Detection and control of individual nuclear spins using a weakly coupled electron spin

Abstract

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify the interaction with a selected nuclear spin and at the same time dynamically suppress decoherence caused by the rest of the spin bath. We are able to address nuclear spins with interaction strengths that are an order of magnitude smaller than the electron spin dephasing rate. Our results provide a route towards tomography with single-nuclear-spin sensitivity and greatly extend the number of available quantum bits for quantum information processing in diamond.

References in corpus (20)

• Quantum Computing
• High-sensitivity diamond magnetometer with nanoscale resolution
• Universal dynamical decoupling of a single solid-state spin from a spin bath
• Single-shot readout of an electron spin in silicon
• High-fidelity projective readout of a solid-state spin quantum register
• Scanning magnetic field microscope with a diamond single-spin sensor
• Solid state quantum memory using the 31P nuclear spin
• Temperature and magnetic field dependent longitudinal spin relaxation in nitrogen-vacancy ensembles in diamond
• Decoherence-protected quantum gates for a hybrid solid-state spin register
• Extending Quantum Coherence in Diamond
• Dynamical Decoupling of a single electron spin at room temperature
• Nanoscale magnetic field mapping with a single spin scanning probe magnetometer
• Decoherence and dynamical decoupling control of nitrogen-vacancy center electron spins in nuclear spin baths
• Sensing distant nuclear spins with a single electron spin
• Single-spin magnetometry with multi-pulse sensing sequences
• Universal enhancement of the optical readout fidelity of single electron spins
• Nuclear spin pair coherence in diamond for atomic scale magnetometry
• Robust control of individual nuclear spins in diamond
• High resolution spectroscopy of single NV defects coupled with nearby ${}^{13}$C nuclear spins in diamond
• Ultra-sensitive Diamond Magnetometry Using Optimal Dynamic Decoupling

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