Mapping the Spatial Distribution of Charge Carriers in LaAlO3/SrTiO3 Heterostructures
arXiv:0710.1395 · doi:10.1038/nmat2223
Abstract
At the interface between complex insulating oxides, novel phases with interesting properties may occur, such as the metallic state reported in the LaAlO3/SrTiO3 system. While this state has been predicted and reported to be confined at the interface, some works indicate a much broader spatial extension, thereby questioning its origin. Here we provide for the first time a direct determination of the carrier density profile of this system through resistance profile mappings collected in cross-section LaAlO3/SrTiO3 samples with a conducting-tip atomic force microscope (CT-AFM). We find that, depending upon specific growth protocols, the spatial extension of the high-mobility electron gas can be varied from hundreds of microns into SrTiO3 to a few nanometers next to the LaAlO3/SrTiO3 interface. Our results emphasize the potential of CT-AFM as a novel tool to characterize complex oxide interfaces and provide us with a definitive and conclusive way to reconcile the body of experimental data in this system.
This updated version contains new experimental data
References in corpus (6)
- Magnetic effects at the interface between nonmagnetic oxides
- Why Some Interfaces Cannot be Sharp
- The role of oxygen vacancies in SrTiO3 at the LaAlO3/SrTiO3 interface
- High Mobility in LaAlO3/SrTiO3 Heterostructures: Origin, Dimensionality and Perspectives
- Origin of charge density at LaAlO3-on-SrTiO3 hetero-interfaces; possibility of intrinsic doping
- Electron energy loss spectroscopy determination of Ti oxidation state at the (001) LaAlO3/SrTiO3 interface as a function of LaAlO3 growth conditions
Cited by in corpus (111)
- Electric Field Control of the LaAlO/SrTiO Interface Ground State
- Tunable Rashba spin-orbit interaction at oxide interfaces
- Unveiling a two-dimensional electron gas with universal subbands at the surface of SrTiO3
- Tuning spin-orbit coupling and superconductivity at the SrTiO3/LaAlO3 interface: a magneto-transport study
- Avoiding the polarization catastrophe in LaAlO3 overlayers on SrTiO3(001) through a polar distortion
- Orbital reconstruction and two-dimensional electron gas at the LaAlO3/SrTiO3 interface
- Physics of SrTiO-based heterostructures and nanostructures: a review
- Two-dimensional superconductivity at a Mott-Insulator/Band-Insulator interface: LaTiO3/SrTiO3
- Profiling the interface electron gas of LaAlO3/SrTiO3 heterostructures by hard X-ray photoelectron spectroscopy
- Dominant mobility modulation by the electric field effect at the LaAlO_3 / SrTiO_3 interface
- Two-dimensional quantum oscillations of the conductance at LaAlO3/SrTiO3 interfaces
- Large capacitance enhancement and negative compressibility of two-dimensional electronic systems at LaAlO/SrTiO interfaces
- Origin of the two-dimensional electron gas at LaAlO3/SrTiO3 interfaces: The role of oxygen vacancies and electronic reconstruction
- Observation of Inverse Edelstein Effect in Rashba-Split 2DEG between SrTiO3 and LaAlO3 at Room Temperature
- Nonlinear Hall effect and multichannel conduction in LaTiO3/SrTiO3 superlattices
- Towards two-dimensional metallic behavior at LaAlO3/SrTiO3 interfaces
- Origin of two-dimensional electron gases at oxide interfaces: insights from theory
- Direct k-space mapping of the electronic structure in an oxide-oxide interface
- Rewritable nanoscale oxide photodetector
- Nanoscale Phenomena in Oxide Heterostructures
- Polarity-induced oxygen vacancies at LaAlO3|SrTiO3 interfaces
- Oxygen vacancies at titanate interfaces: two-dimensional magnetism and orbital reconstruction
- Conducting interfaces between band insulating oxides: the LaGaO3/SrTiO3
- Polar catastrophe and electronic reconstructions at the LaAlO3/SrTiO3 interface: evidence from optical second harmonic generation
- Two-dimensional Superconductors with Atomic-scale Thicknesses
- Parallel electron-hole bilayer conductivity from electronic interface reconstruction
- Two-dimensional electron liquid state at LaAlO3-SrTiO3 interfaces
- Dynamical response and confinement of the electrons at the LaAlO3/SrTiO3 interface
- Rashba induced magnetoconductance oscillations in the LaAlO3-SrTiO3 heterostructure
- Controlling the density of the 2DEG at the SrTiO3/LaAlO3 interface
- Mechanisms of charge transfer and redistribution in LaAlO3/SrTiO3 revealed by high-energy optical conductivity
- Electronic structure induced reconstruction and magnetic ordering at the LaAlOSrTiO interface
- Electronic charges and electric potential at LaAlO3/SrTiO3 interfaces studied by core-level photoemission spectroscopy
- Oxide superlattices with alternating p and n interfaces
- In-plane electronic confinement in superconducting LaAlO/SrTiO nanostructures
- Stoichiometry control of the electronic properties of the LaAlO_3/SrTiO_3 heterointerface
- Ferroelectric Dead Layer Driven by a Polar Interface
- Gate-tunable band structure of the LaAlO-SrTiO interface
- Antisymmetric magnetoresistance of the SrTiO3/LaAlO3 interface
- Current-driven spin orbit field in LaAlO3/SrTiO3 heterostructures
- Persistent photoconductivity in 2-dimensional electron gases at different oxide interfaces
- Ab initio study of the two-dimensional metallic state at the surface of SrTiO3: importance of oxygen vacancies
- Tuning the metal-insulator transition in d^1 and d^2 perovskites by epitaxial strain: a first principles-based study
- Band offsets and density of Ti3+ states probed by X-ray photoemission on LaAlO3/SrTiO3 heterointerfaces and their LaAlO3 and SrTiO3 bulk precursors
- Prediction of a spin-polarized two-dimensional electron gas at the LaAlO3/EuO(001) interface
- A First-Principles Study of the Electronic Reconstructions of LaAlO3/SrTiO3 Heterointerfaces and Their Variants
- Nanometer-scale striped surface terminations on fractured SrTiO surfaces
- Interface relaxation and electrostatic charge depletion in the oxide heterostructure LaAlO3/SrTiO3
- New insights into the electron trapping mechanism in LaAlO_3 / SrTiO3 heterostructures
- Seebeck effect in the conducting LaAlO_{3}/SrTiO_{3} interface
- Controlling Kondo-like Scattering at the SrTiO3-based Interfaces
- Gate Tunable In- and Out-Of-Plane Spin-Orbit Coupling and Spin Splitting Anisotropy at LaAlO3/SrTiO3 (110) Interface
- Appearance and disappearance of ferromagnetism in ultra-thin LaMnO on SrTiO substrate: a viewpoint from first-principles
- Modulation of the superconducting critical temperature due to quantum confinement at the LaAlO/SrTiO interface
- Nanoscale rectification at the LaAlO3/SrTiO3 interface
- Electron energy loss spectroscopy determination of Ti oxidation state at the (001) LaAlO3/SrTiO3 interface as a function of LaAlO3 growth conditions
- Photoresponse dynamics in amorphous-LaAlO/SrTiO interfaces
- Shape Resonances in superconducting gaps in a 2DEG at oxide-oxide interface
- Large band offset as driving force of 2-dimensional electron confinement: the case of SrTiO/SrZrO interface
- Effect of disorder on superconductivity and Rashba spin-orbit coupling in LaAlO3/SrTiO3 interfaces
- A switchable two-dimensional electron gas based on ferroelectric Ca:SrTiO
- Correlated electronic states of SrVO3 revealed by angle-resolved photoemission spectroscopy
- Detection of confined current paths on oxide surfaces by local-conductivity atomic force microscopy with atomic resolution
- Electronic structure of the SrTiO/LaAlO interface revealed by resonant soft x-ray scattering
- Mechanism to Generate a Two-Dimensional Electron Gas at the Surface of the Charge-Ordered Semiconductor BaBiO3
- Electronic phase separation at LaAlO3/SrTiO3 interfaces tunable by oxygen deficiency
- Orientation-dependent electron-phonon coupling in interfacial superconductors LaAlO3/KTaO3
- Large polarons as key quasiparticles in SrTiO3 and SrTiO3-based heterostructures
- Large Negative Electronic Compressibility of LaAlO3-SrTiO3 Interfaces with Ultrathin LaAlO3 Layers
- Tuning Rashba spin-orbit coupling at LaAlO3/SrTiO3 interfaces by band filling
- Metallicity of the SrTiO3 surface induced by room temperature evaporation of alumina
- Evolution of the SrTiO surface electronic state as a function of LaAlO overlayer thickness
- Upper critical field as a probe for multiband superconductivity in bulk and interfacial STO
- Enhanced spin-orbit coupling and charge carrier density suppression in LaAl1-xCrxO3/SrTiO3 heterointerfaces
- Visualizing nanoscale electronic band alignment at the LaCaMnO/Nb:SrTiO interface
- Microstructure and interface studies of LaVO3/SrVO3 superlattices
- Anomalous response to gate voltage application in mesoscopic LaAlO_3/SrTiO_3 devices
- Assessing electron beam sensitivity for SrTiO and LaSrMnO using electron energy loss spectroscopy
- Infrared ellipsometry study of the confined electrons in a high-mobility -AlO/SrTiO heterostructure
- Metal-insulator transition at the LaAlO3/SrTiO3 interface revisited: A hybrid functional study
- Self-consistent iteration procedure in analyzing reflectivity and spectroscopic ellipsometry data of multilayered materials and their interfaces
- Electronic charge redistribution in LaAlO(001) thin films deposited at SrTiO(001) substrate: First principles analysis and the role of stoichiometry
- Electronic Structure of Oxide Interfaces: A Comparative Analysis of GdTiO/SrTiO and LaAlO/SrTiO Interfaces
- The Conducting Channel at the LaAlO/SrTiO Interface
- Two components for one resistivity in LaVO3/SrTiO3 heterostructures
- Polarization screening and induced carrier density at the interface of LaAlO overlayer on SrTiO (001)
- Raman and fluorescence contributions to resonant inelastic soft x-ray scattering on LaAlO/SrTiO heterostructures
- Structural transition in LaVO3/SrVO3 superlattices and its influence on transport properties
- Influence of oxygen pressure and aging on LaAlO3 films grown by pulsed laser deposition on SrTiO3 substrates
- Probing Quantum Confinement and Electronic Structure at Polar Oxide Interfaces
- A survey of fractured SrTiO surfaces: from the micro-meter to nano-meter scale
- Long-range electronic reconstruction to a -dominated Fermi surface below the LaAlO/SrTiO interface
- Interplay between sheet resistance increase and magnetotransport properties in
- Oxide tunnel junctions supporting a two-dimensional electron gas
- Temperature-Dependent Band Structure of SrTiO Interfaces
- Two-dimensional electron systems in perovskite oxide heterostructures: Role of the polarity-induced substitutional defects
- Infrared study of the quasi-two-dimensional electron system at the interface between SrTiO and crystalline or amorphous LaAlO
- Laterally-confined two-dimensional electron gases in self-patterned LaAlO3/SrTiO3 interfaces
- Artificial quantum confinement in LAO3/STO heterostructure
- Effect of oxygen vacancy on structural, electronic and magnetic properties of La-based oxide interfaces
- Thermal Activation and Quantum Field Emission in a Sketch-Based Oxide Nano Transistor
- Gate voltage control of the / interface electrical properties
- Direct Imaging of Sketched Conductive Nanostructures at the LaAlO3/SrTiO3 Interface
- The Vortex Signature of Discrete Ferromagnetic Dipoles at the LaAlO/SrTiO Interface
- Understanding the role of exchange and correlations in complex oxides under strain and oxide heterostructures
- A tool to estimate the critical dynamics and thickness of superconducting films and interfaces
- In situ investigation of conducting interface formation in LaAlO3/SrTiO3 heterostructure
- δ-doped LaAlO3-SrTiO3 interface: Electrical transport and characterization of the interface potential
- Structural phase transitions in Ruddlesden-Popper phases of strontium titanate: {\em ab initio} and inhomogeneous Ginzburg-Landau approaches
- Polarity-field driven conductivity in SrTiO/LaAlO: a hybrid functional study
- Local inhomogeneities resolved by scanning probe techniques and their impact on local 2DEG formation in oxide heterostructures