Photoinduced electron-electron pairing in the extended Falicov-Kimball model

Abstract

By employing the time-dependent exact diagonalization method, we investigate the photoexcited states of the excitonic insulator in the extended Falicov-Kimball model (EFKM). We here show that the pulse irradiation can induce the interband electron-electron pair correlation in the photoexcited states, while the excitonic electron-hole pair correlation in the initial ground state is strongly suppressed. We also show that the photoexcited states contains the eigenstates of the EFKM with a finite number of interband electron-electron pairs, which are responsible for the enhancement of the electron-electron pair correlation. The mechanism found here is due to the presence of the internal SU(2) pairing structure in the EFKM and thus it is essentially the same as that for the photoinduced $\eta$-pairing in the repulsive Hubbard model reported recently [T. Kaneko et al., Phys. Rev. Lett. $122$, 077002 (2019)]. This also explains why the nonlinear optical response is effective to induce the electron-electron pairs in the photoexcited states of the EFKM. Furthermore, we show that, unlike the $\eta$-pairing in the Hubbard model, the internal SU(2) structure is preserved even for a nonbipartite lattice when the EFKM has the direct-type band structure, in which the pulse irradiation can induce the electron-electron pair correlation with momentum $\mathbf{q}$ = $\text{0}$ in the photoexcited states. We also discuss briefly the effect of a perturbation that breaks the internal SU(2) structure.

arXiv comment15 pages, 13 figures

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