Electronic properties of a heavy-fermion U(Ru0.92Rh0.08)2Si2 single crystal

Abstract

We report the crystal structure and highly-anisotropic magnetic, transport and thermal properties of an exceptionally good single crystal of U(Ru0.92Rh0.08)2Si2 prepared using a modified Czochralski method. Our study, that also includes neutron diffraction results, shows all the heavy-fermion signatures of pristine URu2Si2 , however, the superconductivity, hidden order and remanent weak antiferromagnetic orders are absent. Instead, the ground state of the doped system can be classified as a spin liquid that preserves the heavy-fermion character. U(Ru0.92Rh0.08)2Si2 exhibits a short-range magnetic order distinguished by reflections of a Lorentzian profile at qIII = (1/2 1/2 1/2) positions that disappear above approx. 15 K. The short-range order seems to be a precursor of a long-range magnetic order that occurs with higher Rh concentration. We indicate that these short-range fluctuations involve, at least partially, inelastic scattering processes.

arXiv comment12 Figures

References in corpus (18)

• Colloquium: Hidden Order, Superconductivity, and Magnetism -- The Unsolved Case of URu2Si2
• Effect of Pressure on Tiny Antiferromagnetic Moment in the Heavy-Electron Compound URu_2Si_2
• High Field Studies of the Hidden Order Transition in URu${}_2$Si${}_2$
• Hidden Order Behaviour in URu2Si2 (A Critical Review of the Status of Hidden Order in 2014)
• Interplay between Fermi surface topology and ordering in URu${}_2$Si${}_2$ revealed through abrupt Hall coefficient changes in strong magnetic fields
• Competing Ordered Phases in URu2Si2: Hydrostatic Pressure and Re-substitution
• Neutron Scattering Study on Competition between Hidden Order and Antiferromagnetism in U(Ru_{1-x}Rh_x)_2Si_2 (x <= 0.05)
• Field-induced spin-density wave beyond hidden order in URu2Si2
• Chemical pressure tuning of URu${}_2$Si${}_2$ via isoelectronic substitution of Ru with Fe
• Antiferromagnetism and Hidden Order in Isoelectronic Doping of URu${}_2$Si${}_2$
• The suppression of hidden order and onset of ferromagnetism in URu2Si2 via Re substitution
• Wilson and Kadowaki-Woods Ratios in Heavy Fermions
• Strict limit on in-plane ordered magnetic dipole moment in URu2Si2
• Lattice dynamics of the heavy fermion compound URu${}_2$Si${}_2$
• Uncovering the Hidden Order in URu2Si2 by Impurity Doping
• Detailed optical spectroscopy of the hybridization gap and the hidden order transition in high quality URu${}_2$Si${}_2$ single crystals
• Neutron Scattering Study of URu${}_{2-x}$Re${}_x$Si${}_2$ with $x$ = 0.10: Driving Order towards Quantum Criticality
• Ultrasonic Study of the Hidden Order and Heavy-Fermion State in URu${}_2$Si${}_2$ with Hydrostatic Pressure, Rh-doping, and High-Magnetic Fields

Cited by in corpus (7)

• Hidden order and beyond: an experimental-theoretical overview of the multifaceted behavior of URu${}_2$Si${}_2$
• Giant magnetoresistance, Fermi surface topology, Shoenberg effect and vanishing quantum oscillations in type-II Dirac semimetal candidates MoSi${}_2$ and WSi${}_2$
• Magnetic structure in U(Ru0.92Rh0.08)2Si2 single crystal studied by neutron diffraction in static magnetic fields up to 24 T
• Fe substitution in URu${}_2$Si${}_2$: singlet magnetism in an extended Doniach phase diagram
• Field-induced phases in a heavy-fermion U(Ru${}_{0.92}$Rh${}_{0.08}$)${}_2$Si${}_2$ single crystal
• Preparation of large Cu3Sn single crystal by Czochralski method
• Collinear antiferromagnetic order in URu${}_2$Si${}_{2-x}$P${}_x$ revealed by neutron diffraction