Gate-dependent Pseudospin Mixing in Graphene/Boron Nitride Moire Superlattices
arXiv:1405.2032 · doi:10.1038/nphys3075
Abstract
Electrons in graphene are described by relativistic Dirac-Weyl spinors with a two-component pseudospin1-12. The unique pseudospin structure of Dirac electrons leads to emerging phenomena such as the massless Dirac cone2, anomalous quantum Hall effect2, 3, and Klein tunneling4, 5 in graphene. The capability to manipulate electron pseudospin is highly desirable for novel graphene electronics, and it requires precise control to differentiate the two graphene sub-lattices at atomic level. Graphene/boron nitride (graphene/BN) Moire superlattice, where a fast sub-lattice oscillation due to B-N atoms is superimposed on the slow Moire period, provides an attractive approach to engineer the electron pseudospin in graphene13-18. This unusual Moire superlattice leads to a spinor potential with unusual hybridization of electron pseudospins, which can be probed directly through infrared spectroscopy because optical transitions are very sensitive to excited state wavefunctions. Here, we perform micro-infrared spectroscopy on graphene/BN heterostructure and demonstrate that the Moire superlattice potential is dominated by a pseudospin-mixing component analogous to a spatially varying pseudomagnetic field. In addition, we show that the spinor potential depends sensitively on the gate-induced carrier concentration in graphene, indicating a strong renormalization of the spinor potential from electron-electron interactions. Our study offers deeper understanding of graphene pseudospin structure under spinor Moire potential, as well as exciting opportunities to control pseudospin in two-dimensional heterostructures for novel electronic and photonic nanodevices.
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Cited by in corpus (23)
- Observation of Moiré Excitons in WSe2/WS2 Heterostructure Superlattices
- Moiré heterostructures as a condensed matter quantum simulator
- Evidence of Gate-Tunable Mott Insulator in Trilayer Graphene-Boron Nitride Moiré Superlattice
- Configure polaritons in twisted -MoO3
- \textit{Ab-initio} Tight-Binding Hamiltonian for Transition Metal Dichalcogenides
- Second generation Dirac cones and inversion symmetry breaking induced gaps in graphene/hexagonal boron nitride
- New generation of moiré superlattices in doubly aligned hBN/graphene/hBN heterostructures
- Moire superlattice effects in graphene/boron-nitride van der Waals heterostructures
- Towards edge engineering of two-dimensional layered transition-metal dichalcogenides by chemical vapor deposition
- Fabry-Pérot resonances in a graphene/hBN Moiré superlattice
- Accurate Measurement of the Gap of Graphene/hBN Moiré Superlattice through Photocurrent Spectroscopy
- Moire miniband features in the angle-resolved photoemission spectra of graphene/hBN heterostructures
- Electronic structure of transferred graphene/h-BN van der Waals heterostructures with nonzero stacking angles by nano-ARPES
- Infrared absorption of closely-aligned heterostructures of monolayer and bilayer graphene with hexagonal boron nitride
- Inter-valley spiral order in the Mott insulating state of a heterostructure of trilayer graphene-boron nitride
- High-order minibands and interband Landau level reconstruction in graphene moire superlattice
- Interaction-induced metallic state in graphene on hexagonal boron nitride
- Enhanced valley polarization of graphene on hBN under circularly polarized light irradiation
- THz conductivity of graphene on boron nitride
- Imaging the Sub-Moiré Potential Landscape using an Atomic Single Electron Transistor
- Negative differential resistance in Van der Waals heterostructures due to moiré-induced spectral reconstruction
- Growth of hexagonal BN crystals by traveling-solvent floating zone
- Observation of Anomalous Moiré Patterns