High resolution spectroscopy of single NV defects coupled with nearby ${}^{13}$C nuclear spins in diamond

Abstract

We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby ${}^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a set of discrete values of the hyperfine coupling strength ranging from 14 MHz to 400 kHz and corresponding to ${}^{13}$C nuclear spins placed at different lattice sites of the diamond matrix. For each lattice site, the hyperfine interaction is further investigated through nuclear spin polarization measurements and by studying the magnetic field dependence of the hyperfine splitting. This work provides informations that are relevant for the development of nuclear-spin based quantum register in diamond.

8 pages, 5 figures

References in corpus (7)

• High-fidelity projective readout of a solid-state spin quantum register
• Dynamic polarization of single nuclear spins by optical pumping of NV color centers in diamond at room temperature
• Ab initio supercell calculations on nitrogen-vacancy center in diamond: its electronic structure and hyperfine tensors
• Coherence of single spins coupled to a nuclear spin bath of varying density
• Excited-state spectroscopy of single NV defects in diamond using optically detected magnetic resonance
• Excited-state spectroscopy using single-spin manipulation in diamond
• Time-averaging within the excited state of the nitrogen-vacancy centre in diamond

Cited by in corpus (63)

• Sensitivity Optimization for NV-Diamond Magnetometry
• Detection and control of individual nuclear spins using a weakly coupled electron spin
• Sensing remote nuclear spins
• Decoherence of dipolar spin ensembles in diamond
• Sensing distant nuclear spins with a single electron spin
• Bulk Nuclear Polarization Enhanced at Room-Temperature by Optical Pumping
• Ultralong Dephasing Times in Solid-State Spin Ensembles via Quantum Control
• Quantum frequency conversion to telecom of single photons from a nitrogen-vacancy center in diamond
• Noisy intermediate-scale quantum computers
• CVD diamond single crystals with NV centres: a review of material synthesis and technology for quantum sensing applications
• Competition between electric field and magnetic field noise in the decoherence of a single spin in diamond
• Local and bulk 13C hyperpolarization in NV-centered diamonds at variable fields and orientations
• Optical polarization of nuclear ensembles in diamond
• Single-shot readout of multiple nuclear spin qubits in diamond under ambient conditions
• Generating Large Cats with Nine Lives: Long-Lived Macroscopically Distinct Superposition States in Atomic Ensembles
• Nonvolatile quantum memory enables sensor unlimited nanoscale spectroscopy of finite quantum systems
• Theoretical model of the dynamic spin polarization of nuclei coupled to paramagnetic point defects in diamond and silicon carbide
• Probing the coherence of solid-state qubits at avoided crossings
• Systematic study of defect-related quenching of NV luminescence in diamond with time correlated single photon counting spectroscopy
• Sidebands in Optically Detected Magnetic Resonance Signals of Nitrogen Vacancy Centers in Diamond
• Entanglement of dark electron-nuclear spin defects in diamond
• Multi-spin-assisted optical pumping of bulk 13C nuclear spin polarization in diamond
• Observing information backflow from controllable non-Markovian multi-channels in diamond
• Free induction decay of single spins in diamond
• Non-flipping 13C spins in NV diamond: Hyperfine and Spatial Characteristics by DFT Simulation of the C510[NV]H252 Cluster
• Coherent population trapping of a single nuclear spin under ambient conditions
• Microwave-Free Nuclear Magnetic Resonance at Molecular Scales
• Dynamic ${}^{14}\mathrm{N}$ nuclear spin polarization in nitrogen-vacancy centers in diamond
• Dynamically Polarizing Spin Register of NV Centers in Diamond using Chopped Laser Pulses
• Measurement of the excited-state transverse hyperfine coupling in NV centers via dynamic nuclear polarization
• Hyperfine level structure in nitrogen-vacancy centers near the ground-state level anticrossing
• Efficient quantum error correction of dephasing induced by a common fluctuator
• Complete Quantum-State Tomography with a Local Random Field
• Vector magnetic field sensing by single nitrogen vacancy center in diamond
• Protection of center-spin coherence by dynamically polarizing nuclear spin core in diamond
• Statistical Inference with Quantum Measurements: Methodologies for Nitrogen Vacancy Centers in Diamond
• Probing the dynamics of a nuclear spin bath in diamond through time-resolved central spin magnetometry
• Broadband Excitation by Chirped Pulses: Application to Single Electron Spins in Diamond
• Spin Coherence and ${}^{14}$N ESEEM Effects of Nitrogen-Vacancy Centers in Diamond with X-band Pulsed ESR
• Resolving Remoter Nuclear Spins in a Noisy Bath by Dynamical Decoupling Design
• Dark State Polarizing a Nuclear Spin in the Vicinity of a Nitrogen-Vacancy Center
• Stimulated Raman Adiabatic control of a nuclear spin in diamond
• Decoherence of Nuclear Spins in the Proximity of Nitrogen Vacancy Centers in Diamond
• Divergent effects of laser irradiation on ensembles of nitrogen-vacancy centers in bulk and nano-diamonds: implications for biosensing
• Continuous microwave hole burning and population oscillations in a diamond spin ensemble
• Laser-written waveguide-integrated coherent spins in diamond
• Effect of inter-system crossing rates and optical illumination on the polarization of nuclear spins nearby nitrogen-vacancy centers
• Strongly polarizing weakly coupled ${}^{13}$C nuclear spins with optically pumped nitrogen-vacancy center
• Magnetic-field-induced delocalization in hybrid electron-nuclear spin ensembles
• Impact of helium ion implantation dose and annealing on dense near-surface layers of NV centers
• Ambiguous Resonances in Multipulse Quantum Sensing with Nitrogen Vacancy Centers
• Strong polarization of individual nuclear spins weakly coupled to nitrogen-vacancy color centers in diamond
• The NV center as a quantum actuator: time-optimal control of nuclear spins
• Optimal photon energies for initialization of hybrid spin quantum registers of NV centers in diamond
• Investigation of room temperature multispin-assisted bulk diamond 13C hyperpolarization at low magnetic fields
• Direct Readout of Nitrogen-Vacancy Hybrid-Spin Quantum Register in Diamond by Photon Arrival Time Analysis
• Nuclear spin temperature reversal via continuous radio-frequency driving
• Defying Conventional Wisdom in Spectroscopy: Power Narrowing on IBM Quantum
• Dynamic-nuclear-polarization-weighted spectroscopy of multi-spin electronic-nuclear clusters
• Optically pumped spin polarization as a probe of many-body thermalization
• Trans-dimensional Hamiltonian model selection and parameter estimation from sparse, noisy data
• Modulator-Assisted Zeno Control of Energy Transfer in Quantum Batteries
• Suppression of spin bath and low-frequency noise for sub-MHz AC magnetometry based on double-dressed spin qubit in diamond