Unprecedented anisotropic metallic state in BaFe2As2 revealed by optical spectroscopy
arXiv:1106.4967 · doi:10.1073/pnas.1100102108
Abstract
An ordered phase showing remarkable electronic anisotropy in proximity to the superconducting phase is now a hot issue in the field of high-transition-temperature superconductivity. As in the case of copper oxides, superconductivity in iron arsenides competes or coexists with such an ordered phase. Undoped and underdoped iron arsenides have a magnetostructural ordered phase exhibiting stripe-like antiferromagnetic spin order accompanied by an orthorhombic lattice distortion; both the spin order and lattice distortion break the tetragonal symmetry of crystals of these compounds. In this ordered state, anisotropy of in-plane electrical resistivity is anomalous and difficult to attribute simply to the spin order and/or the lattice distortion. Here, we present the anisotropic optical spectra measured on detwinned BaFe2As2 crystals with light polarization parallel to the Fe planes. Pronounced anisotropy is observed in the spectra, persisting up to an unexpectedly high photon energy of about 2 eV. Such anisotropy arises from an anisotropic energy gap opening below and slightly above the onset of the order. Detailed analysis of the optical spectra reveals an unprecedented electronic state in the ordered phase.
7 pages, 7 figures, accepted to PNAS
References in corpus (37)
- Magnetic Order versus superconductivity in the Iron-based layered La(O1-xFx)FeAs systems
- Evidence for an electron nematic phase transition in underdoped iron pnictide superconductors
- Magnetic order in BaFe2As2, the parent compound of the FeAs based superconductors in a new structural family
- Nematic Fermi Fluids in Condensed Matter Physics
- Theory of Electron Nematic Order in LaOFeAs
- Intra-unit-cell electronic nematicity of the high-Tc copper-oxide pseudogap states
- Broken rotational symmetry in the pseudogap phase of a high-Tc superconductor
- Symmetry breaking orbital anisotropy on detwinned Ba(Fe1-xCox)2As2 above the spin density wave transition
- Ising and Spin orders in Iron-based Superconductors
- Spin Waves and Magnetic Exchange Interactions in CaFe2As2
- Ferro-Orbital Order and Strong Magnetic Anisotropy in the Parent Compounds of Iron-Pnictide Superconductors
- Spin-orbital frustrations and anomalous metallic state in iron-pnictide superconductors
- Effects of nematic fluctuations on the elastic properties of iron arsenide superconductors
- Lattice and magnetic instabilities in CaFe2As2: A single crystal neutron diffraction study
- First order structural phase transition in CaFeAs
- Magnetism and Charge Dynamics in Iron Pnictides
- Uniaxial strain detwinning of CaFe2As2 and BaFe2As2: optical and transport study
- Nodal Spin Density Wave and band topology of the FeAs based materials
- A key role for unusual spin dynamics in ferropnictides
- Observation of Dirac Cone Electronic Dispersion in BaFe2As2
- Orbital Order and Spontaneous Orthorhombicity in Iron Pnictides
- Magnetic and structural transitions in layered FeAs systems: AFe2As2 versus RFeAsO compounds
- Spin and Lattice Structure of Single Crystal SrFe2As2
- Orbital Ordering and Unfrustrated Magnetism from Degenerate Double Exchange in the Iron Pnictides
- Orbital-dependent modifications of electronic structure across magneto-structural transition in BaFe2As2
- Universal Decomposition of the Low-Frequency Conductivity Spectra of Iron-Pnictides Uncovering Fermi-Liquid Behavior
- Evolution of the optical spectrum with doping in iron pnictides Ba(Fe1-xCox)2As2
- Anisotropic charge dynamics in detwinned Ba(FeCo)As
- Paramagnetic Spin Correlations in CaFe2As2 Single Crystals
- Topological and Transport Properties of Dirac Fermions in Antiferromagnetic Metallic Phase of Iron-Based Superconductors
- Conductivity anisotropy in the antiferromagnetic state of iron pnictides
- Phonon anomaly in BaFe2As2
- Orbital-weight redistribution triggered by spin order in the pnictides
- Formation of partial energy gap below the structural phase transition and the rare-earth element substitution effect on infrared phonons in ReFeAsO (Re=La, Nd, and Sm)
- Crystal Symmetry and Magnetic Order in Iron Pnictides: a Tight Binding Wannier Function Analysis
- Theoretical Investigation of Optical Conductivity in Ba [Fe(1-x)Co(x)]2 As2
- Theory of Orbital Nematicity in Underdoped Iron Arsenides
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- Visualization of Electron Nematicity and Unidirectional Antiferroic Fluctuations at High Temperatures in NaFeAs
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- Magnetic interactions in iron superconductors: A review
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