Pulse-width-induced polarization enhancement of optically-pumped N-V electron spin in diamond
arXiv:1912.06284
Abstract
The nitrogen-vacancy (N-V) center in diamond is a widely-used platform for quantum information processing and metrology. The electron-spin state of N-V center could be initialized and readout optically, and manipulated by resonate microwave fields. In this work, we analyze the dependence of electron-spin initialization on widths of laser pulses. We build a numerical model to simulate this process and verify the simulation results in experiment. Both simulations and experiments reveal a fact that shorter laser pulses are helpful to the electron-spin polarization. We therefore propose to use extremely-short laser pulses for electron-spin initialization. In this new scheme, the spin-state contrast could be improved about 10% in experiment by using laser pulses as short as 4 ns in width. Furthermore, we provide a mechanism to explain this effect which is due to the occupation time in the meta-stable spin-singlet states of N-V center. Our new scheme is applicable in a broad range of NV-based applications in the future.
7 pages, 4 figures
References in corpus (11)
- High-fidelity projective readout of a solid-state spin quantum register
- Nanoscale magnetic imaging of a single electron spin under ambient conditions
- Dynamic polarization of single nuclear spins by optical pumping of NV color centers in diamond at room temperature
- Decoherence-protected quantum gates for a hybrid solid-state spin register
- Detection and control of individual nuclear spins using a weakly coupled electron spin
- Polarization and readout of coupled single spins in diamond
- Efficient readout of a single spin state in diamond via spin-to-charge conversion
- Optical properties of the nitrogen-vacancy singlet levels in diamond
- Phonon-Induced Population Dynamics and Intersystem Crossing in Nitrogen-Vacancy Centers
- State-selective intersystem crossing in nitrogen-vacancy centers
- Efficient electrical spin readout of NV- centers in diamond