Large nonsaturating magnetoresistance and signature of non-degenerate Dirac nodes in ZrSiS

Abstract

While the discovery of Dirac and Weyl type excitations in electronic systems is a major breakthrough in recent condensed matter physics, finding appropriate materials for fundamental physics and technological applications, is an experimental challenge. In all the reported materials, linear dispersion survives only up to a few hundred meV from the Dirac or Weyl nodes. On the other hand, real materials are subject to uncontrolled doping during preparation and thermal effect near room temperature can hinder the rich physics. In ZrSiS, ARPES measurements have shown an unusually robust linear dispersion (up to $\sim$2 eV) with multiple non-degenerate Dirac nodes. In this context, we present the magnetotransport study on ZrSiS crystal, which represents a large family of materials (\textit{WHM} with \textit{W} = Zr, Hf; \textit{H} = Si, Ge, Sn; \textit{M} = O, S, Se, Te) with identical band topology. Along with extremely large and non-saturating magnetoresistance (MR), $\sim$ 1.4 $\times$ 10${}^5$ \% at 2 K and 9 T, it shows strong anisotropy depending on the direction of the magnetic field. Quantum oscillation and Hall effect measurements have revealed large hole and small electron Fermi pockets. Non-trivial $\pi$ Berry phase confirms the Dirac fermionic nature for both types of charge carriers. The long-sought relativistic phenomenon of massless Dirac fermions, known as Adler-Bell-Jackiw chiral anomaly, has also been observed.

10 pages, 13 figures

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• Chemical Principles of Topological Semimetals
• Nodal-knot semimetals
• Dirac Line-nodes and Effect of Spin-orbit Coupling in Non-symmorphic Critical Semimetal MSiS (M=Hf, Zr)
• Unconventional mass enhancement around the Dirac nodal loop in ZrSiS
• Nearly massless Dirac fermions and strong Zeeman splitting in the nodal-line semimetal ZrSiS probed by de Haas--van Alphen quantum oscillations
• Tunability of the topological nodal-line semimetal phase in ZrSiX-type materials
• Topological Semimetals in Square-Net Materials
• High mobility in a van der Waals layered antiferromagnetic metal
• Quantum Transport in Topological Semimetals under Magnetic Fields
• Giant anisotropic magnetoresistance and planar Hall effect in the Dirac semimetal Cd3As2
• Quantum transport evidence of Weyl fermions in an epitaxial ferromagnetic oxide
• Rules for Phase Shifts of Quantum Oscillations in Topological Nodal-line Semimetals
• Weyl-link semimetals
• Observation of topological nodal-line fermionic phase in GdSbTe
• Flat optical conductivity in ZrSiS due to two-dimensional Dirac bands
• Thermoelectric quantum oscillations in ZrSiS
• Two-dimensional Spin-Orbit Dirac Point in Monolayer HfGeTe
• Giant magnetoresistance of Dirac plasma in high-mobility graphene
• Magnetotransport properties and evidence of topological insulating state in LaSbTe
• Planar Hall effect in type II Dirac semimetal VAl${}_3$
• Quantum oscillation studies of topological semimetal candidate ZrGeM (M=S, Se, Te)
• Evidence of topological insulator state in the semimetal LaBi
• Unusual magneto-transport from Si-square nets in topological semimetal HfSiS
• Floquet multi-Weyl points in crossing-nodal-line semimetals
• Origin of the Extremely Large Magnetoresistance in the Semimetal YSb
• Extremely large magnetoresistance in topologically trivial semimetal $\alpha$-WP${}_2$
• Excitonic Instability and Pseudogap Formation in Nodal Line Semimetal ZrSiS
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• Ideal inner nodal chain semimetals in Li2XY (X = Ca, Ba; Y = Si, Ge) materials
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• Crossing-Line-Node Semimetals: General Theory and Application to Rare-Earth Trihydrides
• Fermi surface topology and signature of surface Dirac nodes in LaBi
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• Electron transport in nodal-line semimetals
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• Probing lattice dynamics and electron-phonon coupling in topological nodal-line semimetal ZrSiS
• Electronic and Magnetic Properties of Topological Semimetal Candidate NdSbTe
• Electronic Transport Evidence for Topological Nodal-Line Semimetals of ZrGeSe single crystals
• Evolving Devil's staircase magnetization from tunable charge density waves in nonsymmorphic Dirac semimetals
• Galvanomagnetic properties of the putative type-II Dirac semimetal PtTe${}_2$
• Observation of multiple nodal-lines in SmSbTe
• Observation of Effective Pseudospin Scattering in ZrSiS
• Observation of Open-Orbit Fermi Surface Topology in Extremely Large Magnetoresistance Semimetal MoAs${}_2$
• Thickness-dependent quantum transport of Weyl fermions in ultra-high-quality SrRuO3 films
• Topology of Triple-Point Metals
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• Chemical pressure effect on the optical conductivity of the nodal-line semimetals ZrSi$Y$ ($Y$=S, Se, Te) and ZrGe$Y$ ($Y$=S, Te)
• Quantum oscillation evidence of topological semimetal phase in ZrSnTe
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• Charge density wave induced nodal lines in LaTe${}_3$
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• Experimental evidence of crystal symmetry protection for the topological nodal line semimetal state in ZrSiS
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