Laser cooled molecules
arXiv:2103.00968 · doi:10.1016/bs.aamop.2021.04.003
Abstract
The last few years have seen rapid progress in the application of laser cooling to molecules. In this review, we examine what kinds of molecules can be laser cooled, how to design a suitable cooling scheme, and how the cooling can be understood and modelled. We review recent work on laser slowing, magneto-optical trapping, sub-Doppler cooling, and the confinement of molecules in conservative traps, with a focus on the fundamental principles of each technique. Finally, we explore some of the exciting applications of laser-cooled molecules that should be accessible in the near term.
arXiv commentReview article prepared for Advances in Atomic, Molecular & Optical Physics. 119 pages, 27 figures
References in corpus (164)
- Quantum phase transition from a superfluid to a Mott insulator in a gas of ultracold atoms
- A High Phase-Space-Density Gas of Polar Molecules
- Search for New Physics with Atoms and Molecules
- Quantum computation with trapped polar molecules
- Cold and Ultracold Molecules: Science, Technology, and Applications
- A toolbox for lattice spin models with polar molecules
- Realizing a lattice spin model with polar molecules
- Quantum-State Controlled Chemical Reactions of Ultracold KRb Molecules
- An atom-by-atom assembler of defect-free arbitrary 2d atomic arrays
- Experimental realization of a long-range antiferromagnet in the Hubbard model with ultracold atoms
- High-fidelity quantum logic gates using trapped-ion hyperfine qubits
- High-fidelity two-qubit quantum logic gates using trapped calcium-43 ions
- Laser cooling of a diatomic molecule
- Varying constants, Gravitation and Cosmology
- Strongly correlated 2D quantum phases with cold polar molecules: controlling the shape of the interaction potential
- Cold molecules: Progress in Quantum Engineering of Chemistry and Quantum Matter
- Magneto-optical trapping of a diatomic molecule
- A precision measurement of the electron's electric dipole moment using trapped molecular ions
- The Buffer Gas Beam: An Intense, Cold, and Slow Source for Atoms and Molecules
- Magneto-optical trapping of diatomic molecules
- Molecules cooled below the Doppler limit
- Environmental Dependence of Masses and Coupling Constants
- Cold Molecule Spectroscopy for Constraining the Evolution of the Fine Structure Constant
- Tunable Superfluidity and Quantum Magnetism with Ultracold Polar Molecules
- Schemes for robust quantum computation with polar molecules
- Laser cooling and slowing of CaF molecules
- An Optical Tweezer Array of Ultracold Molecules
- Molecules Near Absolute Zero and External Field Control of Atomic and Molecular Dynamics
- Precision Measurement of Time-Reversal Symmetry Violation with Laser-Cooled Polyatomic Molecules
- Sisyphus Laser Cooling of a Polyatomic Molecule
- Radio Frequency Magneto-Optical Trapping of CaF with High Density
- Coherence and Raman sideband cooling of a single atom in an optical tweezer
- Building one molecule from a reservoir of two atoms
- Laser Cooling of Optically Trapped Molecules
- 3-D Magneto-Optical Trap of Yttrium Monoxide
- Universal rate constants for reactive collisions of ultracold molecules
- Stable Topological Superfluid Phase of Ultracold Polar Fermionic Molecules
- Realizing Fractional Chern Insulators with Dipolar Spins
- Ultracold molecules for measuring the electron's electric dipole moment
- Improved limits for violations of local position invariance from atomic clock comparisons
- Direct observation of bimolecular reactions of ultracold KRb molecules
- Dipolar Exchange Quantum Logic Gate with Polar Molecules
- Many-body dynamics of dipolar molecules in an optical lattice
- Radiative force from optical cycling on a diatomic molecule
- Holographic generation of micro-trap arrays for single atoms
- Magneto-Optical Trap for Polar Molecules
- Destabilization of dark states and optical spectroscopy in Zeeman-degenerate atomic systems
- Seconds-scale coherence in a tweezer-array optical clock
- Direct Laser Cooling of a Symmetric Top Molecule
- Sub-millikelvin dipolar molecules in a radio-frequency magneto-optical trap
- Laser radiation pressure slowing of a molecular beam
- Magneto-electrostatic trapping of ground state OH molecules
- Optoelectrical cooling of polar molecules to sub-millikelvin temperatures
- Robust encoding of a qubit in a molecule
- Universal gates based on targeted phase shifts in a 3D neutral atom array
- Ultracold polar molecules as qudits
- Laser-Cooled Polyatomic Molecules for Improved Electron Electric Dipole Moment Searches
- Polyatomic candidates for cooling of molecules with lasers from simple theoretical concepts
- Measuring the electric dipole moment of the electron in BaF
- Ultracold molecules for quantum simulation: rotational coherences in CaF and RbCs
- Quantum Dynamics of Ultracold Na + Na_2 collisions
- Microwave shielding of ultracold polar molecules
- Second-Scale Nuclear Spin Coherence Time of Trapped Ultracold NaK Molecules
- -Enhanced Imaging of Molecules in an Optical Trap
- Λ-enhanced Sub-Doppler Cooling of Lithium Atoms in D1 Gray Molasses
- Magnetically-Trapped Molecules Efficiently Loaded from a Molecular MOT
- Resonant collisional shielding of reactive molecules using electric fields
- Polyatomic Molecules as Quantum Sensors for Fundamental Physics
- Magnetic trapping and coherent control of laser-cooled molecules
- Design for a fountain of YbF molecules to measure the electron's electric dipole moment
- Ultracold molecules: new probes on the variation of fundamental constants
- Dipolar evaporation of reactive molecules to below the Fermi temperature
- Collisional Cooling of Ultracold Molecules
- Observation of Collisions between Two Ultracold Ground-State CaF Molecules
- Quasi-Universal Dipolar Scattering in Cold and Ultracold Gases
- Controlling the scattering length of ultracold dipolar molecules
- Ultracold Rb-OH collisions and prospects for sympathetic cooling
- Rotational state microwave mixing for laser cooling of complex diatomic molecules
- 1D Magneto-Optical Trap of Polyatomic Molecules
- Deceleration of neutral molecules in macroscopic traveling traps
- Laser cooling of molecules
- A search for varying fundamental constants using Hz-level frequency measurements of cold CH molecules
- Suppression of inelastic collisions of polar state molecules in an electrostatic field
- Grey-molasses optical-tweezer loading: Controlling collisions for scaling atom-array assembly
- A Scalable Quantum Computing Platform Using Symmetric-Top Molecules
- Demonstration of a Sensitive Method to Measure Nuclear Spin-Dependent Parity Violation
- Magneto-optical trapping forces for atoms and molecules with complex level structures
- Deep laser cooling and efficient magnetic compression of molecules
- Molecular lattice clock with long vibrational coherence
- Universal ultracold collision rates for polar molecules of two alkali-metal atoms
- High accuracy theoretical investigations of CaF, SrF, and BaF and implications for laser-cooling
- Probing weak force induced parity violation by high resolution mid-infrared molecular spectroscopy
- A robust entangling gate for polar molecules using magnetic and microwave fields
- Molecular Asymmetry and Optical Cycling: Laser Cooling Asymmetric Top Molecules
- Prospects for Quantum Computing with an Array of Ultracold Polar Paramagnetic Molecules
- Continuous Centrifuge Decelerator for Polar Molecules
- An intense, cold, velocity-controlled molecular beam by frequency-chirped laser slowing
- Characteristics of a magneto-optical trap of molecules
- State-to-state control of ultracold molecular reactions
- Universal model for exoergic bimolecular reactions and inelastic processes
- Forming a single molecule by magnetoassociation in an optical tweezer
- Synthetic dimensions in ultracold molecules: quantum strings and membranes
- On the Prospects for Laser Cooling of TlF
- Molecular assembly of ground state cooled single atoms
- Dispersion interactions and reactive collisions of ultracold polar molecules
- Coupling ultracold atoms to a superconducting coplanar waveguide resonator
- Three-dimensional Doppler, polarization-gradient, and magneto-optical forces for atoms and molecules with dark states
- Improved magneto-optical trapping of a diatomic molecule
- Extending rotational coherence of interacting polar molecules in a spin-decoupled magic trap
- Magnetic Trapping of Molecules via Optical Loading and Magnetic Slowing
- Shielding ultracold dipolar molecular collisions with electric fields
- Methods for measuring the electron EDM using ultracold YbF molecules
- Magnetic Trapping of Cold Methyl Radicals
- Quantum interference-enhanced deep sub-Doppler cooling of 39 K atoms in gray molasses
- Modeling magneto-optical trapping of CaF molecules
- Spectroscopic characterization of aluminum monofluoride with relevance to laser cooling and trapping
- Buffer-gas cooling, high-resolution spectroscopy and optical cycling of barium monofluoride molecules
- Long term measurement of the Sr clock frequency at the limit of primary Cs clocks
- Collisions Between Ultracold Molecules and Atoms in a Magnetic Trap
- Measurement of the variation of electron-to-proton mass ratio using ultracold molecules produced from laser-cooled atoms
- Trapping of molecular Oxygen together with Lithium atoms
- Surface-induced heating of cold polar molecules
- Structures, Branching Ratios and Laser Cooling Scheme for 138BaF Molecule
- Modeling sympathetic cooling of molecules by ultracold atoms
- A molecular fountain
- Optical cycling, radiative deflection and laser cooling of barium monohydride (BaH)
- A Moving Magnetic Trap Decelerator: a New Source for Cold Atoms and Molecules
- Zeeman-tuned rotational level-crossing spectroscopy in a diatomic free radical
- Ultracold spin-polarized mixtures of 2Sigma molecules with S-state atoms: Collisional stability and implications for sympathetic cooling
- Coherent Bichromatic Force Deflection of Molecules
- Enhanced -violating nuclear magnetic quadrupole moment effects in laser-coolable molecules
- Coupling Rydberg atoms to microwave fields in a superconducting coplanar waveguide resonator
- Prospects for laser cooling of polyatomic molecules with increasing complexity
- The prospects of sympathetic cooling of NH molecules with Li atoms
- Theoretical study of YbOH to search for the nuclear magnetic quadrupole moment
- Optical shielding of destructive chemical reactions between ultracold ground-state NaRb molecules
- Prospects for rapid deceleration of small molecules by optical bichromatic forces
- Franck-Condon tuning of optical cycling centers by organic functionalization
- The Hyperfine Molecular Hubbard Hamiltonian
- Sideband cooling of molecules in optical traps
- Prospects for a Narrow Line MOT in YO
- Long rotational coherence times of molecules in a magnetic trap
- Laser cooling and magneto-optical trapping of molecules analyzed using optical Bloch equations and the Fokker-Planck-Kramers equation
- Observation and laser spectroscopy of ytterbium monomethoxide, YbOCH
- Precision measurements with polar molecules: the role of the black body radiation
- Radiation Pressure Force from Optical Cycling on a Polyatomic Molecule
- Principles and design of a Zeeman-Sisyphus decelerator for molecular beams
- Cold atomic and molecular collisions: approaching the universal loss regime
- A Zeeman slower for diatomic molecules
- The effect of hyperfine interactions on ultracold molecular collisions: NH(^3Sigma^-) with Mg(^1S) in magnetic fields
- Direct frequency comb laser cooling and trapping
- Deflection of a Molecular Beam Using the Bichromatic Stimulated Force
- Emulating optical cycling centers in polyatomic molecules
- Bright, continuous beams of cold free radicals
- Stark deceleration of CaF molecules in strong- and weak-field seeking states
- Enhancing dipolar interactions between molecules using state-dependent optical tweezer traps
- The Molecular Hubbard Hamiltonian: Field Regimes and Molecular Species
- Suppressed spontaneous emission for coherent momentum transfer
- Large molasses-like cooling forces for molecules using polychromatic optical fields: A theoretical description
- Ultracold Chemistry and its Reaction Kinetics
- Observation of Microwave Shielding of Ultracold Molecules
- A general Zeeman slower for type-II transitions and polar molecules
- A general approach to state-dependent optical tweezer traps for polar molecules
- Frequency-doubled Nd:YAG MOPA laser system with programmable rectangular pulses up to 200 microseconds
Cited by in corpus (45)
- Quantum state manipulation and cooling of ultracold molecules
- Opportunities for Fundamental Physics Research with Radioactive Molecules
- Ultracold Sticky Collisions: Theoretical and Experimental Status
- Measuring the stability of fundamental constants with a network of clocks
- Laser cooling for quantum gases
- Quantum control of molecules for fundamental physics
- An ultracold molecular beam for testing fundamental physics
- Optical cycling of AlF molecules
- Deceleration and trapping of SrF molecules
- Characterizing the Fundamental Bending Vibration of a Linear Polyatomic Molecule for Symmetry Violation Searches
- Efficient conversion of closed-channel dominated Feshbach molecules of NaK to their absolute ground state
- Benchmarking of the Fock space coupled cluster method and uncertainty estimation: Magnetic hyperfine interaction in the excited state of BaF
- Absorption spectroscopy for laser cooling and high-fidelity detection of barium monofluoride molecules
- Ultracold LiCr: a new pathway to quantum gases of paramagnetic polar molecules
- Engineering field-insensitive molecular clock transitions for symmetry violation searches
- Intensity-borrowing mechanisms pertinent to laser cooling of linear polyatomic molecules
- Accurate theoretical determination of the ionization potentials of CaF, SrF, and BaF
- Laser cooling of barium monofluoride molecules using synthesized optical spectra
- Optical cycling in polyatomic molecules with complex hyperfine structure
- Characterizing the Zeeman slowing force for CaF molecules
- Collisions in a dual-species magneto-optical trap of molecules and atoms
- Laser cooling of molecules
- Isotopologue-selective laser cooling of molecules
- Hyperfine structure of the state of AlCl and its relevance to laser cooling and trapping
- Direct measurement of high-lying vibrational repumping transitions for molecular laser cooling
- Intercombination line photoassociation spectroscopy of RbYb
- Laser cooled 137BaF molecules for measuring nuclear-spin-dependent parity violation
- Molecular laser cooling using serrodynes: Implementation, characterization and prospects
- An Electro-Optical Trap for Polar Molecules
- High-resolution spectroscopy of barium monofluoride: Odd isotopologues, hyperfine structure and isotope shifts
- Wavelength modulation laser spectroscopy of NO at 17 m
- Low-noise environment for probing fundamental symmetries
- Magnetic hyperfine structure constants of BaF in the and excited states
- A novel method to determine the phase-space distribution of a pulsed molecular beam
- Production and spectroscopy of cold radioactive molecules
- Ground-state selection via many-body superradiant decay
- Engineered Molecular Clock Transitions for Symmetry Violation Searches
- Measurement of the Electric Dipole Moment of AlCl by Stark Level Spectroscopy
- Atomic Parity Violation: Standard Model Tests
- Narrowline Laser Cooling and Spectroscopy of Molecules via Stark States
- A stable 2 W continuous-wave 261.5 nm laser for cooling and trapping aluminum monochloride
- Radioactive Molecules as Laboratories of Fundamental Physics
- A survey of nuclear quadrupole deformation in order to estimate the nuclear MQM and its relative contribution to the atomic EDM
- Non-resonant cavity for intensity buildup of multiple lasers
- Automated Graph-Based Detection of Quantum Control Schemes: Application to Molecular Laser Cooling