Brightening of dark excitons in monolayers of semiconducting transition metal dichalcogenides
arXiv:1612.02867 · doi:10.1088/2053-1583/aa5521
Abstract
We present low temperature magneto-photoluminescence experiments which demonstrate the brightening of dark excitons by an in-plane magnetic field applied to monolayers of different semiconducting transition metal dichalcogenides. For both WSe and WS monolayers, the dark exciton emission is observed at 50 meV below the bright exciton peak and displays a characteristic doublet structure which intensity is growing with , while no magnetic field induced emission peaks appear for MoSe monolayer. Our experiments also show that the MoS monolayer has a dark exciton ground state with a dark-bright exciton splitting energy of 100 meV.
arXiv comment7 pages, 3 figures
References in corpus (39)
- Atomically thin MoS2: A new direct-gap semiconductor
- Coupled spin and valley physics in monolayers of MoS2 and other group-VI dichalcogenides
- Control of valley polarization in monolayer MoS2 by optical helicity
- Valley polarization in MoS2 monolayers by optical pumping
- MoS_2 as an ideal material for valleytronics: valley-selective circular dichroism and valley Hall effect
- Exciton Binding Energy and Nonhydrogenic Rydberg Series in Monolayer WS2
- Evolution of Electronic Structure in Atomically Thin Sheets of WS2 and WSe2
- Observation of giant bandgap renormalization and excitonic effects in a monolayer transition metal dichalcogenide semiconductor
- Electrical Control of Two-Dimensional Neutral and Charged Excitons in a Monolayer Semiconductor
- Optoelectronics with electrically tunable PN diodes in a monolayer dichalcogenide
- Optical Generation of Excitonic Valley Coherence in Monolayer WSe2
- Direct observation of the transition from indirect to direct bandgap in atomically thin epitaxial MoSe2
- Optical signature of symmetry variations and spin-valley coupling in atomically thin tungsten dichalcogenides
- k.p theory for two-dimensional transition metal dichalcogenide semiconductors
- Probing Excitonic Dark States in Single-layer Tungsten Disulfide
- Three-band tight-binding model for monolayers of group-VIB transition metal dichalcogenides
- Exciton Binding Energy of Monolayer WS2
- Valley Splitting and Polarization by the Zeeman Effect in Monolayer MoSe2
- Electronic properties of the MoS2-WS2 heterojunction
- Photocarrier relaxation in two-dimensional semiconductors
- Indirect-to-direct band-gap crossover in few-layer MoTe
- Large spin splitting in the conduction band of transition metal dichalcogenide monolayers
- Probing excitonic states in ultraclean suspended two-dimensional semiconductors by photocurrent spectroscopy
- Direct observation of spin-polarised bulk bands in an inversion-symmetric semiconductor
- Identification of excitons, trions and biexcitons in single-layer WS2
- Measurement of high exciton binding energy in the monolayer transition-metal dichalcogenides WS2 and WSe2
- Exciton fine structure and spin decoherence in monolayers of transition metal dichalcogenides
- Splitting between Bright and Dark excitons in Transition Metal Dichalcogenide Monolayers
- Nonanalyticity, Valley Quantum Phases, and Light-like Exciton Dispersion in Monolayer TMDs: Theory and First-Principles Calculations
- Spin-orbit engineering in transition metal dichalcogenide alloy monolayers
- Exciton band structure in layered MoSe2: from a monolayer to the bulk limit
- Control of Exciton Valley Coherence in Transition Metal Dichalcogenide Monolayers
- Polarization analysis of excitons in monolayer and bilayer transition-metal dichalcogenides
- Optical investigation of monolayer and bulk tungsten diselenide (WSe) in high magnetic fields
- Broad Band Optical Properties of Large Area Monolayer CVD Molybdenum Disulfide
- Spin-flip processes and radiative decay of dark intravalley excitons in transition metal dichalcogenide monolayers
- Tuning valley polarization in a WSe2 monolayer with a tiny magnetic field
- Ultra-low power threshold for laser induced changes in optical properties of 2D Molybdenum dichalcogenides
- Well separated trion and neutral excitons on superacid treated MoS2 monolayers
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- Excitonic linewidth approaching the homogeneous limit in MoS2 based van der Waals heterostructures : accessing spin-valley dynamics
- In-plane Propagation of Light in Transition Metal Dichalcogenide Monolayers: Optical Selection Rules
- Probing dark excitons in atomically thin semiconductors via near-field coupling to surface plasmon polaritons
- Two-dimensional semiconductors in the regime of strong light-matter coupling
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- Valley-selective chiral phonon replicas of dark excitons and trions in monolayer WSe2
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- Imaging Spin Dynamics in Monolayer WS2 by Time-Resolved Kerr Rotation Microscopy
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- Dark trions and biexcitons in WS2 and WSe2 made bright by e-e scattering
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- Magnetooptics of layered two-dimensional semiconductors and heterostructures: progress and prospects
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- Rydberg series of dark excitons and the conduction band spin-orbit splitting in monolayer WSe
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- Incoherent phonon population and exciton-exciton annihilation in monolayer WS2 revealed by time-resolved spontaneous Raman scattering
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- Optical fingerprint of bright and dark localized excitonic states in atomically thin 2D materials
- Dark-state impact on the exciton recombination of WS2 monolayers as revealed by multi-time-scale pump-and-probe spectroscopy
- Excitons and trions in WSSe monolayers
- Theory of the Coherent Response of Magneto-Excitons and Magneto-Biexcitons in Monolayer Transition Metal Dichalcogenides
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- Many-Body Effect of Mesoscopic Localized States in MoS Monolayer
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- Intrinsic edge excitons in two-dimensional MoS
- Quadrupolar and dipolar excitons in symmetric trilayer heterostructures: Insights from first principles theory
- Magnetic field mixing and splitting of bright and dark excitons in monolayer MoSe2
- Raman scattering excitation in monolayers of semiconducting transition metal dichalcogenides
- Large photoluminescence enhancement by an out-of-plane magnetic field in exfoliated WS flakes
- Photoluminescence kinetics of dark and bright excitons in atomically thin MoS
- Brightening odd-parity excitons in transition-metal dichalcogenides: Rashba spin-orbit interaction, skyrmions, and cavity polaritons
- Engineering Purcell factor anisotropy for dark and bright excitons in two dimensional semiconductors
- Magneto-Optical Measurements of the Negatively Charged 2 Exciton in WSe
- Exchange-split multiple Rydberg series of excitons in anisotropic quasi two-dimensional ReS
- Multidimensional sensing of proximity magnetic fields via intrinsic activation of dark excitons in WSe/CrCl heterostructure
- Extremely high excitonic -factors in 2D crystals by alloy-induced admixing of band states
- Trapping the carrier in the spin-locked MoS2 atomic valley by absorption of chiral L-cysteine
- Observation of anisotropic dispersive dark exciton dynamics in CrSBr
- Optical response of WSe-based vertical tunneling junction
- Magnetic proximity effect on excitonic spin states in Mn-doped layered hybrid perovskites
- Dark-Exciton-Mediated Fano Resonance from a Single Gold Nanostructure Deposited on Monolayer WS2 at Room Temperature
- Rydberg series of intralayer K-excitons in WSe multilayers
- Unconventional bright ground-state excitons in monolayer TiI from first-principles calculations
- Magnetic Field-Tunable Repulsive Exciton-Exciton Interaction in the van der Waals Antiferromagnet NiPS
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