Stimulated Rayleigh Scattering Enhanced by a Longitudinal Plasma Mode in a Periodically Driven Dirac Semimetal CdAs
arXiv:2112.13113 · doi:10.1103/PhysRevLett.129.207402
Abstract
Using broadband (12-45 THz) multi-terahertz spectroscopy, we show that stimulated Rayleigh scattering dominates the transient optical conductivity of cadmium arsenide, a Dirac semimetal, under an optical driving field at 30 THz. The characteristic dispersive lineshape with net optical gain is accounted for by optical transitions between light-induced Floquet subbands, strikingly enhanced by the longitudinal plasma mode. Stimulated Rayleigh scattering with an unprecedentedly large refractive index change may pave the way for slow light generation in conductive solids at room temperature.
arXiv comment29 pages, 11 figures
References in corpus (32)
- Three Dimensional Dirac Semimetal and Quantum Transports in Cd3As2
- Photovoltaic Hall effect in graphene
- Observation of Floquet-Bloch states on the surface of a topological insulator
- Floquet Engineering of Quantum Materials
- Light-induced anomalous Hall effect in graphene
- An optically stimulated superconducting-like phase in K3C60 far above equilibrium Tc
- Topological nature of nonlinear optical effects in solids
- Selective scattering between Floquet-Bloch and Volkov states in a topological insulator
- Creating stable Floquet-Weyl semimetals by laser-driving of 3D Dirac materials
- Light-Induced Charge Density Wave in LaTe
- A High-Performance Mid-infrared Optical Switch Enabled by Bulk Dirac Fermions in Cd3As2
- Ultrafast Broadband Photodetectors based on Three-dimensional Dirac Semimetal Cd3As2
- Evidence for metastable photo-induced superconductivity in KC
- Microscopic theory for the light-induced anomalous Hall effect in graphene
- Efficient Terahertz Harmonic Generation with Coherent Acceleration of Electrons in the Dirac Semimetal Cd3As2
- Floquet Weyl Semimetal Induced by Off-Resonant Light
- Non-perturbative high-harmonic generation in the three-dimensional Dirac semimetal CdAs
- Magneto-optical signature of massless Kane electrons in Cd3As2
- 3D Dirac semimetal Cd3As2: A review of material properties
- Interband optical conductivity of the [001]-oriented Dirac semimetal Cd3As2
- Floquet analysis of excitations in materials
- Chiral pumping effect induced by rotating electric fields
- Bicircular light tuning of magnetic symmetry and topology in Dirac semimetal CdAs
- Optical Hall conductivity of a Floquet Topological Insulator
- Terahertz time-domain spectroscopy of transient metallic and superconducting states
- Pump driven normal-to-excitonic insulator transition: Josephson oscillations and signatures of BEC-BCS crossover in time-resolved ARPES
- Efficient generation of extreme terahertz harmonics in 3D Dirac semimetals
- Floquet topological phase of nondriven -wave nonequilibrium excitonic insulators
- Optical parametric amplification of phase-stable terahertz-to-midinfrared pulses studied in the time domain
- Dynamics of quasiparticles in graphene under intense circularly polarized light
- All Optical Measurement Proposed for the Photovoltaic Hall Effect
- Tracking ultrafast change of multiterahertz broadband response functions in a photoexcited Dirac semimetal CdAs thin film
Cited by in corpus (5)
- Disentangling the Competing Mechanisms of Light-Induced Anomalous Hall Conductivity in Three-Dimensional Dirac Semimetal
- Observation of Terahertz Spin Hall Conductivity Spectrum in GaAs with Optical Spin Injection
- Population inversion and ultrafast terahertz nonlinearity of transient Dirac fermions in CdAs
- Anomalous Hall transport by optically injected isospin degree of freedom in Dirac semimetal thin film
- Correction of broadband terahertz electro-optic sampling with GaSe crystals