A key role for unusual spin dynamics in ferropnictides
arXiv:0807.3737 · doi:10.1038/nphys1160
Abstract
The 2008 discovery of superconducting ferropnictides with Tc~26K-56K introduced a new family of materials into the category of high Tc superconductors. The ongoing project of understanding the superconducting mechanism and pairing symmetry has already revealed a complicated and often contradictory underlying picture of the structural and magnetic properties. There is an almost unprecedented sensitivity of the calculated magnetism and Fermi surface to structural details that prohibits correspondence with experiment. Furthermore, experimental probes of the order parameter symmetry are in surprisingly strong disagreement, even considering the relative immaturity of the field. Here we outline all of the various and seemingly contradictory evidences, both theoretical and experimental, and show that they can be rectified if the system is assumed to be highly magnetic with a spin density wave that is well-defined but with magnetic twin and anti-phase boundaries that are dynamic on the time-scale of experiments. Under this assumption, we find that our calculations can accurately reproduce even very fine details of the structure, and a natural explanation for the temperature separation of structural and magnetic transitions is provided. Thus, our theory restores agreement between experiment and theory in crucial areas, making further cooperative progress possible on both fronts. We believe that fluctuating magnetic domains will be an essential component of unravelling the interplay between magnetic interactions and superconductivity in these newest high Tc superconductors.
References in corpus (33)
- Superconductivity at 38 K in the iron arsenide (Ba1-xKx)Fe2As2
- Magnetic Order versus superconductivity in the Iron-based layered La(O1-xFx)FeAs systems
- LaFeAsOF: A low carrier density superconductor near itinerant magnetism
- Superconductivity at 41 K and its competition with spin-density-wave instability in layered CeOFFeAs
- Observation of Fermi-surface-dependent nodeless superconducting gaps in Ba0.6K0.4Fe2As2
- Magnetic order in BaFe2As2, the parent compound of the FeAs based superconductors in a new structural family
- Structural and magnetic phase diagram of CeFeAsO1-xFx and its relationship to high-temperature superconductivity
- Pressure induced superconductivity in CaFeAs
- Origin of the ~150 K Anomaly in LaOFeAs; Competing Antiferromagnetic Superexchange Interactions, Frustration, and Structural Phase Transition
- Correlated electronic structure of LaOFeAs
- Superconductivity up to 29 K in SrFe2As2 and BaFe2As2 at high pressures
- The challenge of unravelling magnetic properties in LaFeAsO
- Pressure-induced volume-collapsed tetragonal phase of CaFe2As2 as seen via neutron scattering
- Phase transitions in LaFeAsO: structural, magnetic, elastic, and transport properties, heat capacity and Mossbauer spectra
- Electron-Hole Symmetry and Magnetic Coupling in Antiferromagnetic LaOFeAs
- Commensurate Spin Density Wave in LaOFeAs: A Local Probe Study
- The Unprecedented Giant Coupling of Fe-spin State and the As-As Hybridization in Iron-Pnictide
- Momentum dependence of the superconducting gap in NdFeAsO1-xFx single crystals measured by angle resolved photoemission spectroscopy
- Electron Correlations in the Low Carrier Density LaFeAsO0.89F0.11 Superconductor (Tc = 28 K)
- Momentum dependence of the superconducting gap in BaKFeAs
- Spin and Lattice Structure of Single Crystal SrFe2As2
- Multiple Nodeless Superconducting Gaps in (Ba0.6K0.4)Fe2As2 Superconductor from Angle-Resolved Photoemission Spectroscopy
- A possible ground state and its electronic structure of a mother material (LaOFeAs) of new superconductors
- Pressure-induced superconductivity in single crystal CaFe2As2
- Structure and Magnetic Order in the NdFeAs(O,F) Superconductor System
- Strong coupling between magnetic and structural order parameters in SrFe2As2
- Magnetic Order of the Iron Spins in NdOFeAs
- Evidence for Strong Itinerant Spin Fluctuations in the Normal State of CeFeAsO(0.89)F(0.11) Iron-Oxypnictides
- Magnetic penetration depth of single crystal SmFeAsO_{1-x}F_y: a fully gapped superconducting state
- Muon spin relaxation studies of magnetic order and superfluid density in antiferromagnetic NdOFeAs, BaFe2As2 and superconducting (Ba,K)Fe2As2
- Lattice Dynamics of LaFeAsO_{1-x}F_{x} and PrFeAsO_{1-y} via Inelastic X-Ray Scattering and First-Principles Calculation
- Large Seebeck coefficients in Iron-oxypnictides : a new route towards n-type thermoelectric materials
- Competition between antiferromagnetic instability and frustrations in Fe-Se
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- The effect of double counting, spin density, and Hund interaction in the different DFT+ functionals
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- Pressure-driven phase transition from antiferromagnetic semiconductor to nonmagnetic metal in two-leg ladders Fe (=Ba or K, =S or Se)
- Effect of disorder on the resistivity anisotropy near the electronic nematic phase transition in pure and electron-doped BaFeAs
- Symmetry preserving lattice collapse in tetragonal SrFe_(2-x)Ru_xAs_2 (x = 0, 0.2) -- a combined experimental and theoretical study
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- In-plane anisotropy of electrical resistivity in the strain-detwinned SrFe2As2
- Pressure versus concentration tuning of the superconductivity in Ba(Fe(1-x)Cox)2As2
- 23Na and 75As NMR Study of Antiferromagnetism and Spin Fluctuations on NaFeAs Single Crystals
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- Evidence for filamentary superconductivity nucleated at antiphase domain walls in antiferromagnetic CaFeAs
- Electron-Phonon Properties of Pnictide Superconductors
- Excitonic spin density wave state in iron pnictides
- Suppression of the structural phase transition and lattice softening in slightly underdoped Ba(1-x)K(x)Fe2As2 with electronic phase separation
- Metal-Insulator Transition and the Role of Electron Correlation in FeO2
- Quasiparticle interference in iron-based superconductors
- Doping dependent Irreversible Magnetic Properties of Ba(Fe1-xCox)2As2 Single Crystals
- First-principles study of magnetic properties in Fe-ladder compound BaFe2S3
- Structural, Magnetic and Electronic Properties of the Iron-Chalcogenide AFeSe (A=K, Cs, Rb, Tl and etc.) Superconductors
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- Magneto-elastically coupled structural, magnetic and superconducting order parameters in BaFe(AsP)
- Muon-spin-rotation study of the magnetic structure in the tetragonal antiferromagnetic state of weakly underdoped BaKFeAs
- Distinct high-T transitions in underdoped BaKFeAs
- Spin-waves in the orthorombic square-lattice Heisenberg models: Application to the iron pnictide materials
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