Properties of donor qubits in ZnO formed by indium ion implantation
arXiv:2212.05230 · doi:10.1103/PhysRevApplied.19.054090
Abstract
Shallow neutral donors (D) in ZnO have emerged as a promising candidate for solid-state spin qubits. Here, we report on the formation of D in ZnO via implantation of In and subsequent annealing. The implanted In donors exhibit optical and spin properties on par with doped donors. The inhomogeneous linewidth of the donor-bound exciton transition is less than 10 GHz, comparable to the optical linewidth of In. Longitudinal spin relaxation times () exceed reported values for Ga donors, indicating that residual In implantation damage does not degrade . Two laser Raman spectroscopy on the donor spin reveals the hyperfine interaction of the donor electron with the spin-9/2 In nuclei. This work is an important step toward the deterministic formation of In donor qubits in ZnO with optical access to a long-lived nuclear spin memory.
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