Ultrafast optical spectroscopy of strongly correlated materials and high-temperature superconductors: a non-equilibrium approach
arXiv:1601.07204 · doi:10.1080/00018732.2016.1194044
Abstract
In the last two decades, non-equilibrium spectroscopies have evolved from avant-garde studies to crucial tools for expanding our understanding of the physics of strongly correlated materials. The possibility of obtaining simultaneously spectroscopic and temporal information has led to insights that are complementary to (and in several cases beyond) those attainable by studying the matter at equilibrium. Multiple phase transitions and new orders arising from competing interactions are benchmark examples where the interplay among electrons, lattice, and spin dynamics can be disentangled because of the different timescales that characterize the recovery of the initial ground state. The nature of the broken-symmetry phases and of the bosonic excitations that mediate the electronic interactions, eventually leading to superconductivity or other exotic states, can be revealed by observing the sub-picosecond dynamics of impulsively excited states. Recent experimental developments have made possible to monitor the time-evolution of both the single-particle and collective excitations under extreme conditions, such as those arising from strong and selective photo-stimulation. Here, we review the most recent achievements in the experimental and theoretical studies of the non-equilibrium electronic, optical, structural and magnetic properties of correlated materials. The focus will be mainly on the prototypical case of correlated oxides that exhibit unconventional superconductivity or other exotic phases, even though the discussion will extend also to other topical systems. The necessity of extending the actual experimental capabilities and the numerical and analytic tools to microscopically treat the non-equilibrium phenomena beyond the simple phenomenological approaches represents one of the most challenging new frontier in physics.
Review, to appear in Advances in physics. 188 pages, 637 references, 77 figures
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- Dynamical correlations and nonequilibrium sum rules in photodoped Hubbard ladders
- Transient selection of competing order in frustrated spin Peierls systems after a quench
- Distinct amplitude mode dynamics upon resonant and off-resonant excitation across the charge density wave energy gap in LaTe3 investigated by time- and angle-resolved photoemission spectroscopy
- Nonequilibrium spectral moment sum rules of the Holstein-Hubbard model
- Nonequilibrium hysteretic phase transitions in periodically light-driven superconductors
- Chirped pulse control over the melting of superconductors
- Intertwined geometries in collective modes of two dimensional Dirac fermions
- Ultrafast Electronic Structure Engineering in 1-TaS: Role of Doping and Amplitude Mode Dynamics
- Floquet spin textures in optically pumped non-Hermitian surface states
- Ultrafast Raman probe of the photoinduced superconducting to normal state transition in the cuprate BiSrCaCuO
- Two-dimensional THz spectroscopy in electronic systems: a many-body diagrammatic approach
- Charge carrier relaxation dynamics in the one-dimensional Kondo lattice model
- Collective Magnetic Excitations in a Photo-excited Electron-doped Cuprate Superconductor
- Capturing reduced-order quantum many-body dynamics out of equilibrium via neural ordinary differential equations
- Tracking the local order parameter through the Hubbard exciton decoherence time in the Mott-Hubbard insulator LaVO3
- Nonequilibrium Dynamics in a Quantum Spin Chain with Pump-Probe Resonant Inelastic X-ray Scattering
- Ultrafast charge-transfer dynamics in CaCuOCl from time-resolved optical reflectivity
- Tracking the surface atomic motion in a coherent phonon oscillation
- Properties and challenges of hot-phonon physics in metals: MgB and other compounds
- Radio-frequency driving of an attractive Fermi gas in a one-dimensional optical lattice
- Dissipative cooling induced by pulse perturbations
- Radiative Higgs mode in photoinduced pairs