Origin of nonlocal resistance in multiterminal graphene on hexagonal-boron-nitride: Fermi surface edge currents rather than Fermi sea topological valley currents

Abstract

The recent observation [R. V. Gorbachev et al., Science {\bf 346}, 448 (2014)] of nonlocal resistance $R_{\mathrm{NL}}$ near the Dirac point (DP) of multiterminal graphene on aligned hexagonal boron nitride (G/hBN) has been interpreted as the consequence of topological valley Hall currents carried by the Fermi sea states just beneath the bulk gap $E_g$ induced by the inversion symmetry breaking. However, the valley Hall conductivity ${\sigma }_{xy}^v$, quantized inside $E_g$, is not directly measurable. Conversely, the Landauer-Büttiker formula, as numerically exact approach to observable nonlocal transport quantities, yields $R_{\mathrm{NL}}\equiv 0$ for the same simplistic Hamiltonian of gapped graphene that generates ${\sigma }_{xy}^v\ne 0$. We combine ab initio with quantum transport calculations to demonstrate that G/hBN wires with zigzag edges host dispersive edge states near the DP that are absent in theories based on the simplistic Hamiltonian. Although such edge states exist also in isolated zigzag graphene wires, aligned hBN is required to modify their energy-momentum dispersion and generate $R_{\mathrm{NL}}\ne 0$ near the DP persisting in the presence of edge disorder. Concurrently, the edge states resolve the long-standing puzzle of why the highly insulating state of G/hBN is rarely observed. We conclude that the observed $R_{\mathrm{NL}}$ is unrelated to Fermi sea topological valley currents conjectured for gapped Dirac spectra.

6 pages, 4 figures, PDF LaTeX; Supplemental Material with 7 additional figures is available from https://wiki.physics.udel.edu/qttg/Publications

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