An optically stimulated superconducting-like phase in K3C60 far above equilibrium Tc

Abstract

The control of non-equilibrium phenomena in complex solids is an important research frontier, encompassing new effects like light induced superconductivity. Here, we show that coherent optical excitation of molecular vibrations in the organic conductor K3C60 can induce a non-equilibrium state with the optical properties of a superconductor. A transient gap in the real part of the optical conductivity and a low-frequency divergence of the imaginary part are measured for base temperatures far above equilibrium Tc=20 K. These findings underscore the role of coherent light fields in inducing emergent order.

40 pages, 23 figures

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• Time-hidden magnetic order in a multi-orbital Mott insulator
• Smart meta-superconductor MgB2 constructed by inhomogeneous phase of luminescent nanocomposite
• Interlayer Dzyaloshinskii-Moriya interactions induced via non-linear phononics in bilayer van der Waals materials
• Temporarily enhanced superconductivity from magnetic fields
• Signature of preformed pairs in angle-resolved photoemission spectroscopy
• Photo-induced Dynamics of Quasicrystalline Excitonic Insulator
• Spin-orbit coupling in organic microcavities: Lower polariton splitting, triplet polaritons, and disorder-induced dark-states relaxation
• Direct driving of electronic and phononic degrees of freedom in a honeycomb bilayer with infrared light
• Role of phonon coupling in driving photo-excited Mott insulators towards a transient superconducting steady state
• Optical control of the current-voltage relation in stacked superconductors
• First-principle based Floquet engineering of solids in the velocity gauge
• Light-induced reorientation transition in an antiferromagnetic semiconductor
• Ultrafast excitation and topological soliton formation in incommensurate charge density wave states
• Scattering resonances and pairing in a Rabi-coupled Fermi gas
• Cavity-assisted magnetization switching in a quantum spin-phonon chain
• Excitonic enhancement of cavity-mediated interactions in a two-band Hubbard model
• mm-wave Rydberg-Rydberg resonances as a witness of intermolecular coupling in the arrested relaxation of a molecular ultracold plasma
• Adiabatic perturbation theory of nonequilibrium light-controlled superconductivity
• Magnetization precession after non-collinear dual optical excitation
• Photoinduced dynamics of excitonic order and Rabi oscillation in the two-orbital Hubbard model
• Parametric control of Meissner screening in light-driven superconductors
• Phonon state tomography of electron correlation dynamics in optically excited solids
• Ultrafast Electron Diffraction: Visualizing Dynamic States of Matter
• High-resolution MHz time- and angle-resolved photoemission spectroscopy based on a tunable vacuum ultraviolet source
• Evidence for bootstrap percolation dynamics in a photo-induced phase transition
• Ephemeral Superconductivity Atop the False Vacuum
• Steady-states and response functions of the periodically driven O(N) scalar field theory
• Ultrafast dynamics of a fermion chain in a terahertz field-driven optical cavity
• Nonequilibrium topological spin textures in momentum space
• Ultrafast dynamics of quantum matter driven by time-energy entangled photons
• Controlling magnetic correlations in a driven Hubbard system far from half-filling
• Surface-acoustic-wave-induced unconventional superconducting pairing
• Meissner effect in non-Hermitian superconductors
• Singularities of Floquet Scattering and Tunneling
• Modifying electronic and structural properties of 2D van der Waals materials via cavity quantum vacuum fluctuations: A first-principles QEDFT study
• Attosecond correlated electron dynamics at C${}_{60}$ giant plasmon resonance
• Floquet Schrieffer-Wolff transform based on Sylvester equations
• A possible experimental test of the nonlinear phononics interpretation of light-induced superconductivity
• Dynamical Approach to Realize Room-Temperature Superconductivity in LaH${}_{10}$
• Floquet engineering of effective pairing interactions in a doped band insulator
• Tuning magnetic interactions with nonequilibrium optical phonon populations: a theoretical study
• Probing microscopic models for system-bath interactions via parametric driving
• Dissipation and non-thermal states in cryogenic cavities
• Magnon Nesting in Driven Two-Dimensional Quantum Magnets
• Decoding the drive-bath interplay: A guideline to enhance superconductivity
• A light-induced charge order mode in a metastable cuprate ladder
• Computable measures of non-Markovianity for Gaussian free fermion systems
• Superconducting gap and its Little-Parks like oscillations with high-order harmonics in lithium intercalated 1T-TiSe${}_2$
• Field induced conducting state in Mott insulator
• Superconductivity of niobium thin films in the BiOCl/Nb heterostructures
• Low-frequency and Moiré Floquet engineering: a review
• Many Electrons and the Photon Field -- The many-body structure of nonrelativistic quantum electrodynamics
• Mechanism for Synchronization of Charge Oscillations in Dimer Lattices
• Phonon-induced disorder in dynamics of optically pumped metals from non-linear electron-phonon coupling
• Dynamical control in a prethermalized molecular ultracold plasma: Local dissipation drives global relaxation
• Optical Pumping of Bardeen-Cooper-Schrieffer Superconductors
• Fate of transient order parameter domain walls in ultrafast experiments
• Dynamically generated quadrupole polarization using Floquet adiabatic evolution
• Photoinduced intradomain dynamics and nonthermal switching of metastable states in the one-dimensional extended Peierls-Hubbard model
• Transient ordering in the Gross-Pitaevskii lattice subject to an energy quench within the disordered phase
• Intertwined geometries in collective modes of two dimensional Dirac fermions
• Radiative Higgs mode in photoinduced $\eta$ pairs
• A Computational Method for Studying Vibrational Mode Dynamics
• Smart metastructure method for increasing TC of Bi(Pb)SrCaCuO high-temperature superconductors
• Superconducting fluctuations observed far above T${}_{\mathrm{c}}$ in the isotropic superconductor K${}_3$C${}_{60}$
• Nonequilibrium hysteretic phase transitions in periodically light-driven superconductors
• Nonequilibrium spectral moment sum rules of the Holstein-Hubbard model
• Terahertz-induced tunnel ionization drives coherent Raman-active phonon in Bismuth
• Enhancement of superconducting pairing via quantum Lyapunov control
• Dissipative cooling induced by pulse perturbations
• Mode-selective ballistic pathway to a metastable electronic phase
• Symmetry breaking driven by petahertz electron acceleration in a centrosymmetric organic superconductor
• High Harmonic Generation in Two-Dimensional Mott Insulators
• Dynamical correlations and nonequilibrium sum rules in photodoped Hubbard ladders
• Physical Mechanism of Superconductivity Part II Superconductivity and Superfluidity
• Quantized Acoustoelectric Floquet Effect in Quantum Nanowires
• Light-driven topological and magnetic phase transitions in thin-layer antiferromagnets
• Nonequilibrium Dynamics in a Quantum Spin Chain with Pump-Probe Resonant Inelastic X-ray Scattering
• Correlative Ultrafast Imaging of a Propagating Photo-Driven Phase Transition Using 4D STEM
• Recent Progress in Ultrafast Dynamics of Transition-Metal Compounds Studied by Time-Resolved X-ray Techniques
• Non-thermal pairing glue of electrons in the steady state
• Charge carrier relaxation dynamics in the one-dimensional Kondo lattice model
• Photoinduced excitonic magnetism in a multiorbital Hubbard system
• Properties and challenges of hot-phonon physics in metals: MgB${}_2$ and other compounds
• Light induced transitions of valley Chern numbers and flat bands in a non-twisted moire graphene-hexagonal boron nitride superlattice
• Radio-frequency driving of an attractive Fermi gas in a one-dimensional optical lattice