Emergent Spin Supersolids in Frustrated Quantum Materials
arXiv:2601.01890 · doi:10.1002/adma.202600005
Abstract
Recent years have witnessed the emergence of spin supersolids in frustrated quantum magnets, establishing a material-based platform for supersolidity beyond its original context in solid helium. A spin supersolid is characterized by the coexistence of longitudinal spin order that breaks lattice translational symmetry and transverse spin order associated with the spontaneous breaking of the spin U(1) symmetry. Extensive experimental investigations, together with advanced numerical studies, have now revealed a coherent and internally consistent picture of these phases, substantially deepening our understanding of supersolidity in quantum magnetic materials. Beyond their fundamental interest as exotic quantum states, potential applications in highly efficient demagnetization cooling have been supported by a giant magnetocaloric effect observed in candidate materials. Moreover, the possible dissipationless spin supercurrents could open promising perspectives for spin transport and spintronic applications. This review summarizes recent progress on emergent spin supersolids in frustrated triangular-lattice quantum antiferromagnets, surveys experimental evidence from thermodynamic and spectroscopic measurements, and compares these results with theoretical studies of minimal models addressing global phase diagrams, ground state properties, and collective excitations. In addition, this review discusses characteristic spin-transport phenomena and outlines future directions for exploring spin supersolids as functional quantum materials.
17 pages + 6 figures, review article
References in corpus (111)
- Spintronics: Fundamentals and applications
- Many-Body Physics with Ultracold Gases
- Quantum Spin Hall Effect and Topological Phase Transition in HgTe Quantum Wells
- Topological Order and the Quantum Spin Hall Effect
- The density-matrix renormalization group in the age of matrix product states
- Direct electronic measurement of the spin Hall effect
- Experimental observation of the spin-Hall effect in a two dimensional spin-orbit coupled semiconductor system
- Spin Seebeck insulator
- Room Temperature Reversible Spin Hall Effect
- The ITensor Software Library for Tensor Network Calculations
- Theory of the Spin Seebeck Effect
- Observation of a dipolar quantum gas with metastable supersolid properties
- Quantum phases from competing short- and long-range interactions in an optical lattice
- Transient supersolid properties in an array of dipolar quantum droplets
- Supersolids: what and where are they ?
- Long-lived and transient supersolid behaviors in dipolar quantum gases
- Supersolid hardcore bosons on the triangular lattice
- Supersolid Order from Disorder: Hard-Core Bosons on the Triangular Lattice
- Supersolid symmetry breaking from compressional oscillations in a dipolar quantum gas
- Enhanced magnetocaloric effect in frustrated magnets
- Unusual ordered phases of highly frustrated magnets: a review
- The low-energy Goldstone mode in a trapped dipolar supersolid
- Excitation spectrum of a trapped dipolar supersolid and its experimental evidence
- Persistent supersolid phase of hard-core bosons on the triangular lattice
- Spin currents and spin superfluidity
- Two-dimensional supersolidity in a dipolar quantum gas
- Quantum Phase Diagram of the Triangular-Lattice XXZ Model in a Magnetic Field
- Supersolid phase of hardcore bosons on triangular lattice
- Superfluid spin transport through antiferromagnetic insulators
- Giant Magnetocaloric Effect in Spin Supersolid Candidate NaBaCo(PO)
- Superfluid Spin Transport through Easy-Plane Ferromagnetic Insulators
- Supercurrent in a room temperature Bose-Einstein magnon condensate
- Experimental Signatures of Spin Superfluid Ground State in Canted Antiferromagnet Cr2O3 via Nonlocal Spin Transport
- On the Supersolid State of Matter
- The nature of spin excitations in the one-third magnetization plateau phase of BaCoSbO
- Evidence of superfluidity in a dipolar supersolid from non-classical rotational inertia
- Possible itinerant excitations and quantum spin state transitions in the effective spin-1/2 triangular-lattice antiferromagnet NaBaCo(PO)
- Dynamical structure factor of the Heisenberg model on the triangular lattice: magnons, spinons, and gauge fields
- Strong quantum fluctuations in a quantum spin liquid candidate with a Co-based triangular lattice
- Rotating a supersolid dipolar gas
- Exponential Thermal Tensor Network Approach for Quantum Lattice Models
- The phase diagram of the antiferromagnetic XXZ model on the triangular lattice
- Microscopic Model Calculations for the Magnetization Process of Layered Triangular-Lattice Quantum Antiferromagnets
- Field Induced Supersolid Phase in Spin-One Heisenberg Models
- Phase diagram of the Shastry-Sutherland Compound SrCu2(BO3)2 under extreme combined conditions of field and pressure
- Pseudo-Goldstone gaps and order-by-quantum-disorder in frustrated magnets
- Supersolid phase induced by correlated hopping in spin-1/2 frustrated quantum magnets
- Extended supersolid phase of frustrated hard-core bosons on a triangular lattice
- Magnetic phases of a highly frustrated magnet, ZnCr2O4, up to an ultra-high magnetic field of 600 T
- Long-distance supercurrent transport in a room-temperature Bose-Einstein magnon condensate
- Spin Supersolidity in Nearly Ideal Easy-axis Triangular Quantum Antiferromagnet NaBaCo(PO)
- Ground States of Spin-1/2 Triangular Antiferromagnets in a Magnetic Field
- Quantum and thermal transitions out of the supersolid phase of a 2D quantum antiferromagnet
- Supersolidity in ultra-cold dipolar gases
- Supersolid phase in spin dimer XXZ systems under magnetic field
- Tangent Space Approach for Thermal Tensor Network Simulations of the 2D Hubbard Model
- Supersolid phase transitions for hardcore bosons on a triangular lattice
- Supersolid Order of Frustrated Hard-Core Bosons in a Triangular Lattice System
- Spin Supersolid in Anisotropic Spin-One Heisenberg Chain
- Spin Excitation Spectra of Anisotropic Spin- Triangular Lattice Heisenberg Antiferromagnets
- Supersolidity in the triangular lattice spin-1/2 XXZ model: A variational perspective
- Can angular oscillations probe superfluidity in dipolar supersolids?
- Novel Magnetic Phases Revealed by Ultra-High Magnetic Field in the Frustrated Magnet ZnCr2O4
- Series-Expansion Thermal Tensor Network Approach for Quantum Lattice Models
- Variational wavefunction study of the triangular lattice supersolid
- Superfluid-Insulator Transitions on the Triangular Lattice
- Dynamical Signatures of Symmetry Broken and Liquid Phases in an Heisenberg Antiferromagnet on the Triangular Lattice
- Unveiling new quantum phases in the Shastry-Sutherland compound SrCu2(BO3)2up to the saturation magnetic field
- NMR evidence for the persistence of spin-superlattice above the 1/8 magnetization plateau in SrCu2(BO3)2
- Frustration enhanced by Kitaev exchange in a triangular antiferromagnet
- Continuum excitations in a spin-supersolid on a triangular lattice
- A striped supersolid phase and the search for deconfined quantum criticality in hard-core bosons on the triangular lattice
- Plaquette Singlet Transition, Magnetic Barocaloric Effect, and Spin Supersolidity in the Shastry-Sutherland Model
- Sound, superfluidity and layer compressibility in a ring dipolar supersolid
- Magnon Pairs and Spin-Nematic Correlation in the Spin-Seebeck Effect
- Superfluid spin transport in ferro- and antiferromagnets
- Spin-1 Heisenberg antiferromagnetic chain with exchange and single-ion anisotropies
- Quantum spin state transitions in spin-1 equilateral triangular lattice antiferromagnet NaBaNi(PO)
- A case study of spin- Heisenberg model in a triangular lattice
- Kinetic frustration induced supersolid in the kagome lattice antiferromagnet in a magnetic field
- Supersolidity and phase diagram of softcore bosons in a triangular lattice
- Double Magnon-Roton Excitations in the Triangular-Lattice Spin Supersolid
- Bose-Einstein condensation of a two-magnon bound state in a spin-one triangular lattice
- Phase Diagram of the Easy-Axis Triangular-Lattice Model
- Continuum of spin excitations in an ordered magnet
- Pair Superfluid and Supersolid of Correlated Hard-Core Bosons on a Triangular Lattice
- Quantum Spin Supersolid as a precursory Dirac Spin Liquid in a Triangular Lattice Antiferromagnet
- Supersolid phase and magnetization plateaus observed in anisotropic spin-3/2 Heisenberg model on bipartite lattices
- Phase diagrams and excitations of anisotropic quantum magnets on the triangular lattice
- Comparative Raman Scattering Study of Crystal Field Excitations in Co-based Quantum Magnets
- Spin Josephson effects in Exchange coupled Anti-ferromagnets
- Spin-supersolid phase in Heisenberg chains: a characterization via Matrix Product States with periodic boundary conditions
- Simulating Spin Dynamics of Supersolid States in a Quantum Ising Magnet
- Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet
- Magnetization plateau and supersolid phases in the spin-1/2 antiferromagnetic Heisenberg model on a tetragonally distorted fcc lattice
- Quantum Heisenberg antiferromagnetic chains with exchange and single--ion anisotropies
- Zeeman split Kramers doublets in spin-supersolid candidate NaBaCo(PO)
- NMR study of supersolid phases in the triangular-lattice antiferromagnet Na2BaCo(PO4)2
- Easy-axis Heisenberg model on the triangular lattice: from supersolid to gapped solid
- From continuum excitations to sharp magnons via transverse magnetic field in the spin-1/2 Ising-like triangular lattice antiferromagnet Na2BaCo(PO4)2
- Possible Observation of Quadrupole Waves in Spin Nematics
- Spin Seebeck Effect of Triangular-lattice Spin Supersolid
- Signatures of rigidity and second sound in dipolar supersolids
- Direct Evidence of a Near-Ideal Jeff = 1/2 Ground State in Triangular-Lattice Na2BaCo(PO4)2
- Modified large- approach to gapless spin liquids, magnetic orders, and dynamics: Application to triangular lattice antiferromagnets
- Spin structures and phase diagrams of the spin- triangular-lattice antiferromagnet NaBaMn(PO) under magnetic field
- Field tunable BKT and quantum phase transitions in spin-1/2 triangular lattice antiferromagnet
- Slow convergence of spin-wave expansion and magnon dispersion in the 1/3 plateau of the triangular XXZ antiferromagnet
- NMR evidence of spin supersolid and Pomeranchuk effect behaviors in the triangular-lattice antiferromagnet RbNi(SeO)
- Giant anomalous Hall conductivity in frustrated magnet EuCo2Al9
- Spin-supersolidity induced quantum criticality and magnetocaloric effect in the triangular-lattice antiferromagnet RbCo(SeO)