Probing photoinduced two-body loss of ultracold non-reactive bosonic NaRb and NaK molecules
arXiv:2103.00510 · doi:10.1103/PhysRevLett.127.163401
Abstract
We probe photo-induced loss for chemically stable bosonic NaRb and NaK molecules in chopped optical dipole traps where the molecules spend a significant time in the dark. We expect the effective two-body decay to be largely suppressed in chopped traps due to the small expected complex lifetimes of about s and s for NaRb and NaK respectively. However, instead we do observe near-universal loss even at the lowest chopping frequencies we can probe. Our data thus either suggest a so far unknown loss mechanism or a drastic underestimation of the complex lifetime by at least one to two orders of magnitude.
References in corpus (26)
- A High Phase-Space-Density Gas of Polar Molecules
- Quantum computation with trapped polar molecules
- Order of Magnitude Smaller Limit on the Electric Dipole Moment of the Electron
- Realizing a lattice spin model with polar molecules
- Quantum-State Controlled Chemical Reactions of Ultracold KRb Molecules
- Ultracold dense samples of dipolar RbCs molecules in the rovibrational and hyperfine ground state
- Ultracold Dipolar Gas of Fermionic NaK Molecules in their Absolute Ground State
- Cold molecules: Progress in Quantum Engineering of Chemistry and Quantum Matter
- Creation of ultracold RbCs molecules in the rovibrational ground state
- Creation of an ultracold gas of ground-state molecules
- A Fermi Degenerate Gas of Polar Molecules
- Reactions of ultracold alkali metal dimers
- New frontiers with quantum gases of polar molecules
- Direct observation of bimolecular reactions of ultracold KRb molecules
- Statistical Aspects of Ultracold Resonant Scattering
- Collisions of ultracold ^{23}Na^{87}Rb molecules with controlled chemical reactivities
- Photo-induced two-body loss of ultracold molecules
- Loss of ultracold RbCs molecules via optical excitation of long-lived two-body collision complexes
- Modeling the adiabatic creation of ultracold, polar molecules
- Collisions of ultracold molecules in bright and dark optical dipole traps
- A quasiclassical method for calculating the density of states of ultracold collision complexes
- Formation of Ultracold NaRb Feshbach Molecules
- Dipolar Collisions of Ultracold Ground-state Bosonic Molecules
- Product state control of bi-alkali chemical reactions
- Steering ultracold reactions through long-lived transient intermediates
- Formation of ultracold weakly bound dimers of bosonic
Cited by in corpus (38)
- Evaporation of microwave-shielded polar molecules to quantum degeneracy
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- Ultracold Gas of Dipolar NaCs Ground State Molecules
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- Microwave shielding of bosonic NaRb molecules
- A Feshbach resonance in collisions between ultracold ground state molecules
- Reactions Between Layer-Resolved Molecules Mediated by Dipolar Exchange
- Diatomic molecules of alkali-metal and alkaline-earth-metal atoms: interaction potentials, dipole moments, and polarizabilities
- Seconds-scale coherence on nuclear spin transitions of ultracold polar molecules in 3D optical lattices
- High density loading and collisional loss of laser cooled molecules in an optical trap
- Complexes formed in collisions between ultracold alkali-metal diatomic molecules and atoms
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- Hyperfine dependent atom-molecule loss analyzed by the analytic solution of few-body loss equations
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- Symmetry breaking in sticky collisions between ultracold molecules
- Microscopy of an ultranarrow Feshbach resonance using a laser-based atom collider: A quantum defect theory analysis
- Resonances in non-universal dipolar collisions
- Ultracold Interactions between Ions and Polar Molecules
- Engineering long-range interactions between ultracold atoms with light
- Trap-induced atom-ion complexes: a time-independent approach
- Dissipative Superfluidity in a Molecular Bose-Einstein Condensate
- Multichannel quantum defect theory with a frame transformation for ultracold atom-molecule collisions in magnetic fields
- Fate of thermalization of ultracold fermions with two-body dissipation
- Lossy Quantum Defect Theory of Ultracold Molecular Collisions
- A versatile apparatus for simultaneous trapping of multiple species of ultracold atoms and ions to enable studies of low energy collisions and cold chemistry
- CaF+CaF interactions in the ground and excited electronic states: implications for collisional losses
- Metastable ferromagnetic clusters in dissipative many-body systems of polar molecules
- Delta-Kick Collimation of Heteronuclear Feshbach Molecules
- Ab initio study of the reactivity of ultracold RbSrRbSr collisions
- Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics
- Ultracold polar molecules for quantum science and technology