Orthorhombic-to-Monoclinic Phase Transition of Ta2NiSe5 Induced by the Bose-Einstein Condensation of Excitons

Abstract

Using the band structure calculation and mean-field analysis of the derived three-chain Hubbard model with phonon degrees of freedom, we discuss the origin of the orthorhombic-to-monoclinic phase transition of the layered chalcogenide Ta${}_2$NiSe${}_5$. We show that the Bose-Einstein condensation of excitonic electron-hole pairs cooperatively induces the instability of the phonon mode at momentum $q\to 0$ in the quasi-one-dimensional Ta-NiSe-Ta chain, resulting in the structural phase transition of the system. The calculated single-particle spectra reproduce the deformation of the band structure observed in the angle-resolved photoemission spectroscopy experiment.

5 pages, 4 figures

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• On the possibility of an excitonic insulator at the semiconductor-semimetal transition
• Bound state formation and nature of the excitonic insulator phase in the extended Falicov-Kimball model
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Cited by in corpus (111)

• Ultrafast Electronic Band Gap Control in an Excitonic Insulator
• Excitonic Bose-Einstein condensation in Ta2NiSe5 above room temperature
• Coherent Order Parameter Oscillations in the Ground State of the Excitonic Insulator Ta2NiSe5
• Nature of symmetry breaking at the excitonic insulator transition: Ta${}_2$NiSe${}_5$
• Excitonic condensation in systems of strongly correlated electrons
• Giant exciton Fano resonance in quasi-one-dimensional Ta${}_2$NiSe${}_5$
• Photo-induced semimetallic states realised in electron-hole coupled insulators
• Strong Coupling Nature of the Excitonic Insulator State in Ta${}_2$NiSe${}_5$
• Direct observation of excitonic instability in Ta2NiSe5
• Photo-induced enhancement of excitonic order
• Electron-Phonon Coupling Mode in Excitonic Insulator
• Band hybridisation at the semimetal-semiconductor transition of Ta${}_2$NiSe${}_5$ enabled by mirror-symmetry breaking
• Phase diagram and collective excitation in excitonic insulator: from the orbital physics viewpoint
• Strong interband interaction in the excitonic insulator phase of Ta${}_2$NiSe${}_5$
• Photo-induced gap closure in an excitonic insulator
• Impact of Electron-Hole Correlations on the 1T-TiSe2 Electronic Structure
• Chiral charge order in 1$T$-TiSe${}_2$: importance of lattice degrees of freedom
• Imaging the coherent propagation of collective modes in the excitonic insulator candidate Ta${}_2$NiSe${}_5$ at room temperature
• Inhibition of the photoinduced structural phase transition in the excitonic insulator Ta${}_2$NiSe${}_5$
• Order, criticality and excitations in the extended Falicov-Kimball model
• Photoinduced multistage phase transitions in Ta2NiSe5
• Collective Modes in Excitonic Insulators: Effects of Electron-Phonon Coupling and Signatures in Optical Response
• Exciton-phonon cooperative mechanism of the triple-$q$ charge-density-wave and antiferroelectric electron polarization in TiSe${}_2$
• Detecting electron-phonon couplings during photo-induced phase transition
• Fate of the excitonic insulator in the presence of phonons
• Realizing intrinsic excitonic insulator by decoupling exciton binding energy from the minimum band gap
• Ultrafast melting and recovery of collective order in the excitonic insulator Ta${}_2$NiSe${}_5$
• Orthorhombic-to-monoclinic transition in Ta${}_2$NiSe${}_5$ due to a zone-center optical phonon instability
• Charge-density wave induced by combined electron-electron and electron-phonon interactions in 1$T$-TiSe${}_2$: A variational Monte Carlo study
• Roles of Hund's rule coupling in excitonic density-wave states
• Phononic soft mode and strong electronic background behavior across the structural phase transition in the excitonic insulator Ta${}_2$NiSe${}_5$ (with Erratum)
• Competition between excitonic charge and spin density waves: Influence of electron-phonon and Hund's rule couplings
• Ultrafast nonequilibrium evolution of excitonic modes in semiconductors
• Critical charge fluctuations and emergent coherence in a strongly correlated excitonic insulator
• Infrared phonon spectra of quasi-one-dimensional Ta${}_2$NiSe${}_5$ and Ta${}_2$NiS${}_5$
• Magnetic field effects in a correlated electron system with spin-state degree of freedom - Implication of an excitonic insulator -
• Bulk Photovoltaic Effect Driven by Collective Excitations in a Correlated Insulator
• Photo-induced phase transition and associated time scales in the excitonic insulator Ta${}_2$NiSe${}_5$
• Excitonic effects in two-dimensional TiSe${}_2$ from hybrid density functional theory
• Lattice dynamics of the excitonic insulator Ta${}_2$Ni(Se${}_{1-x}$S${}_x$)${}_5$
• Second order Josephson effect in excitonic insulators
• Role of electron-phonon coupling in excitonic insulator candidate Ta2NiSe5
• Microscopic quantum interference in excitonic condensation of Ta${}_2$NiSe${}_5$
• Doping-controlled transition from excitonic insulator to semimetal in Ta${}_2$NiSe${}_5$
• Photoinduced enhancement of excitonic order in the two-orbital Hubbard model
• Effect of Cu intercalation and pressure on excitonic interaction in 1T-TiSe2
• Hybridization-gap Formation and Superconductivity in the Pressure-induced Semimetallic Phase of the Excitonic Insulator Ta${}_2$NiSe${}_5$
• A New Era of Excitonic Insulators
• Nonlinear spectroscopy of collective modes in excitonic insulator
• Photo-excited Dynamics in the Excitonic Insulator Ta2NiSe5
• Nonequilibrium dynamics in the pump-probe spectroscopy of excitonic insulators
• FFLO Excitonic State in the Three-Chain Hubbard Model for Ta${}_2$NiSe${}_5$
• Quantum noise spectroscopy of dynamical critical phenomena
• Disentangling lattice and electronic instabilities in the excitonic insulator candidate Ta${}_2$NiSe${}_5$ by nonequilibrium spectroscopy
• Topological excitonic corner states and nodal phase in bilayer quantum spin Hall insulators
• Signatures of ultrafast reversal of excitonic order in Ta${}_2$NiSe${}_5$
• Bardasis-Schrieffer polaritons in excitonic insulators
• Temperature-dependent evolutions of excitonic superfluid plasma frequency in a srong excitonic insulator candidate, Ta${}_2$NiSe${}_5$
• Superconductivity in Nb2Pd3Te5 and Chemically-Doped Ta2Pd3Te5
• Anomalous excitonic phase diagram in band-gap-tuned Ta2Ni(Se,S)5
• Orbital diamagnetic susceptibility in excitonic condensation phase
• Electric and magnetic multipoles and bond orders in excitonic insulators
• Collective excitations of the U(1)-symmetric exciton insulator in a cavity
• Terahertz parametric amplification as a reporter of exciton condensate dynamics
• Room Temperature Thermoelectric Properties of Isostructural Selenides Ta2PdS6 and Ta2PdSe6
• Low-energy excitation spectra in the excitonic phase of cobalt oxides
• Evidence for an Excitonic Insulator State in Ta${}_2$Pd${}_3$Te${}_5$
• Topological charge pumping in excitonic insulators
• Photoinduced electron-electron pairing in the extended Falicov-Kimball model
• Excitonic phase transition in the extended three-dimensional Falicov-Kimball model
• Tunneling-tip-induced collapse of the charge gap in the excitonic insulator Ta${}_2$NiSe${}_5$
• Spin Seebeck Effect in Nonmagnetic Excitonic Insulators
• Ultrafast charge carrier and exciton dynamics in an excitonic insulator probed by time-resolved photoemission spectroscopy
• Evolution of the electronic structure in Ta${}_2$NiSe${}_5$ across the structural transition revealed by resonant inelastic x-ray scattering
• Ta2NiSe5: a candidate topological excitonic insulator with multiple band inversions
• Finite-temperature photoemission in the extended Falicov-Kimball model: a case study for Ta${}_2$NiSe${}_5$
• Effects of Disorder on the Transport of Collective Modes in an Excitonic Condensate
• Photoinduced metallization of excitonic insulators
• Excitonic Insulator State of the Extended Falicov-Kimball Model in the Cluster Dynamical Impurity Approximation
• Excitonic Phase Diagram of the Three-Chain Hubbard Model for Semiconducting and Semimetallic Ta${}_2$NiSe${}_5$
• Pressure suppression of the excitonic insulator state in Ta2NiSe5 observed by optical conductivity
• Optical signatures of exciton-polarons from diagrammatic Monte Carlo
• Theory of Orbital Susceptibility on Excitonic Insulator
• Third-harmonic generation in excitonic insulators
• Theory of time-crystalline behaviour mediated by phonon squeezing in Ta2NiSe5
• First- and second-order phase transitions between the uniform and FFLO excitonic states in the three-chain Hubbard model for Ta2NiSe5
• Excitonic insulators and Gross-Neveu models
• Temperature effects in excitonic condensation driven by the lattice distortion
• Finite-temperature properties of excitonic condensation in the extended Falicov-Kimball model: Cluster mean-field-theory approach
• Spin texture and spin current in excitonic phases of the two-band Hubbard model
• Excitonic Order and Superconductivity in the Two-Orbital Hubbard Model: Variational Cluster Approach
• Collective modes and Raman response in Ta${}_2$NiSe${}_5$
• Hidden excitonic quantum states with broken time-reversal symmetry
• Exciton condensation in an extended spinless Falicov Kimball model in the presence of orbital magnetic fields
• FFLO Superconductivity Mediated by Excitonic Fluctuation in Semimetallic Ta${}_2$NiSe${}_5$
• Electronic and Optical Properties of Ta${}_2$NiSe${}_5$ Monolayer: A First-principles Study
• Excitonic Josephson effect in double-layer graphene junctions
• Electronic band structure in pristine and Sulfur-doped Ta${}_2$NiSe${}_5$
• Excitonic Tunneling in the AB-bilayer Graphene Josephson Junctions
• Strong enhancement of magnetic susceptibility induced by spin-nematic fluctuations in an excitonic insulating system with spin-orbit coupling
• Detecting photoelectrons from spontaneously formed excitons
• Photoinduced dynamics of excitonic order and Rabi oscillation in the two-orbital Hubbard model
• Anomalous phonon Grüneisen parameters in semiconductor Ta${}_2$NiS${}_5$
• Effects of magnetic fields and orbital angular momentum on excitonic condensation in two-orbital Hubbard model
• Photo-induced Dynamics of Quasicrystalline Excitonic Insulator
• Gate tuning of coupled electronic and structural phase transition in atomically thin Ta${}_2$NiSe${}_5$
• Elastic Soft Mode and Electric Quadrupole Response in Excitonic Insulator Candidate (Ta${}_{0.952}$V${}_{0.048}$)${}_2$NiSe${}_5$: Contribution of Electron-Phonon Interaction
• Symmetry breaking states in the half-filled two-orbital Hubbard model with crystalline electric field
• Magnetic-field effect on excitonic condensation emergent in extended Falicov-Kimball model
• Unveiling Excitonic Insulator Signatures in Ta${}_2$NiSe${}_5$
• Long-lived relaxation channel and exciton-phonon coupling in Ta2NiSe5 via non-degenerate pump-probe spectroscopy