Molecules cooled below the Doppler limit
arXiv:1703.00580 · doi:10.1038/nphys4241
Abstract
The ability to cool atoms below the Doppler limit -- the minimum temperature reachable by Doppler cooling -- has been essential to most experiments with quantum degenerate gases, optical lattices and atomic fountains, among many other applications. A broad set of new applications await ultracold molecules, and the extension of laser cooling to molecules has begun. A molecular magneto-optical trap has been demonstrated, where molecules approached the Doppler limit. However, the sub-Doppler temperatures required for most applications have not yet been reached. Here we cool molecules to 50 uK, well below the Doppler limit, using a three-dimensional optical molasses. These ultracold molecules could be loaded into optical tweezers to trap arbitrary arrays for quantum simulation, launched into a molecular fountain for testing fundamental physics, and used to study ultracold collisions and ultracold chemistry.
arXiv comment8 pages, 6 figures
References in corpus (26)
- Cold and Ultracold Molecules: Science, Technology, and Applications
- A toolbox for lattice spin models with polar molecules
- Order of Magnitude Smaller Limit on the Electric Dipole Moment of the Electron
- An atom-by-atom assembler of defect-free arbitrary 2d atomic arrays
- Laser cooling of a diatomic molecule
- Magneto-optical trapping of a diatomic molecule
- Magneto-optical trapping of diatomic molecules
- Laser cooling and slowing of CaF molecules
- Sisyphus Laser Cooling of a Polyatomic Molecule
- Magneto-Optical Trap for Polar Molecules
- Sub-millikelvin dipolar molecules in a radio-frequency magneto-optical trap
- Optoelectrical cooling of polar molecules to sub-millikelvin temperatures
- Design for a fountain of YbF molecules to measure the electron's electric dipole moment
- Sub-Doppler laser cooling of fermionic 40K atoms in three-dimensional gray optical molasses
- Laser slowing of CaF molecules to near the capture velocity of a molecular MOT
- An intense, cold, velocity-controlled molecular beam by frequency-chirped laser slowing
- Characteristics of a magneto-optical trap of molecules
- On the Prospects for Laser Cooling of TlF
- Three-dimensional Doppler, polarization-gradient, and magneto-optical forces for atoms and molecules with dark states
- Improved magneto-optical trapping of a diatomic molecule
- Modeling magneto-optical trapping of CaF molecules
- Lifetime of the A(v'=0) state and Franck-Condon factor of the A-X(0-0) transition of CaF measured by the saturation of laser-induced fluorescence
- Modeling sympathetic cooling of molecules by ultracold atoms
- A molecular fountain
- Zeeman-tuned rotational level-crossing spectroscopy in a diatomic free radical
- Principles and design of a Zeeman-Sisyphus decelerator for molecular beams
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- Cold molecules: Progress in Quantum Engineering of Chemistry and Quantum Matter
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- Quantum control of molecular rotation
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- A Fermi Degenerate Gas of Polar Molecules
- Precision Measurement of Time-Reversal Symmetry Violation with Laser-Cooled Polyatomic Molecules
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- Dipolar Exchange Quantum Logic Gate with Polar Molecules
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- Microwave shielding of ultracold polar molecules
- -Enhanced Imaging of Molecules in an Optical Trap
- Spectroscopy of short-lived radioactive molecules: A sensitive laboratory for new physics
- Magnetically-Trapped Molecules Efficiently Loaded from a Molecular MOT
- Resonant collisional shielding of reactive molecules using electric fields
- Polyatomic Molecules as Quantum Sensors for Fundamental Physics
- Sticky collisions of ultracold RbCs molecules
- Magnetic trapping and coherent control of laser-cooled molecules
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- Controlling the scattering length of ultracold dipolar molecules
- Observation of Collisions between Two Ultracold Ground-State CaF Molecules
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