Giant magnetoresistance, Fermi surface topology, Shoenberg effect and vanishing quantum oscillations in type-II Dirac semimetal candidates MoSi${}_2$ and WSi${}_2$

Abstract

We performed comprehensive theoretical and experimental studies of the electronic structure and the Fermi surface topology of two novel quantum materials, MoSi${}_2$ and WSi${}_2$. The theoretical predictions of the electronic structure in the vicinity of the Fermi level was verified experimentally by thorough analysis of the observed quantum oscillations in both electrical resistivity and magnetostriction. We established that the Fermi surface sheets in MoSi${}_2$ and WSi${}_2$ consist of 3D dumbbell-shaped hole-like pockets and rosette-shaped electron-like pockets, with nearly equal volumes. Based on this finding, both materials were characterized as almost perfectly compensated semimetals. In conjunction, the magnetoresistance attains giant values of $10^4$ and $10^5\%$ for WSi${}_2$ and MoSi${}_2$, respectively. In turn, the anisotropic magnetoresistance achieves $-95$ and $-98\%$ at $T=2$K and in $B=14$T for WSi${}_2$ and MoSi${}_2$, respectively. Furthermore, for both compounds we observed the Shoenberg effect in their Shubnikov-de Haas oscillations that persisted at as high temperature as $T=25$K in MoSi${}_2$ and $T=12$K in WSi${}_2$. In addition, we found for MoSi${}_2$ a rarely observed spin-zero phenomenon. Remarkably, the electronic structure calculations revealed type-II Dirac cones located near 480 meV and 710 meV above the Fermi level in MoSi${}_2$ and WSi${}_2$, respectively.

arXiv comment33 pages, 8 figures, +(Supplemental Material: 6 pages, 5 figures); Accepted for publication in Physical Review B

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• Quantum Oscillations of the Quasiparticle Lifetime in a Metal
• Transverse thermoelectric conversion in the mixed-dimensional semimetal WSi${}_2$
• Comprehensive investigation of Quantum Oscillations in Semimetal Using an ac Composite Magnetoelectric Technique with Ultrahigh Sensitivity
• Room temperature spin-orbit torque efficiency in sputtered low-temperature superconductor delta-TaN
• Temperature-driven changes in the Fermi surface of graphite
• Floquet composite Dirac semimetals
• Anomalous quantum oscillations from boson-mediated interband scattering
• Fermi surface and Berry phase analysis for Dirac nodal line semimetals: cautionary tale to SrGa${}_2$ and BaGa${}_2$