Spin Dynamics of the Spin-1/2 Kagome Lattice Antiferromagnet ZnCu_3(OH)_6Cl_2
arXiv:cond-mat/0610539 · doi:10.1103/PhysRevLett.98.107204
Abstract
We have performed thermodynamic and neutron scattering measurements on the S=1/2 kagome lattice antiferromagnet Zn Cu_3 (OH)_6 Cl_2. The susceptibility indicates a Curie-Weiss temperature of ~ -300 K; however, no magnetic order is observed down to 50 mK. Inelastic neutron scattering reveals a spectrum of low energy spin excitations with no observable gap down to 0.1 meV. The specific heat at low-T follows a power law with exponent less than or equal to 1. These results suggest that an unusual spin-liquid state with essentially gapless excitations is realized in this kagome lattice system.
4 pages, 3 figures; v2: Updates to authors list and references; v3: Updated version; v4: Published version
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- Proximate Dirac spin liquid in honeycomb lattice - XXZ model: Numerical study and application to cobaltates
- Impurity-induced resonant spinon zero modes in Dirac quantum spin-liquids
- Magnetic resonance as a local probe for kagomé magnetism in Barlowite Cu(OH)FBr
- Quantum-critical scaling properties of the two-dimensional random-singlet state
- Disorder effects in the quantum kagome antiferromagnet ZnCu3(OH)6Cl2
- Signatures of fractionalization in spin liquids from interlayer thermal transport
- Recent progress on magnetic-field studies on quantum-spin-liquid candidates
- Classical and quantum order in hyperkagome antiferromagnets
- Spin Waves in the Ferromagnetic Ground State of the Kagome Staircase System Co3V2O8
- Classification of quantum phases for the star-lattice antiferromagnet via a projective symmetry group analysis
- Semionic resonating valence bond states
- The route to magnetic order in the spin- kagome Heisenberg antiferromagnet: The role of interlayer coupling
- Structure Factors of the Kagome-Lattice Heisenberg antiferromagnets at finite temperatures
- Semiclassical spin liquid state of easy axis Kagome antiferromagnets
- Thermodynamics of the kagome-lattice Heisenberg antiferromagnet with arbitrary spin
- Possible chiral spin liquid state in the kagome Heisenberg model
- Quantum phases of the frustrated XY models on the honeycomb lattice
- Destruction of valence-bond order in a sawtooth chain with a Dzyaloshinskii-Moriya term
- Cross-over from an incommensurate singlet spiral state with a vanishingly small spin-gap to a valence bond solid state in dimerized frustrated ferromagnetic spin-chains
- Magnetization Plateau Observed by Ultra-High Field Faraday Rotation in a Kagomé Antiferromagnet Herbertsmithite
- Breakdown of Fermi liquid behavior near the hot spots in a two-dimensional model: A two-loop renormalization group analysis
- Impurities in triangular lattice spin 1/2 antiferromagnet
- Ineffectiveness of the Dzyaloshinskii-Moriya interaction in the dynamical quantum phase transition in the ITF model
- Spin Correlations in the Geometrically Frustrated Pyrochlore Tb2Mo2O7
- Structure factor of low-energy spin excitations in a S=1/2 kagome antiferromagnet
- Numerical evidence for a chiral spin liquid in the XXZ antiferromagnetic Heisenberg model on the kagome lattice at magnetization
- Muon-Spin Spectroscopy of the organometallic spin 1/2 kagome-lattice compound Cu(1,3-benzenedicarboxylate)
- Ordered Phases of the Anisotropic Kagome Lattice Antiferromagnet in a Field
- Topological Superconductivity in Metal/Quantum-Spin-Ice Heterostructures
- Electronic tunability of the frustrated triangular-lattice cluster magnet LiZnMoO
- Sc_{2}Ga_{2}CuO_{7}: A possible Quantum spin liquid near the percolation threshold
- Spin Liquid States at the vicinity of metal-insulator transition
- Freezing of the Lattice in the Kagome Lattice Heisenberg Antiferromagnet Zn-barlowite ZnCu(OD)FBr
- Competeing orders in spin-1 and spin-3/2 XXZ Kagome antiferromagnets: A series expansion study
- Linear independence of nearest-neighbor valence bond states in several two-dimensional lattices
- Ising-type quantum spin liquid state in PrMgAlO
- Topological phases of the Kitaev-Hubbard Model at half-filling
- Transition-metal distribution in kagome antiferromagnet CoCu3(OH)6Cl2 revealed by resonant x-ray diffraction
- Raman scattering in correlated thin films as a probe of chargeless surface states
- Ultralow-temperature heat transport in the quantum spin liquid candidate Ca10Cr7O28 with bilayer kagome lattice
- Magnetic phase diagram of CuZn(OH)FBr studied by neutron-diffraction and SR techniques
- Schwinger Boson mean field theory of kagome Heisenberg antiferromagnet with Dzyaloshinskii-Moriya interaction
- Structures of magnetic excitations in the spin-1/2 kagome-lattice antiferromagnets CsCuSnF and RbCuSnF
- Low-Energy Excitations in Quantum Spin-Liquids Identified by Optical Spectroscopy
- Theory of Néel and Valence-Bond-Solid Phases on the Kagome Lattice of Zn-paratacamite
- Doping on the kagome lattice: A variational Monte-Carlo study of the model
- Resonating Valence-Bond State in an Orbitally Degenerate Quantum Magnet with Dynamical Jahn-Teller Effect
- Sign structures for short-range RVB states on small kagome clusters
- Antiferromagnetism in kagome -CuMg(OH)Br
- Probing quantum spin liquids in equilibrium using the inverse spin Hall effect
- Spin- kagome Heisenberg antiferromagnet with strong breathing anisotropy
- Frustrated Magnetism in Triangular Lattice TlYbS Crystals Grown via Molten Flux
- Infrared phonons as a probe of a spin-liquid states in herbertsmithite ZnCu3(OH)6Cl2
- Ghost modes and continuum scattering in the dimerized distorted kagome lattice antiferromagnet RbCuSnF
- Emergence of the spin polarized domains in the kagome lattice Heisenberg antiferromagnet Zn-barlowite (ZnCu)Cu(OD)FBr
- Kondo physics in the algebraic spin liquid
- Unification of parton and coupled-wire approaches to quantum magnetism in two dimensions
- Evolution of the commensurate and incommensurate magnetic phases of the S = 3/2 kagome staircase Co3V2O8 in an applied field
- Thermodynamic, magnetic and transport properties of the repulsive Hubbard model on the kagome lattice
- Influence of Dzyaloshinskii-Moriya interactions on magnetic structure of a spin-1/2 deformed kagome lattice antiferromagnet
- Doped Valence Bond Solid and Superconductivity on the Shastry-Sutherland Lattice
- Spin dynamics in Heisenberg triangular antiferromagnets: A muSR study of LiCrO2
- Helical order and multiferroicity in the quasi-kagome system KCuAsO(OD)
- Dynamic Spin Fluctuations in the Frustrated Spin Chain Compound LiCuSbO
- Quantum critical spin-liquid-like behavior in S = 1/2 quasikagome lattice CeRh1-xPdxSn investigated using muon spin relaxation and neutron scattering
- The Herbertsmithite Hamiltonian: SR measurements on single crystals
- Three-dimensional nematic spin liquid in the stacked triangular lattice 6H-B structure
- Optical conductivity of visons in Z2 spin liquids close to a VBS transition on the kagome lattice
- Partial ferromagnetic ordering and indirect exchange interaction in spatially anisotropic kagome antiferromagnet Cs_2Cu_3CeF_{12}
- Unveiling the physics of the doped phase of the Kagome model
- Dynamic magnetism in the disordered hexagonal double perovskite BaTiMnO
- Possible realization of three-dimensional quantum spin liquid behavior in HoVO4
- Static impurities in the S=3/2 kagome lattice
- Electronic Density of States of a Quantum Spin Liquid with Spinon Fermi Surface. II. Zeeman Magnetic Field Effects
- Heat conduction in herbertsmithite: field dependence at the onset of the quantum spin liquid regime
- Chiral Broken Symmetry Descendants of the Kagomé Lattice Chiral Spin Liquid
- Signatures for spinons in the quantum spin liquid candidate CaCrO
- Role of chemical pressure on the electronic and magnetic properties of spin-1/2 kagome mineral averievite
- Heat transport in magnetic fields by quantum spin liquid in the organic insulators EtMe3Sb[Pd(dmit)2]2 and κ-(BEDT-TTF)2Cu2(CN)3
- Evidence for a Parity Broken Monoclinic Ground State in the S = 1/2 Kagomé Antiferromagnet Herbertsmithite
- Magnetic properties and magnetic structure of the frustrated quasi-one-dimensional antiferromagnet SrCuTeO
- Heavy fermion spin liquid in herbertsmithite
- First-principles characterization of the magnetic properties of Cu(OH)Br
- NMR evidence of spinon localization in kagome antiferromagnet YCu(OH)Br[Br(OH)]
- Fermionic spin liquid analysis of the paramagnetic state in Volborthite
- Nuclear relaxation rates in the Herbertsmithite Kagome antiferromagnets ZnCu3(OH)6Cl2
- Dynamical coupling of dilute magnetic impurities with quantum spin liquid state in the S = 3/2 dimer compound Ba3ZnRu2O9
- Synthesis and pressure and field dependent magnetic properties of the Kagome-bilayer spin liquid CaCrO
- The Kagome Antiferromagnet: A Schwinger-Boson Mean-Field Theory Study
- Magnetic field-induced instability of the cooperative paramagnetic state in ZnCo(OD)Cl
- A density-wave-like transition in the polycrystalline V3Sb2 sample with bilayer kagome lattice
- Short-range order and hidden energy scale in geometrically frustrated magnets
- Two-dimensional phase diagram of the charge density wave in doped CsVSb
- First-principles study of an organometallic S=1/2 kagome compound
- Controlling the stoichiometry of the triangular lattice antiferromagnet LiZnMoO
- Fractionalized gapless quantum vortex liquids
- Three-dimensional higher-order saddle points induced flat bands in Co-based kagome metals
- Novel quantum spin liquid ground state in the trimer rhodate BaNbRhO
- Classical phase diagram of the stuffed honeycomb lattice
- Spin liquid fingerprints in the thermal transport of a Kitaev-Heisenberg ladder
- Phase diagram of a bilinear-biquadratic spin-1 model on the triangular lattice from density matrix renormalization group simulations
- Spatially anisotropic kagome antiferromagnet with Dzyaloshinskii-Moriya interaction
- Suppression of the antiferromagnetic order by Zn doping in a possible Kitaev material NaCoTeO
- Electrical and thermal transport properties of kagome metals AVSb (A=K, Rb, Cs)
- Quantum spin liquid and magnetic order in a two-dimensional non-symmorphic lattice: considering the distorted Kagome lattice of Volborthite
- Effect of quenched disorder on a quantum spin liquid state of triangular-lattice antiferromagnet 1T-TaS
- Gapless dynamic magnetic ground state in the charge-gapped trimer iridate BaNbIrO
- Emergence of gravity from interacting simplices
- Low-energy Majorana states in spin-liquid transitions in a three-dimensional Kitaev model
- : Heavy Lanthanides on Spin-1/2 Kagome Magnets
- Formation of collective spins in frustrated clusters
- Ferrimagnetic 120 magnetic structure in Cu2OSO4
- Tuning of magnetic frustration in Kagomé lattices {[Cu(CO)](ClO)} and {[Cu(CO)](ClO)} through rigid and flexible ligands
- The specific heat and magnetic properties of a spin-1/2 ladder including butterfly-shaped unit blocks
- Pristine Mott Insulator from an Exactly Solvable Spin-1/2 Kitaev Model
- Signatures of spin-triplet excitations in optical conductivity of valence bond solids
- Impurity effects in the quantum kagome system ZnCu3(OH)6Cl2
- Rapid filling of the spin gap with temperature in the Schwinger-boson mean-field theory of the antiferromagnetic Heisenberg kagome model
- Tunable moire spinons in magnetically encapsulated twisted van der Waals quantum spin-liquids
- Piercing the Dirac spin liquid: From a single monopole to chiral states
- Neel and Valence Bond Crystal Order on a Distorted Kagome Lattice: Implications For Zn-Paratacamite
- Controlling magnetic frustration in 1T-TaS via Coulomb engineered long-range interactions
- Li doping kagome spin liquid compounds
- Emergent gauge dynamics of highly frustrated magnets
- Variational Monte Carlo study of gapless spin liquid in the spin- XXZ antiferromagnetic model on the kagome lattice
- Breakdown of Linear Spin-wave Theory and Existence of Spinon Bound States in the Frustrated Kagome Lattice Antiferromagnet
- Effects of Dzyaloshinskii-Moriya interactions in volborthite: Magnetic orders and thermal Hall effect
- Study of the bilinear biquadratic Heisenberg model on a honeycomb lattice via Schwinger bosons
- Schwinger boson study of the -- kagome Heisenberg antiferromagnet with Dzyaloshinskii-Moriya interactions
- Magnetic phase diagram and Mott transition of the half-filled 1/5-depleted Hubbard model with frustration
- Family of exactly solvable models with an ultimative quantum paramagnetic ground state
- Exploiting polarization dependence in two dimensional coherent spectroscopy: examples of CeZrO and NdZrO
- Distinct-symmetry spin liquid states and phase diagram of Kitaev-Hubbard model
- Engineering frustrated Rydberg spin models by graphical Floquet modulation
- Thermodynamic Properties of Kagome Antiferromagnets with different Perturbations
- Combinatorial exploration of quantum spin liquid candidates in the herbertsmithite material family
- Chemistry of the spin-1/2 kagome Heisenberg antiferromagnet
- Incommensurate Phase of a Triangular Frustrated Heisenberg Model Studied via Schwinger-Boson Mean-Field Theory
- Widely Spaced Planes of Magnetic Dimers in the Ba6Y2Rh2Ti2O17-δ Hexagonal Perovskite
- Magnetic Frustration in a Mn Honeycomb Lattice Induced by Mn-O-O-Mn Pathways
- Universal scaling behavior of heavy fermion compounds
- Finite size effects in the Z_2 spin liquid on the kagome lattice
- Bulk Crystal Growth and Single-Crystal-to-Single-Crystal Phase Transitions in the Averievite CsClCu5V2O10
- Spin glassiness and power law scaling in a quasi-triangular spin-1/2 compound
- Spin-1/2 Ising-Heisenberg Cairo pentagonal model in the presence of an external magnetic field: Effect of Landé g-factors
- Thermodynamic, dynamic and transport properties of quantum spin liquid in herbertsmithite from experimental and theoretical point of view
- Emergence of a Dimer-Dimer Interaction in the Low-Energy Effective Quantum-Dimer Model of a Diamond-Like-Decorated Square-Lattice Heisenberg Antiferromagnets with Further Neighbor Couplings
- Quantum Thermal Hall effect of chiral spinons on a Kagome strip
- Signatures of a gapless quantum spin liquid in the Kitaev material NaCoZnSbO
- Discovering Strongly Correlated Quantum Spin Liquid
- Using Random Boundary Conditions to simulate disordered quantum spin models in 2D-systems
- Breathing-Driven Metal-Insulator Transition in Correlated Kagome Systems
- Optical conductivity and surface plasmon modes of U(1) spin liquid states with large spinon Fermi surfaces
- Fractional Spin Quantum Hall Effect in Weakly Coupled Spin Chain Arrays
- Phase diagram and thermal Hall conductivity of spin-liquid Kekulé-Kitaev model
- Spinon Majorana fermions
- Finite Temperature Magnetism in the Triangular Lattice Antiferromagnet KErTe2
- Magnetic transition in the Kagomé system SmSbZnO
- Crystal chemistry criteria of the existence of spin liquids on the kagome lattice
- Survival of magnetic correlations above ordering temperature in a ferromagnetically ordered classical kagomé magnet: Li9Cr3(P2O7)3(PO4)2
- Nature of the 1/3 Magnetization Plateau in Spin-1/2 Kagome Antiferromagnets
- Effects of exchange distortions in the magnetic Kagome lattice
- Electric Field Response In Breathing Pyrochlores
- Double-layer Kagome Metals Pt3Tl2 and Pt3In2
- Thermal Hall response of an abelian chiral spin liquid at finite temperatures
- Thermal features of Heisenberg antiferromagnets on edge- versus corner-sharing triangular-based lattices: A message from spin waves
- A Promising Method for Strongly Correlated Electrons in Two Dimensions: Gutzwiller-Guided Density Matrix Renormalization Group
- Universal behavior of quantum spin liquid and optical conductivity in the insulator herbertsmithite
- Magnetically disordered ground state in the triangular-lattice antiferromagnets RbYb(VO) and CsYb(VO)
- Momentum selective optical absorption in triptycene molecular membrane
- Magnetic excitations in the 1/3 plateau state in InCu(OH)Cl
- Nonlinear optical conductivity of spin liquids with large spinon Fermi surfaces
- Recent progress in quantum spin liquids, fractional magnetization plateaus, and unconventional superconductivity in kagome lattices
- Strong relevance of Zinc impurity in the spin- Kagome quantum antiferromagnets: a variational study
- Impact of Oxidation State on the Valence-bond-glass Physics in the lithium-intercalated MoO Cluster Mott Insulators
- Strong coupling of lattice and orbital excitations in quantum magnet CaCrO: Anomalous temperature dependence of Raman phonons
- Power-law dynamics in the spin-liquid kagome lattices SrCr8Ga4O19 and ZnCu3(OH)6Cl2
- Continuous interpolation between the fully frustrated Ising and quantum dimer models
- Quantifying the Phase Diagram and Hamiltonian of Kagome Antiferromagnets: Bridging Theory and Experiment
- Witnessing Disorder in Quantum Magnets
- Entanglement studies of resonating valence bonds on the frustrated square lattice
- Disorder-induced spin excitation continuum and spin-glass ground state in the inverse spinel CuGaO
- Spinon mediation of witness spin dynamics in herbertsmithite
- Emergent Spin-Singlet Pairing in the Frustrated Kagome Metal ScMnAlSi
- Dynamical spin correlations in kagome antiferromagnets: comparison of Abrikosov fermion and Schwinger boson approaches beyond mean field
- Evidence for a string-net matter
- New S=1/2 Kagome Antiferromagnets ACuSnF: A=Cs and Rb
- Quantum to classical transition in the ground state of a spin- quantum antiferromagnet
- Magnetism of kagome metals studied by SR
- Effect of Dirac Spinons on ARPES signatures of Herbertsmithe
- Slow spin dynamics in the hyper-honeycomb Lattice [(C2H5)3NH]2Cu2(C2O4)3 revealed by 1H NMR studies
- Effects of the Crystalline Electric Field in the Quantum Spin Liquid Candidate
- Quantum spin liquids by geometric lattice design
- Magnetodielectric Properties in Two Dimensional Magnetic Insulators
- Electron correlation effects and spin-liquid state in the Herbertsmithite Kagome lattice
- Signatures of a Majorana-Fermi surface in the Kitaev magnet AgLiIrO
- Phase-space networks and connectivity of the kagome antiferromagnet
- Emergence of topological defects and spin liquid in a two-orbital spin-fermion model on the honeycomb lattice
- Spin Liquid Mimicry in the Hydroxide Double Perovskite CuSn(OH) Induced by Correlated Proton Disorder
- Spin liquid and ferroelectricity close to a quantum critical point in PbCuTeO
- Spin disorder state induced by Mg doping in a Kitaev material NaCoSbO
- Strongly frustrated 2D magnetism in a 3D hexagonal perovskite
- Finite Spinon Density-of-States in Triangular-Lattice Delafossite TlYbSe