Determination of the Position of a Single Nuclear Spin from Free Nuclear Precessions Detected by a Solid-State Quantum Sensor
arXiv:1806.00177 · doi:10.1103/PhysRevB.98.121405
Abstract
We report on a nanoscale quantum-sensing protocol which tracks a free precession of a single nuclear spin and is capable of estimating an azimuthal angle---a parameter which standard multipulse protocols cannot determine---of the target nucleus. Our protocol combines pulsed dynamic nuclear polarization, a phase-controlled radiofrequency pulse, and a multipulse AC sensing sequence with a modified readout pulse. Using a single nitrogen-vacancy center as a solid-state quantum sensor, we experimentally demonstrate this protocol on a single 13C nuclear spin in diamond and uniquely determine the lattice site of the target nucleus. Our result paves the way for magnetic resonance imaging at the single-molecular level.
arXiv comment21 pages, 15 figures, updated Ref. [39] (J. Zopes et al. arXiv:1806.04883)
References in corpus (25)
- Magnetometry with nitrogen-vacancy defects in diamond
- High Resolution Magnetic Resonance Spectroscopy Using Solid-State Spins
- Universal control and error correction in multi-qubit spin registers in diamond
- Sub-millihertz magnetic spectroscopy with a nanoscale quantum sensor
- Detection and control of individual nuclear spins using a weakly coupled electron spin
- Quantum sensing with arbitrary frequency resolution
- Nanoscale NMR Spectroscopy and Imaging of Multiple Nuclear Species
- Sensing remote nuclear spins
- Sensing distant nuclear spins with a single electron spin
- Nuclear spin pair coherence in diamond for atomic scale magnetometry
- High-Resolution Correlation Spectroscopy of 13C Spins Near a Nitrogen-Vacancy Center in Diamond
- Nanoscale nuclear magnetic resonance with a 1.9-nm-deep nitrogen-vacancy sensor
- Pulsed polarisation for robust DNP
- Scanning probe microscopy with chemical contrast by nanoscale nuclear magnetic resonance
- Probing molecular dynamics at the nanoscale via an individual paramagnetic center
- Solution nuclear magnetic resonance spectroscopy on a nanostructured diamond chip
- Tutorial: Magnetic resonance with nitrogen-vacancy centers in diamond---microwave engineering, materials science, and magnetometry
- One- and two-dimensional nuclear magnetic resonance spectroscopy with a diamond quantum sensor
- Towards chemical structure resolution with nanoscale nuclear magnetic resonance spectroscopy
- Robust techniques for polarization and detection of nuclear spin ensembles
- Non-flipping 13C spins in NV diamond: Hyperfine and Spatial Characteristics by DFT Simulation of the C510[NV]H252 Cluster
- Positioning Nuclear Spins in Interacting Clusters for Quantum Technologies and Bio-imaging
- Delayed entanglement echo for individual control of a large number of nuclear spins
- The diamond Nitrogen-Vacancy center as a probe of random fluctuations in a nuclear spin ensemble
- Imaging nuclear spins weakly coupled to a probe paramagnetic center
Cited by in corpus (14)
- Atomic-scale imaging of a 27-nuclear-spin cluster using a single-spin quantum sensor
- Three-dimensional localization spectroscopy of individual nuclear spins with sub-Angstrom resolution
- Randomisation of Pulse Phases for Unambiguous and Robust Quantum Sensing
- Magnetic field imaging by hBN quantum sensor nanoarray
- Three-dimensional nuclear spin positioning using coherent radio-frequency control
- Construction and operation of a tabletop system for nanoscale magnetometry with single nitrogen-vacancy centers in diamond
- Parallel detection and spatial mapping of large nuclear spin clusters
- Reconstruction-free quantum sensing of arbitrary waveforms
- Detection and control of single proton spins in a thin layer of diamond grown by chemical vapor deposition
- Spin coherence and depths of single nitrogen-vacancy centers created by ion implantation into diamond via screening masks
- Multidimensional spectroscopy of nuclear spin clusters in diamond
- Suppression of Pulsed Dynamic Nuclear Polarization by Many-Body Spin Dynamics
- Systematic investigation of dynamic nuclear polarization with boron vacancy in hexagonal boron nitride
- Estimation of nuclear polarization via discrete measurement of NV center spin evolution