23Na and 75As NMR Study of Antiferromagnetism and Spin Fluctuations on NaFeAs Single Crystals

Abstract

We report the ${}^{23}$Na and ${}^{75}$As NMR studies on NaFeAs single crystals. The structure transition temperature $T_S$ (55 K) and the spin density wave (SDW) transition temperature $T_{SDW}$ (40.5 K) are determined by the NMR line splits. The spin-lattice relaxation rates indicate that the spin fluctuations are strongly enhanced just below $T_S$ and drive a second order SDW transition. A fluctuating feature of the SDW ordering is also seen below the $T_{SDW}$. We further performed high-pressure NMR studies on NaFeAs, and found that the $T_{SDW}$ increases by $\sim$7 K and the magnetic moment increases by 30% under 2.5 GPa pressure.

high pressure data added

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