Efficient single photon emission from a high-purity hexagonal boron nitride crystal
arXiv:1606.04124 · doi:10.1103/PhysRevB.94.121405
Abstract
Among a variety of layered materials used as building blocks in van der Waals heterostructures, hexagonal boron nitride (hBN) appears as an ideal platform for hosting optically-active defects owing to its large bandgap ( eV). Here we study the optical response of a high-purity hBN crystal under green laser illumination. By means of photon correlation measurements, we identify individual defects emitting a highly photostable fluorescence under ambient conditions. A detailed analysis of the photophysical properties reveals a high quantum efficiency of the radiative transition, leading to a single photon source with very high brightness. These results illustrate how the wide range of applications offered by hBN could be further extended to photonic-based quantum information science and metrology.
arXiv comment5 pages, 4 figures
References in corpus (17)
- Van der Waals heterostructures
- Boron nitride substrates for high-quality graphene electronics
- Photonic quantum technologies
- Light-emitting diodes by bandstructure engineering in van der Waals heterostructures
- Hexagonal boron nitride is an indirect bandgap semiconductor
- Chemical control of the charge state of nitrogen-vacancy centers in diamond
- Photo-induced Doping in Graphene/Boron Nitride Heterostructures
- Temperature Dependence of Wavelength Selectable Zero-Phonon Emission from Single Defects in Hexagonal Boron Nitride
- Surface-induced charge state conversion of nitrogen-vacancy defects in nanodiamonds
- Defect-related photoluminescence of hexagonal boron nitride
- Room temperature stable single-photon source
- Coupling of excitons and defect states in boron-nitride nanostructures
- Excitons and stacking order in h-BN
- Bright and photostable single-photon emitter in silicon carbide
- Narrow-band single-photon emission in the near infrared for quantum key distribution
- Single photon emission from ZnO nanoparticles
- Measuring the second order correlation function and the coherence time using random phase modulation
Cited by in corpus (77)
- Tunable and high purity room-temperature single photon emission from atomic defects in hexagonal boron nitride
- Color centers in hexagonal boron nitride monolayers: A group theory and ab-initio analysis
- Optical properties of atomically thin transition metal dichalcogenides: Observations and puzzles
- Optical Signatures of Quantum Emitters in Suspended Hexagonal Boron Nitride
- Revealing multiple classes of stable quantum emitters in hexagonal boron nitride with correlated cathodoluminescence, photoluminescence, and strain mapping
- Position-controlled quantum emitters with reproducible emission wavelength in hexagonal boron nitride
- Stark Tuning of Single-Photon Emitters in Hexagonal Boron Nitride
- Spin-Dependent Quantum Emission in Hexagonal Boron Nitride at Room Temperature
- Single spin resonance in a van der Waals embedded paramagnetic defect
- Defect states in hexagonal boron nitride: Assignments of observed properties and prediction of properties relevant to quantum computation
- Single photon emitters in hexagonal boron nitride: A review of progress
- Optical absorption and emission mechanisms of single defects in hexagonal boron nitride
- Single artificial atoms in silicon emitting at telecom wavelengths
- Single photon emission from graphene quantum dots at room temperature
- First-principles identification of single photon emitters based on carbon clusters in hexagonal boron nitride
- Narrowband quantum emitters over large spectral range with Fourier-limited linewidth in hexagonal boron nitride
- Cubic-scaling all-electron GW calculations with a separable density-fitting space-time approach
- Phonon-assisted emission and absorption of individual color centers in hexagonal boron nitride
- Wide-field spectral super-resolution mapping of optically active defects in hBN
- Direct observation of water mediated single proton transport between hBN surface defects
- Band gap measurements of monolayer h-BN and insights into carbon-related point defects
- Exciton-phonon coupling in the UV absorption and emission spectra of bulk hexagonal boron nitride
- Blue-Light-Emitting Color Centers in High-Quality Hexagonal Boron Nitride
- Coupling of deterministically activated quantum emitters in hexagonal boron nitride to plasmonic surface lattice resonances
- Magnetic imaging with spin defects in hexagonal boron nitride
- Coherent dynamics of multi-spin centers in hexagonal boron nitride
- Very Large and Reversible Stark Shift Tuning of Single Emitters in Layered Hexagonal Boron Nitride
- Two-photon interference from a quantum emitter in hexagonal boron nitride
- Single Photon Emitters in Boron Nitride: More Than a Supplementary Material
- Giant shift upon strain on the fluorescence spectrum of VN color centers in -BN
- Polarization and localization of single-photon emitters in hexagonal boron nitride wrinkles
- Origin of nonclassical light emission from defects in multi-layer hexagonal boron nitride
- Phonon-induced multi-color correlations in hBN single-photon emitters
- Engineering Quantum Light Sources with Flat Optics
- Carrier recombination mechanism at defects in wide band gap two-dimensional materials from first principles
- Organic molecules as origin of visible-range single photon emission from hexagonal boron nitride and mica
- Probing the Optical Dynamics of Quantum Emitters in Hexagonal Boron Nitride
- Cubic BN optical gap and intragap optically active defects
- An ultrastable and robust single-photon emitter in hexagonal boron nitride
- Quantum light in curved low dimensional hexagonal boron nitride systems
- Spatial and spectral dynamics in STEM hyperspectral imaging using random scan patterns
- Luminescent defects in a few-layer h-BN film grown by molecular beam epitaxy
- Acoustically modulated optical emission of hexagonal boron nitride layers
- Investigating the fast spectral diffusion of a quantum emitter in hBN using resonant excitation and photon correlations
- Phonon sidebands of color centers in hexagonal boron nitride
- Cathodoluminescence monitoring of quantum emitter activation in hexagonal boron nitride
- Possible nanophotonics applications of the defect in hexagonal boron nitride
- Top-down integration of a hBN quantum emitter in a monolithic photonic waveguide
- Fingerprinting quantum emitters in hexagonal boron nitride using strain
- Efficient Optical Quantification of Heterogeneous Emitter Ensembles
- Controlling Photoluminescence Spectra of hBN Color Centers by Selective Phonon-Assisted Excitation: A Theoretical Proposal
- Direct visualization and effects of atomic-scale defects on the optoelectronic properties of hexagonal boron nitride
- Time-dependent Mandel Q parameter analysis for a hexagonal boron nitride single photon source
- Quantum efficiency and vertical position of quantum emitters in hBN determined by Purcell effect in hybrid metal-dielectric planar photonic structures
- Observation and Spectral Assignment of a Family of Hexagonal Boron Nitride Lattice Defects
- Polarization study of single color centers in aluminum nitride
- Benchmarking the integration of hexagonal boron nitride crystals and thin films into graphene-based van der Waals heterostructures
- The effect of electron-phonon interactions on the spectral properties of single defects in hexagonal boron nitride
- Spontaneous emission of color centers at 4eV in hexagonal boron nitride under hydrostatic pressure
- Photon statistics analysis of h-BN quantum emitters with pulsed and continuous-wave excitation
- Magnetic-field dependent VB- spin decoherence in hexagonal boron nitrides: A first-principles study
- Large-Scale Statistical Analysis of Defect Emission in hBN: Revealing Spectral Families and Influence of Flakes Morphology
- Current-induced brightening of vacancy-related emitters in hexagonal boron nitride
- First-principles computational methods for quantum defects in two-dimensional materials: A perspective
- Manipulating the wavelength of single photons in insulating van der Waals heterostructures: theory and application to bilayer hexagonal boron nitride
- as a 2 eV Single-Photon Emitter Candidate in Hexagonal Boron Nitride
- Creating Quantum Emitters in Hexagonal Boron Nitride Deterministically on Chip-Compatible Substrates
- Reproducible generation of green-emitting color centers in hBN using oxygen annealing
- Secure Quantum Key Distribution Using a Room-Temperature Quantum Emitter
- Single Photon Emission from Plasma Treated 2D Hexagonal Boron Nitride
- Free-Space Quantum Key Distribution with Single Photons from Defects in Hexagonal Boron Nitride
- Generation of phonon quantum states and quantum correlations among single photon emitters in hexagonal boron nitride
- Robust Solid State Quantum System Operating at 800 K
- Deterministic generation of single B centers in hBN by one-to-one conversion from UV centers
- Insights into the Nature of Quantum Emitters in Electron-Irradiated hexagonal Boron Nitride
- Resonant Excitation of Quantum Emitters in Hexagonal Boron Nitride
- Decoherence of V spin defects in monoisotopic hexagonal boron nitride