Measurement of the variation of electron-to-proton mass ratio using ultracold molecules produced from laser-cooled atoms
arXiv:1908.08722 · doi:10.1038/s41467-019-11761-1
Abstract
Experimental techniques to manipulate cold molecules have seen great development in recent years. The precision measurements of cold molecules are expected to give insights into fundamental physics. We use a rovibrationally pure sample of ultracold KRb molecules to improve the measurement on the stability of electron-to-proton mass ratio (). The measurement is based upon a large sensitivity coefficient of the molecular spectroscopy, which utilizes a transition between nearly a degenerate pair of vibrational levels each associated with a different electronic potential. Observed limit on temporal variation of is year, which is better by a factor of five compared with the most stringent laboratory molecular limits to date. Further improvements should be straightforward, because our measurement was only limited by statistical errors.
arXiv comment10 pages, 4 figures
References in corpus (15)
- Cold and Ultracold Molecules: Science, Technology, and Applications
- The fundamental constants and their variation: observational status and theoretical motivations
- Frequency ratio of two optical clock transitions in Yb and constraints on the time-variation of fundamental constants
- A precision measurement of the electron's electric dipole moment using trapped molecular ions
- Improved limit on a temporal variation of from comparisons of Yb and Cs atomic clocks
- Precision Test of Mass Ratio Variations with Lattice-Confined Ultracold Molecules
- Coherent transfer of photoassociated molecules into the rovibrational ground state
- Stability of the proton-to-electron mass ratio
- Enhanced sensitivity to variation of in molecular spectra
- New limits on variation of the fine-structure constant using atomic dysprosium
- The coupling of the X and a states of KRb
- Ab initio calculation of the KRb dipole moments
- Blackbody radiation shift assessment for a lutetium ion clock
- Search for the electron electric dipole moment using -doublet levels in PbO
- Prospects for Narrow-line Cooling of KRb Molecules in Rovibrational Ground State
Cited by in corpus (29)
- Polyatomic Molecules as Quantum Sensors for Fundamental Physics
- Laser cooled molecules
- Enhanced Sensitivity to Ultralight Bosonic Dark Matter in the Spectra of the Linear Radical SrOH
- Long term measurement of the Sr clock frequency at the limit of primary Cs clocks
- Quantum control of molecules for fundamental physics
- Magnetic Feshbach resonances in collisions of NaK with K
- A terahertz vibrational molecular clock with systematic uncertainty at the level
- Diatomic molecules of alkali-metal and alkaline-earth-metal atoms: interaction potentials, dipole moments, and polarizabilities
- Ultracold molecules in the absolute ground state
- Molecular Collisions: from Near-cold to Ultra-cold
- Transition strength measurements to guide magic wavelength selection in optically trapped molecules
- Fourier transform spectroscopy, relativistic electronic structure calculation, and coupled-channel deperturbation analysis of the fully mixed and states of Cs
- Interaction potentials, electric moments, polarizabilities, and chemical reactions of YbCu, YbAg, and YbAu molecules
- Prospects of nuclear-coupled-dark-matter detection via correlation spectroscopy of I and Ca
- Diatomic rovibronic transitions as potential probes for proton-to-electron mass ratio across cosmological time
- Nondestructive dispersive imaging of rotationally excited ultracold molecules
- Prospect for precision quantum logic spectroscopy of vibrational overtone transitions in molecular oxygen ions
- Zeeman-Sisyphus Deceleration for Heavy Molecules with Perturbed Excited-State Structure
- Hyperfine structure of the state of AlCl and its relevance to laser cooling and trapping
- Laser cooled 137BaF molecules for measuring nuclear-spin-dependent parity violation
- Searching for New Fundamental Interactions via Isotopic Shifts in Molecular Lattice Clocks
- Accurate Determination of Blackbody Radiation Shifts in a Strontium Molecular Lattice Clock
- Quantum Sensing Using Atomic Clocks for Nuclear and Particle Physics
- High-resolution spectroscopy of barium monofluoride: Odd isotopologues, hyperfine structure and isotope shifts
- Magnetic hyperfine structure constants of BaF in the and excited states
- Varying fundamental constants cosmography
- Measurement of the Electric Dipole Moment of AlCl by Stark Level Spectroscopy
- High-sensitivity molecular spectroscopy of SrOH using magneto-optical trapping
- Simultaneous Zeeman deceleration of polyatomic free radical with lithium atoms