Probing photoinduced two-body loss of ultracold non-reactive bosonic NaRb and NaK molecules
arXiv:2103.00510 · doi:10.1103/PhysRevLett.127.163401
Abstract
We probe photo-induced loss for chemically stable bosonic NaRb and NaK molecules in chopped optical dipole traps where the molecules spend a significant time in the dark. We expect the effective two-body decay to be largely suppressed in chopped traps due to the small expected complex lifetimes of about s and s for NaRb and NaK respectively. However, instead we do observe near-universal loss even at the lowest chopping frequencies we can probe. Our data thus either suggest a so far unknown loss mechanism or a drastic underestimation of the complex lifetime by at least one to two orders of magnitude.
References in corpus (13)
- A High Phase-Space-Density Gas of Polar Molecules
- Ultracold dense samples of dipolar RbCs molecules in the rovibrational and hyperfine ground state
- Ultracold Dipolar Gas of Fermionic NaK Molecules in their Absolute Ground State
- Cold molecules: Progress in Quantum Engineering of Chemistry and Quantum Matter
- Creation of ultracold RbCs molecules in the rovibrational ground state
- Reactions of ultracold alkali metal dimers
- New frontiers with quantum gases of polar molecules
- Collisions of ultracold ^{23}Na^{87}Rb molecules with controlled chemical reactivities
- Loss of ultracold RbCs molecules via optical excitation of long-lived two-body collision complexes
- Modeling the adiabatic creation of ultracold, polar molecules
- Collisions of ultracold molecules in bright and dark optical dipole traps
- Formation of Ultracold NaRb Feshbach Molecules
- Steering ultracold reactions through long-lived transient intermediates
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- Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics
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