Effects of Disorder on the Transport of Collective Modes in an Excitonic Condensate

Abstract

An excitonic insulator (EI) is an unconventional quantum phase of matter in which excitons, bound pairs of electrons and holes, undergo Bose--Einstein condensation, forming a macroscopic coherent state. While its existence was first hypothesized half a century ago, the EI has eluded experimental observation in bulk materials for decades. In the last few years, a resurgence of interest in the subject has been driven by the identification of several candidate materials suspected to support an excitonic condensate. However, one obstacle in verifying the nature of these systems has been to find signatures of the EI that distinguish it from a normal insulator. To address this, we focus on a clear qualitative difference between the two phases: the existence of Goldstone modes born by the spontaneous breaking of a $U(1)$ symmetry in the EI. Even if this mode is gapped, as occurs in the case of an approximate symmetry, this branch of collective modes remains a fundamental feature of the low-energy dynamics of the EI provided the symmetry-breaking is small. We study a simple model that realizes an excitonic condensate, and use mean field theory within the random-phase approximation to determine its collective modes. We subsequently develop a diagrammatic method to incorporate the effects of disorder perturbatively, and use it to determine the scattering rate of the collective modes. We interpret our results within an an effective field theory. The collective modes are found to be robust against symmetry-preserving disorder, implying an experimental fingerprint unique to the EI: the ballistic propagation of low-lying modes over mesoscopic distances, at electronic-scale velocities. We suggest this could affect thermal transport at low temperatures, and could be observed via spatially-resolved pump-probe spectroscopy through the coherent response of phonons that hybridize with the collective modes.

arXiv comment21 pages, 10 figures. v3: Incorporated peer review feedback

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• Evidence of ideal excitonic insulator in bulk MoS2 under pressure
• A New Era of Excitonic Insulators
• Polaron spectroscopy of a bilayer excitonic insulator
• Theory of competing excitonic orders in insulating WTe${}_2$ monolayers
• Leaky exciton condensates in transition metal dichalcogenide moiré bilayers
• Excitonic insulator phase and dynamics of condensate in a topological one-dimensional model
• Stabilization of sliding ferroelectricity through exciton condensation