Dielectric nano-antennas for strain engineering in atomically thin two-dimensional semiconductors

Abstract

Atomically thin two-dimensional semiconducting transition metal dichalcogenides (TMDs) can withstand large levels of strain before their irreversible damage occurs. This unique property offers a promising route for control of the optical and electronic properties of TMDs, for instance by depositing them on nano-structured surfaces, where position-dependent strain can be produced on the nano-scale. Here, we demonstrate strain-induced modifications of the optical properties of mono- and bilayer TMD WSe${}_2$ placed on photonic nano-antennas made from gallium phosphide (GaP). Photoluminescence (PL) from the strained areas of the TMD layer is enhanced owing to the efficient coupling with the confined optical mode of the nano-antenna. Thus, by following the shift of the PL peak, we deduce the changes in the strain in WSe${}_2$ deposited on the nano-antennas of different radii. In agreement with the presented theory, strain up to $\approx 1.4\%$ is observed for WSe${}_2$ monolayers. We also estimate that $>3\%$ strain is achieved in bilayers, accompanied with the emergence of a direct bandgap in this normally indirect-bandgap semiconductor. At cryogenic temperatures, we find evidence of the exciton confinement in the most strained nano-scale parts of the WSe${}_2$ layers, as also predicted by our theoretical model. Our results, of direct relevance for both dielectric and plasmonic nano-antennas, show that strain in atomically thin semiconductors can be used as an additional parameter for engineering light-matter interaction in nano-photonic devices.

peer-reviewed version, 4 figures main text, 5 figures supporting information

References in corpus (6)

• Magnetic light
• k.p theory for two-dimensional transition metal dichalcogenide semiconductors
• Evidence of high-temperature exciton condensation in 2D atomic double layers
• A strain tunable single-layer MoS2 photodetector
• Variation of the fundamental band gap nature in curved two-dimensional WS2
• Impact of strain on the optical fingerprint of monolayer transition metal dichalcogenides

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