Understanding the role of exchange and correlations in complex oxides under strain and oxide heterostructures

Abstract

The study of complex oxides and oxide heterostructures have dominated the field of experimental and theoretical condensed matter research for the better part of the last few decades. Powerful experimental techniques like molecular beam epitaxy and pulsed laser deposition have made fabrication of oxide heterostructures with atomically sharp interfaces possible, while more and more sophisticated handling of exchange and correlations within first principles methods including density functional theory (DFT) supplemented with Hubbard U corrections and hybrid functionals, and beyond DFT techniques like dynamical mean field theory (DMFT) have made understanding of such correlated oxides and oxide interfaces easier. The emergence of the high mobility two dimensional electron gas with fascinating properties like giant photoconductance, large negative magnetoresistance, superconductivity, ferromagnetism, and the mysterious coexistence of the latter two have indeed caught the attention of condensed matter community at large. Similarly strain tuning of oxides have generated considerable interest particularly after the recent discovery of piezoelectric methods of strain generation. Theoretical understanding and prediction of the possible exotic phases emerging in such complex oxides both under strain and in heterostructures will eventually lead to better design of device applications in this new emerging field of oxide electronics, along with possible discovery of exotic physics in condensed matter systems which may be of wider significance! In this review we briefly look at theoretical studies of novel phenomena in oxides under strain and oxide heterostructures, and try to understand the role of exchange and particularly correlation in giving rise to such exotic electronic states.

References in corpus (8)

• Magnetic effects at the interface between nonmagnetic oxides
• Origin of charge density at LaAlO3-on-SrTiO3 hetero-interfaces; possibility of intrinsic doping
• Avoiding the polarization catastrophe in LaAlO3 overlayers on SrTiO3(001) through a polar distortion
• Electronic reconstruction at SrMnO3-LaMnO3 superlattice interfaces
• Carrier-controlled ferromagnetism in SrTiO3
• Electronic structure induced reconstruction and magnetic ordering at the LaAlO${}_3|$SrTiO${}_3$ interface
• Charge states and magnetic ordering in LaMnO3/SrTiO3 superlattices
• Dimer Mott Insulator in an Oxide Heterostructure

Cited by in corpus (3)

• The importance of electronic correlations in exploring the exotic phase diagram of layered Li${}_x$MnO${}_2$
• Tuning Electronic and Optical Properties of 2D/3D Construction based on Hybrid Perovskites through Interfacial Charge Transfer: Towards Higher Efficiency Solar Cells
• Decoupling the effects of geometry and nature of strain in LaMnO${}_3$: Interplay of dynamic correlations and uniaxial strain driving magnetic phase transitions