Electronic transport, metal-insulator transition, and Wigner crystallization in transition metal dichalcogenide monolayers

Abstract

Two recent electronic transport experiments from Columbia University and Harvard University have reported record high mobility and low channel densities in transition metal dichalcogenide (TMD) WSe${}_2$ monolayers [J. Pack, et al., arXiv:2310.19782; A. Y. Joe, et al., Phys. Rev. Lett. 132, 056303 (2024)]. A two-dimensional (2D) metal-insulator transition (MIT) is demonstrated in the Columbia sample at low densities, a regime where the formation of a Wigner crystal (WC) is theoretically anticipated in the absence of disorder. We employ the finite-temperature Boltzmann theory to understand the low-temperature transport properties of monolayer TMDs, taking into account realistic disorder scattering. We analyze the experimental results, focusing on the 2D MIT behavior and the influence of temperature and density on mobility and resistivity in the metallic phase. We provide a discussion of the nontrivial carrier density dependence of our transport results. Our analysis elucidates the linear-in-$T$ resistivity in the metallic phase, attributing it to Friedel oscillations associated with screened charged impurities. Furthermore, we explore whether Coulomb disorder could lead to the MIT through either a quantum Anderson localization transition or a classical percolation transition. Our theoretical estimates of the disorder-induced MIT critical densities, although smaller, are within a factor of ~2 of the experimental critical density. We examine the exceptionally high melting temperature ~10 K of WCs observed experimentally in the MoSe${}_2$ systems at low density, an order of magnitude larger than the pristine melting temperature. This suggests that the observed 2D low-density MIT behavior is likely a result of the complex interplay between disorder effects and interaction-driven WC physics, offering a comprehensive understanding of the low-temperature transport phenomena in TMD monolayers.

arXiv comment25 pages, 9 figures

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