Ultracold Gas of Dipolar NaCs Ground State Molecules
arXiv:2206.00652 · doi:10.1103/PhysRevLett.130.113002
Abstract
We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a peak density of cm. We demonstrate comprehensive quantum state control by preparing the molecules in a specific electronic, vibrational, rotational, and hyperfine state. Employing the tunability and strength of the permanent electric dipole moment of NaCs, we induce dipole moments of up to 2.6 D. Dipolar systems of NaCs molecules are uniquely suited to explore strongly interacting phases in dipolar quantum matter.
arXiv comment6 pages, 5 figures
References in corpus (52)
- Feshbach Resonances in Ultracold Gases
- A High Phase-Space-Density Gas of Polar Molecules
- The physics of dipolar bosonic quantum gases
- Quantum computation with trapped polar molecules
- Cold and Ultracold Molecules: Science, Technology, and Applications
- A toolbox for lattice spin models with polar molecules
- Realizing a lattice spin model with polar molecules
- Stimulated Raman adiabatic passage in physics, chemistry and beyond
- Condensed Matter Theory of Dipolar Quantum Gases
- Quantum Simulators: Architectures and Opportunities
- Ultracold dense samples of dipolar RbCs molecules in the rovibrational and hyperfine ground state
- Strongly correlated 2D quantum phases with cold polar molecules: controlling the shape of the interaction potential
- Ultracold Dipolar Gas of Fermionic NaK Molecules in their Absolute Ground State
- Creation of ultracold RbCs molecules in the rovibrational ground state
- Controlling the quantum stereodynamics of ultracold bimolecular reactions
- Creation of an ultracold gas of ground-state molecules
- Calculation of accurate permanent dipole moments of the lowest states of heteronuclear alkali dimers using extended basis sets
- Quantum gas of rovibronic ground-state molecules in an optical lattice
- Quantum Phases of Cold Polar Molecules in 2D Optical Lattices
- A Fermi Degenerate Gas of Polar Molecules
- Reactions of ultracold alkali metal dimers
- New frontiers with quantum gases of polar molecules
- Long-Lived Ultracold Molecules with Electric and Magnetic Dipole Moments
- Direct observation of bimolecular reactions of ultracold KRb molecules
- Evaporation of microwave-shielded polar molecules to quantum degeneracy
- Ultracold polar molecules as qudits
- Statistical Aspects of Ultracold Resonant Scattering
- Microwave shielding of ultracold polar molecules
- Assembly of a rovibrational ground state molecule in an optical tweezer
- Resonant collisional shielding of reactive molecules using electric fields
- Dipolar evaporation of reactive molecules to below the Fermi temperature
- Controlling the scattering length of ultracold dipolar molecules
- Loss of ultracold RbCs molecules via optical excitation of long-lived two-body collision complexes
- Tuning of dipolar interactions and evaporative cooling in a three-dimensional molecular quantum gas
- Modeling the adiabatic creation of ultracold, polar molecules
- Universal ultracold collision rates for polar molecules of two alkali-metal atoms
- Transition from a polaronic condensate to a degenerate Fermi gas of heteronuclear molecules
- Collisions of ultracold molecules in bright and dark optical dipole traps
- Coherent Microwave Control of Ultracold NaK Molecules
- Forming a single molecule by magnetoassociation in an optical tweezer
- Probing photoinduced two-body loss of ultracold non-reactive bosonic NaRb and NaK molecules
- Ultracold Sticky Collisions: Theoretical and Experimental Status
- Adiabatic population transfer via multiple intermediate states
- Adimensional theory of shielding in ultracold collisions of dipolar rotors
- Dipolar Collisions of Ultracold Ground-state Bosonic Molecules
- Resonant dipolar collisions of ultracold molecules induced by microwave dressing
- Hyperfine structure of alkali-metal diatomic molecules
- Accurate Determination of the Dynamical Polarizability of Dysprosium
- Observation of interference between resonant and detuned STIRAP in the adiabatic creation of NaK molecules
- Overlapping Bose-Einstein Condensates of Na and Cs
- A High Phase-Space Density Gas of NaCs Feshbach Molecules
- Efficient conversion of closed-channel dominated Feshbach molecules of NaK to their absolute ground state
Cited by in corpus (34)
- Observation of Bose-Einstein Condensation of Dipolar Molecules
- Quantum state manipulation and cooling of ultracold molecules
- Collisionally Stable Gas of Bosonic Dipolar Ground State Molecules
- Ultracold Sticky Collisions: Theoretical and Experimental Status
- Microwave shielding of bosonic NaRb molecules
- Effective potential and superfluidity of microwave-dressed polar molecules
- Diatomic molecules of alkali-metal and alkaline-earth-metal atoms: interaction potentials, dipole moments, and polarizabilities
- Double Microwave Shielding
- Electro-association of ultracold dipolar molecules into tetramer field-linked states
- Observation of photoassociation resonances in ultracold atom-molecule collisions
- Three-Body Recombination of Ultracold Microwave-Shielded Polar Molecules
- Efficient Pathway to NaCs Ground State Molecules
- Enhanced quantum state transfer via feedforward cancellation of optical phase noise
- Long distance optical conveyor-belt transport of ultracold Cs and Rb atoms
- Realizing multiband states with ultracold dipolar quantum simulators
- A planar cloverleaf antenna for the creation of circularly polarized microwave fields
- The iSWAP gate with polar molecules: Robustness criteria for entangling operations
- Highly Efficient Creation and Detection of Ultracold Deeply-Bound Molecules via Chainwise Stimulated Raman Shortcut-to-Adiabatic Passage
- Spin Squeezing with Itinerant Dipoles: A Case for Shallow Lattices
- Probing rotational decoherence with a trapped-ion planar rotor
- Dressed-State Spectroscopy and Magic Trapping of Microwave-Shielded NaCs Molecules
- Fast and robust production of quantum superposition states by the fractional shortcut to adiabaticity
- Dissipative Superfluidity in a Molecular Bose-Einstein Condensate
- Macroscopic Particle Transport in Dissipative Long-Range Bosonic Systems
- Quantum Interference in Atomic Systems
- Genetics-based deperturbation analysis for the spin-orbit coupled and states of LiRb
- Highly Efficient Creation and Detection of Deeply-bound Molecules via Invariant-based Inverse Engineering with Feasible Modified Drivings
- Broad Feshbach resonance with a large background scattering length in a fermionic atom-molecule mixture
- Beyond-mean-field phases of rotating dipolar condensates
- CaF+CaF interactions in the ground and excited electronic states: implications for collisional losses
- A versatile apparatus for simultaneous trapping of multiple species of ultracold atoms and ions to enable studies of low energy collisions and cold chemistry
- Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics
- Electric-Field Control of Josephson Oscillations in Dipolar Bose-Einstein Condensates
- Automated Graph-Based Detection of Quantum Control Schemes: Application to Molecular Laser Cooling