Magnetization dependent tunneling conductance of ferromagnetic barriers
arXiv:2106.13930 · doi:10.1038/s41467-021-26973-7
Abstract
Recent experiments on van der Waals antiferrmagnets such as CrI3, CrCl3 and MnPS3 have shown that using atomically thin layers as tunnel barriers and measuring the temperature () and magnetic field () dependence of the conductance allows their magnetic phase diagram to be mapped. In contrast, barriers made of CrBr3 -- the sole van der Waals ferromagnet investigated in this way -- were found to exhibit small and featureless magnetoconductance, seemingly carrying little information about magnetism. Here we show that -- despite these early results -- the conductance of CrBr3 tunnel barriers does provide detailed information about the magnetic state of atomically thin CrBr3 crystals for both above and below the Curie temperature ( K). Our analysis establishes that the tunneling conductance depends on and exclusively through the magnetization , over the entire temperature range investigated (2-50 K). The phenomenon is reproduced in detail by the spin-dependent Fowler-Nordheim model for tunneling, and is a direct manifestation of the spin splitting of the CrBr3 conduction band. These findings demonstrate that the investigation of magnetism by tunneling conductance measurements is not limited to antiferromagnets, but can also be applied to ferromagnetic materials.
References in corpus (19)
- Spintronics: Fundamentals and applications
- Magnetic 2D materials and heterostructures
- Giant Tunneling Magnetoresistance in Spin-Filter van der Waals Heterostructures
- Probing magnetism in 2D van der Waals crystalline insulators via electron tunneling
- Direct observation of van der Waals stacking dependent interlayer magnetism
- Colloquium: Spintronics in graphene and other two-dimensional materials
- Direct photoluminescence probing of ferromagnetism in monolayer two-dimensional CrBr3
- Atomically Thin CrCl3: An in-Plane Layered Antiferromagnetic Insulator
- Evolution of interlayer and intralayer magnetism in three atomically thin chromium trihalides
- Magnon-assisted tunnelling in van der Waals heterostructures based on CrBr3
- One million percent tunnel magnetoresistance in a magnetic van der Waals heterostructure
- Giant enhancement of interlayer exchange in an ultrathin 2D magnet
- Spin-flop transition in atomically thin MnPS crystals
- Determining the phase diagram of atomically thin layered antiferromagnet CrCl
- Magnetic Two-Dimensional Chromium Trihalides: A Theoretical Perspective
- Micromagnetometry of two-dimensional ferromagnets
- Magnetic domains and domain wall pinning in two-dimensional ferromagnets revealed by nanoscale imaging
- Tailored tunnel magnetoresistance response in three ultrathin chromium trihalides
- Imaging and control of critical spin fluctuations in two-dimensional magnets