Equilibrium Parametric Amplification in Raman-Cavity Hybrids
arXiv:2312.14243 · doi:10.1103/PhysRevLett.133.116901
Abstract
Parametric resonances and amplification have led to extraordinary photoinduced phenomena in pump-probe experiments. While these phenomena manifest themselves in out-of-equilibrium settings, here, we present the striking result of parametric amplification in equilibrium. In particular, we demonstrate that quantum and thermal fluctuations of a Raman-active mode amplifies light inside a cavity, at equilibrium, when the Raman mode frequency is twice the cavity mode frequency. This noise-driven amplification leads to the creation of an unusual parametric Raman polariton, intertwining the Raman mode with cavity squeezing fluctuations, with smoking gun signatures in Raman spectroscopy. In the resonant regime, we show the emergence of not only quantum light amplification but also localization and static shift of the Raman mode. Apart from the fundamental interest of equilibrium parametric amplification our study suggests a resonant mechanism for controlling Raman modes and thus matter properties by cavity fluctuations. We conclude by outlining how to compute the Raman-cavity coupling, and suggest possible experimental realization
as accepted in PRL
References in corpus (52)
- Ultrastrong coupling between light and matter
- Observation of a Discrete Time Crystal
- Observation of discrete time-crystalline order in a disordered dipolar many-body system
- Light-induced anomalous Hall effect in graphene
- An optically stimulated superconducting-like phase in K3C60 far above equilibrium Tc
- Conductivity in organic semiconductors hybridized with the vacuum field
- Phase space representation of quantum dynamics
- Ultrastrong coupling of the cyclotron transition of a two-dimensional electron gas to a THz metamaterial
- Nonlinear phononics: A new ultrafast route to lattice control
- Nonthermal pathways to ultrafast control in quantum materials
- Metastable ferroelectricity in optically strained
- Petahertz Spintronics
- Light-Induced Charge Density Wave in LaTe
- Cavity Quantum Materials
- Amplified Emission by Atoms and Lasing in Photonic Time Crystals
- Observation of a dissipative time crystal
- Strongly-Correlated Electron-Photon Systems
- Observation of a continuous time crystal
- Colloquium: Quantum and Classical Discrete Time Crystals
- Evidence for metastable photo-induced superconductivity in KC
- QED description of Raman scattering from molecules in plasmonic cavities
- Ultrastrong Coupling in the Near-field of Complementary Split Ring Resonators
- Observation of Low Energy Raman Modes in Twisted Bilayer Graphene
- Observation of Three-Photon Spontaneous Parametric Downconversion in a Superconducting Parametric Cavity
- Raman fingerprints of atomically precise graphene nanoribbons
- Optical Stabilization of Fluctuating High Temperature Ferromagnetism in YTiO
- Terahertz sum-frequency excitation of a Raman-active phonon
- Sum-frequency ionic Raman scattering
- Large Enhancement of Ferro-Magnetism under Collective Strong Coupling of YBCO Nanoparticles
- Parametric amplification of optical phonons
- Large-scale mapping of moiré superlattices by Raman imaging of interlayer breathing mode and moiré phonons
- Time crystals in a shaken atom-cavity system
- Cavity-Enhanced Ultrafast Transient Absorption Spectroscopy
- Self-similar dynamics of order parameter fluctuations in pump-probe experiments
- Parametric excitation of an optically silent Goldstone-like phonon mode
- Higgs-mediated optical amplification in a non-equilibrium superconductor
- Parametric resonance of Josephson plasma waves: A theory for optically amplified interlayer superconductivity in YBaCuO
- Emergent parametric resonances and time-crystal phases in driven BCS systems
- Direct Measurement of Anharmonic Decay Channels of a Coherent Phonon
- Realization of a periodically driven open three-level Dicke model
- Cavity control of nonlinear phononics
- Controlling the magnetic state of the proximate quantum spin liquid -RuCl with an optical cavity
- Dynamical mean-field study of a photon-mediated ferroelectric phase transition
- Light-induced topological magnons in two-dimensional van der Waals magnets
- Parametrically amplified phase-incoherent superconductivity in YBaCuO
- Population inversion and dynamical phase transitions in a driven superconductor
- Tunable cryogenic THz cavity for strong light-matter coupling in complex materials
- Dynamical phases transitions in periodically driven Bardeen-Cooper-Schrieffer systems
- Non-Gaussian superradiant transition via three-body ultrastrong coupling
- Condensate formation in a dark state of a driven atom-cavity system
- Local Fluctuations in Cavity Control of Ferroelectricity
- Resonant squeezed light from photonic Cooper pairs