Moiré Excitons in Van der Waals Heterostructures
arXiv:1807.03771 · doi:10.1038/s41586-019-0975-z
Abstract
In van der Waals (vdW) heterostructures formed by stacking two monolayer semiconductors, lattice mismatch or rotational misalignment introduces an in-plane moiré superlattice. While it is widely recognized that a moiré superlattice can modulate the electronic band structure and lead to novel transport properties including unconventional superconductivity and insulating behavior driven by correlations, its influence on optical properties has not been investigated experimentally. We present spectroscopic evidence that interlayer excitons are confined by the moiré potential in a high-quality MoSe2/WSe2 heterobilayer with small rotational twist. A series of interlayer exciton resonances with either positive or negative circularly polarized emission is observed in photoluminescence, consistent with multiple exciton states confined within the moiré potential. The recombination dynamics and temperature dependence of these interlayer exciton resonances are consistent with this interpretation. These results demonstrate the feasibility of engineering artificial excitonic crystals using vdW heterostructures for nanophotonics and quantum information applications.
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- Theory of coherent phonons coupled to excitons
- Confined Trions and Mott-Wigner States in a Purely Electrostatic Moiré Potential
- Thickness and twist angle dependent interlayer excitons in metal monochalcogenide heterostructures
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- Magic continuum in twisted bilayer square lattice with staggered flux
- Quantum Geometric Exciton Drift Velocity
- Multi-flavor Dirac fermions in Kekulé-distorted graphene bilayers
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- Tunable Interband Transitions in Twisted h-BN/Graphene Heterostructures
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- Theory of intervalley-coherent AFM order and topological superconductivity in tWSe
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- Non-bosonic moiré excitons
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- Twisting in h-BN bilayers and their angle-dependent properties
- Moiré induced electronic structure modifications in monolayer VS on Au(111)
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- Correlating 3D atomic defects and electronic properties of 2D materials with picometer precision
- Tuning color centers at a twisted interface
- AC-Stark Spectroscopy of Interactions between Moiré Excitons and Polarons
- Theory of interlayer exciton dynamics in 2D TMDCs Heterolayers under the influence of strain reconstruction and disorder
- Robustness of momentum-indirect interlayer excitons in MoS2/WSe2 heterostructure against charge carrier doping
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- Trion confinement in monolayer MoSe2 by carbon nanotube local gating
- Electrically tunable and enhanced nonlinearity of moiré exciton-polaritons in transition metal dichalcogenide bilayers
- Highly tunable quantum light from moiré trapped excitons
- Spatially mixed moiré excitons in two-dimensional van der Waals superlattices
- Moiré excitons in generalized Wigner crystals
- Exciton Transport under Periodic Potential in MoSe2/WSe2 Heterostructures
- Emergence of Meron Kekulé lattices in twisted Néel antiferromagnets
- Purely electronic model for exciton-polaron formation in moiré heterostructures
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- Robust Interlayer Exciton Interplay in Twisted van der Waals Heterotrilayer on a Broadband Bragg Reflector up to Room Temperature
- Valley-controlled many-body exciton interactions in monolayer WSe phototransistors
- Effective long-range attraction of moiré excitons under the influence of atomic reconstructions and anisotropic screening
- Moire-Engineered Excitonic Landscape and Phonon-Mediated Recombination in Twisted WSe2 Bilayers
- Quantum Geometry Driven Finite-Momentum Exciton Fluctuations in Flat-Band Systems
- Graphene as a Tunable Nonradiative Bath for Moiré Excitons
- Supermoiré-trapped quadrupolar exciton
- Interaction enhanced inter-site hoppings for holons and interlayer exciton insulators in moiré correlated insulators
- Quantum siphoning of finely spaced interlayer excitons in reconstructed MoSe2/WSe2 heterostructures
- Atomic Regional Superfluids in two-dimensional Moiré Time Crystals
- Manipulate Quantum Emission by Interface States between Multi-component Moiré Lattice and Metasurface
- Trion-phonon interaction in atomically thin semiconductors
- Non-local interactions and supersolidity of moiré excitons
- Phonon Renormalization in Reconstructed MoS Moiré Superlattices
- Magnetic and nematic order of Bose-Fermi mixtures in moiré superlattices of 2D semiconductors
- Observation of symmetry-protected selection rules in periodically driven quantum systems
- Moiré exciton dynamics and moiré exciton-phonon interaction in a WSe/MoSe heterobilayer
- Designer quantum matter in van der Waals heterostructures
- Observation of Anomalous Moiré Patterns
- Gate-modulated reflectance spectroscopy for detecting excitonic species in two-dimensional semiconductors
- Experimental realisation of Dual Periodicity Moiré Superlattice in a MoSe/WSe Heterobilayer
- Room temperature interlayer exciton valley polarization and valley Hall effect
- Localized Interlayer Excitons in MoSe2-WSe2 Heterostructures without a Moiré Potential
- Moiré potential, lattice corrugation, and band gap spatial variation in a twist-free MoS2/MoTe2 heterobilayer
- Exciton-Anyon Binding in Fractional Chern Insulators: Spectral Fingerprints
- Realization of Nearly Dispersionless Bands with Strong Orbital Anisotropy from Destructive Interference in Twisted Bilayer MoS2