cooper pairing properties with electric and magnetic dipolar fermions
- Realization of Heisenberg models of spin systems with polar molecules in pendular states
- A general approach to state-dependent optical tweezer traps for polar molecules
- Expedited thermalization dynamics in incommensurate systems
- Fermionic non-Abelian fractional Chern insulators from dipolar interactions
- Spin and density self-ordering in dynamic polarization gradients fields
- A quantum Monte Carlo study of the long-ranged site-diluted XXZ-model as realized by polar molecules
- Long-range interaction in an open boundary-driven Heisenberg spin lattice: A far-from-equilibrium transition to ballistic transport
- Quantum phases of hardcore bosons in two coupled chains: A density matrix renormalization group study
- Anisotropic Polarizability of Ultracold Ground-state NaRb Molecules
- Equilibrium phases of dipolar lattice bosons in the presence of random diagonal disorder
- Dynamics of ultracold dipolar particles in a confined geometry and tilted fields
- Transversal effects on the ground-state of hard-core dipolar bosons in one-dimensional optical lattices
- Spin dynamics dominated by superexchange via virtual molecules
- Quantum phase transitions in networks of Lipkin-Meshkov-Glick models
- Chiral topological phases in optical lattices without synthetic fields
- Quantum spiral spin-tensor magnetism
- Quantum phases of quadrupolar Fermi gases in coupled one-dimensional systems
- Tuning the Drude weight of Dirac-Weyl fermions in one-dimensional ring traps
- Nondestructive dispersive imaging of rotationally excited ultracold molecules
- Fulde-Ferrell-Larkin-Ovchinnikov pairing states of a polarized dipolar Fermi gas trapped in a one-dimensional optical lattice
- The effect of disorder on the phase diagrams of hard-core lattice bosons with cavity-mediated long-range and nearest-neighbor interactions
- Effect of long-range interactions on multipartite entanglement in Heisenberg chains
- Interaction-induced topological superconductivity in antiferromagnet-superconductor junctions
- Relaxation timescales and prethermalisation in d-dimensional long-range quantum spin models
- Long-lived multilevel coherences and spin-1 dynamics encoded in the rotational states of ultracold molecules
- Quantum walk versus classical wave: Distinguishing ground states of quantum magnets by spacetime dynamics
- The Role of Interspecies Interactions in the Preparation of a Low-entropy Gas of Polar Molecules in a Lattice
- Quench dynamics of dipolar fermions in a one-dimensional harmonic trap
- Correlation versus dissipation in a non-Hermitian Anderson impurity model
- Two-dimensional XY Ferromagnet Induced by Long-range Interaction
- Thermal Area Law in Long-Range Interacting Systems
- Temporal Talbot interferometer of strongly interacting molecular Bose-Einstein condensate
- Maximizing the capture velocity of molecular magneto-optical traps with Bayesian optimization
- Quantum reaction-limited reaction-diffusion dynamics of noninteracting Bose gases
- Topological phonons in arrays of ultracold dipolar particles
- Order-by-disorder and emergent Kosterlitz-Thouless phase in triangular Rydberg array
- Incommensurability effects on dipolar bosons in optical lattices
- Magnetic properties and quench dynamics of two interacting ultracold molecules in a trap
- Hubbard parameters for programmable tweezer arrays
- Geometric representation of spin correlations and applications to ultracold systems
- Lifetimes of local excitations in disordered dipolar quantum systems
- Dipolar bosons in one dimension: the case of longitudinal dipole alignment
- Floquet Hamiltonian Engineering of an Isolated Many-Body Spin System
- Nonequilibrium steady states of Bose-Einstein condensates with a local particle loss in double potential barriers
- Bounding the finite-size error of quantum many-body dynamics simulations
- Density-wave steady-state phase of dissipative ultracold fermions with nearest-neighbor interactions
- Time dependence of few-body Förster interactions among ultracold Rydberg atoms
- Near-threshold bound states of the dipole-dipole interaction
- A Model for Scattering with Proliferating Resonances: Many Coupled Square Wells
- Duality between disordered nodal semimetals and systems with power-law hopping
- Phase diagrams of the disordered Bose-Hubbard model with cavity-mediated long-range and nearest-neighbor interactions
- Anomalous Behavior of Magnetic Susceptibility Obtained by Quench Experiments in Isolated Quantum Systems
- Characterization of the lowest excited-state ro-vibrational level of NaRb
- Mimicking quantum correlation of a long-range Hamiltonian by finite-range interactions
- An in-situ method for measuring the non-linear response of a Fabry-Perot cavity
- Comprehensive characterization of an apparatus for cold electromagnetic dysprosium dipoles
- A generalized effective spin-chain formalism for strongly interacting spinor gases in optical lattice
- Phase diagram of non-Hermitian BCS superfluids in a dissipative asymmetric Hubbard model
- Dissipation induced transition between delocalization and localization in the three-dimensional Anderson model
- Quantum criticality in chains of planar rotors with dipolar interactions
- Beyond the Spin Model Approximation for Ramsey Spectroscopy
- Adiabatic state preparation of stripe phases with strongly magnetic atoms
- Exact Continuum Representation of Long-range Interacting Systems and Emerging Exotic Phases in Unconventional Superconductors
- Spin Squeezing with Itinerant Dipoles: A Case for Shallow Lattices
- Dipolar Bose-Hubbard Model in finite-size real-space cylindrical lattices
- Quantifying Entanglement in Cluster States Built with Error-Prone Interactions
- Reducing Collective Quantum State Rotation Errors with Reversible Dephasing
- Exactly solvable dynamics and signatures of integrability in an infinite-range many-body Floquet spin system
- Topological phase and lattice structures in spin chain models
- Excitations and impurity dynamics in a fermionic Mott insulator with nearest-neighbor interactions
- Spectral properties of Levy Rosenzweig-Porter model via supersymmetric approach
- Resonances in non-universal dipolar collisions
- Orthogonality catastrophe beyond bosonization from post-selection
- Decay rates and energies of free magnons and bound states in dissipative XXZ chains
- Bosonic molecules in a lattice: unusual fluid phase from multichannel interactions
- Symmetry-protected topological phase transitions and robust chiral order on a tunable zigzag lattice
- More current with less particles due to power-law hopping
- Momentum-selective pair creation of spin excitations in dipolar bilayers
- Single-particle localization in a two-dimensional Rydberg spin system
- Universal scaling at a pre-thermal dark state
- Reducing backaction when measuring temporal correlations in quantum systems
- Time optimal quantum state transfer in a fully-connected quantum computer
- Cluster truncated Wigner approximation for bond-disordered Heisenberg spin models
- Maximizing information obtainable by quantum sensors through the Quantum Zeno Effect
- Vibrational quenching of the electronic ground state in ThO in cold collisions with He
- Anti-Drude Metal of Bosons
- Classical crystal formation of dipoles in two dimensions
- Reactive collisions of two ultracold particles in a harmonic trap
- A low-cost four-component relativistic coupled cluster linear response theory based on perturbation sensitive natural spinors
- Spin-Depairing-Induced Exceptional Fermionic Superfluidity
- Class of codes correcting absorptions and emissions
- Transparent Electrodes for High E-Field Production Using A Buried ITO Layer
- Correlations generated from high-temperature states: nonequilibrium dynamics in the Fermi-Hubbard model
- String order in dipole-blockaded quantum liquids
- Localization of Pairs in One-Dimensional Quasicrystals with Power-Law Hopping
- Interacting in-plane molecular dipoles in a zig-zag chain
- Geometrically Frustrated Coarsening Dynamics in Spinor Bose-Fermi Mixtures
- Locality of gapped ground states in systems with power-law decaying interactions
- Spin Waves and Dielectric Softening of Polar Molecule Condensates
- Excitation transfer in disordered spin chains with long-range exchange interactions
- Collective Effects in Linear Spectroscopy of Dipole-Coupled Molecular Arrays
- Relaxation dynamics of an unlike spin pair system
- Triplet Superfluidity on a triangular ladder with dipolar fermions
- Rotational properties of two interacting cold polar molecules: linear, symmetric, and asymmetric tops
- Quantum simulation of long range quantum spin glass with strong area-law violation using trapped ions
- Clock Factorized Quantum Monte Carlo Method for Long-range Interacting Systems
- Quasi-molecular bosonic complexes -- a pathway to atomic analog of SQUID with controlled sensitivity
- Probing rotational decoherence with a trapped-ion planar rotor
- Scale-invariant phase transition of disordered bosons in one dimension
- Condensation to a strongly correlated dark fluid of two dimensional dipolar excitons
- Robust storage qubits in ultracold polar molecules
- Signatures of Integrability and Exactly Solvable Dynamics in an Infinite-Range Many-Body Floquet Spin System
- Dressed-State Spectroscopy and Magic Trapping of Microwave-Shielded NaCs Molecules
- Pair Approximating the Action For Molecular Rotations in Path Integral Monte Carlo
- String-Breaking Dynamics in Quantum Adiabatic and Diabatic Processes
- Lattice models with long-range and number-non-conserving interactions with Zeeman excitations of ultracold magnetic atoms
- DiPolMol-Py: A Python package for calculations for ground-state molecules
- Delocalization in two and three-dimensional Rydberg gases
- Measuring molecular electric dipoles using trapped atomic ions and ultrafast laser pulses
- Ferroelectric quantum phase transition with cold polar molecules
- Dissipative cooling of spin chains by a bath of dipolar particles
- Atom recoil in collectively interacting dipoles using quantized vibrational states
- On the complex behaviour of the density in composite quantum systems
- Many-body spin Hall effect with space-inversion symmetry
- Analogy between Boltzmann machines and Feynman path integrals
- Implementing a Fast Unbounded Quantum Fanout Gate Using Power-Law Interactions
- Ab-Initio Approach to Many-Body Quantum Spin Dynamics
- Long-range interactions from gauge fields via dimensional mismatch
- Efficient Learning of Long-Range and Equivariant Quantum Systems
- Absence of Landau damping in driven three-component Bose-Einstein condensate in optical lattices
- Superconductivity in doped planar Dirac insulators: A renormalization group study
- Itinerant ferromagnetism of a dipolar Fermi gas with Raman-induced spin-orbit coupling
- Energy diffusion in the long-range interacting spin systems
- Bounding the Classical Capacity of Multilevel Damping Quantum Channels
- Reaction-diffusion dynamics of the weakly dissipative Fermi gas
- Beating the natural Grover bound for low-energy estimation and state preparation
- Proposal for realizing quantum-spin systems on a two-dimensional square lattice with Dzyaloshinskii-Moriya interaction by Floquet engineering using Rydberg atoms
- Many body population trapping in ultracold dipolar gases
- Steady-State Quantum Zeno Effect of Driven-Dissipative Bosons with Dynamical Mean-Field Theory
- Exact Solvability Of Entanglement For Arbitrary Initial State in an Infinite-Range Floquet System
- Magnetic monopole induced polarons in atomic superlattices
- Detecting high-dimensional entanglement by randomized product projections
- Quantum Zeno blockade in optomechanical systems
- Bound states in two-dimensional Fermi systems with quadratic band touching
- Optical lattice quantum simulator of dynamics beyond Born-Oppenheimer
- Emission photon statistics in collectively interacting dipole atom arrays in the low-intensity limit
- Quantum Point Contact with Local Two-body Loss
- Multi-state detection and spatial addressing in a microscope for ultracold molecules
- Trapping and binding by dephasing
- Chiral phases and dynamics of dipoles in triangular optical ladders
- Ultracold coherent control of molecular collisions at a Förster resonance
- Lossy Quantum Defect Theory of Ultracold Molecular Collisions
- Microwave-assisted coherent control of ultracold polar molecules with a ladder-type rotational states
- Quantum walks assisted by particle number fluctuations
- Covariance-based method for eigenstate factorization and generalized singlets
- Nonlinear dynamics and energy transfer for two rotating dipoles in an external field: A three-dimensional analysis
- Roaming pathways and survival probability in real-time collisional dynamics of cold and controlled bialkali molecules
- Impurity and soliton dynamics in a Fermi gas with nearest-neighbor interactions
- Universal Aspects of High-Temperature Relaxation Dynamics in Random Spin Models
- Unfolding multi-particle quantum correlations hidden in decoherence
- Damping-free collective oscillations of a driven two-component Bose gas in optical lattices
- Lifshitz transition in the phase diagram of two-leg - ladder systems at low filling
- Energy-level statistics in strongly disordered systems with power-law hopping
- Two-state Bogoliubov theory of a molecular Bose gas
- Higher-order topological quantum paramagnets
- Clustering of steady-state correlations in open systems with long-range interactions
- Emergent Berezinskii-Kosterlitz-Thouless deconfinement in super-Coulombic plasmas
- Quantum walkers in a disordered lattice with power-law hopping
- Effect of spin-orbit coupling in one-dimensional quasicrystals with power-law hopping
- Narrowline Laser Cooling and Spectroscopy of Molecules via Stark States
- Fermi-Hubbard gas with three-body losses: symmetries and dark states
- Optimal quantum spatial search with one-dimensional long-range interactions
- Asymptotic behavior of correlation functions of one-dimensional polar-molecules on optical lattices
- Ramsey interferometry of Rydberg ensembles inside microwave cavities
- Quantum phases of hard-core dipolar bosons in coupled 1D optical lattices
- Bosonic Haldane insulator in the presence of local disorder: A quantum Monte Carlo study
- Programmable order by disorder effect and underlying phases through dipolar quantum simulators
- Bogoliubov theory of a Bose-Einstein condensate of rigid rotor molecules
- Spin and thermal current scaling at a -junction of XX spin chains
- Electric-Field Control of Josephson Oscillations in Dipolar Bose-Einstein Condensates
- Scalable platform for qudit-based quantum computing using polar molecules
- Control of Dipolar Dynamics by Geometrical Programming
- Hyperfine van der Waals repulsion between open-shell polar molecules
- Metastable ferromagnetic clusters in dissipative many-body systems of polar molecules
- Topological floating phase of dipolar bosons in an optical ladder
- Floquet thermalization by power-law induced permutation symmetry breaking
- Persistence of the Berezinskii-Kosterlitz-Thouless transition with long-range couplings
- Quantum optimal control of the Dicke manifold in dipolar Rydberg atom arrays
- Metal-Insulator Coexistence and Gap-Crossing Domain-Wall Modes in an Aubry-André Model with Nonlocal Hopping
- Bose-Hubbard model with power-law hopping in one dimension
- Suppression of the horizon effect in pairing correlation functions of - chains after a quantum quench
- Stabilizing confined quasiparticle dynamics in one-dimensional polar lattice gases
- Adiabatic Quantum Zeno Dynamics of Bosonic Atom Pairs with Large Inelastic Losses
- Simultaneous Zeeman deceleration of polyatomic free radical with lithium atoms