Field-tunable toroidal moment and anomalous Hall effect in noncollinear antiferromagnetic Weyl semimetal Co1/3TaS2

Abstract

Combining magnetism with band topology provides various novel phases that are otherwise impossible. Among several cases, noncollinear metallic antiferromagnets can reveal particularly rich topological physics due to their diverse magnetic ground states. However, there are only a few experimental studies due to the lack of suitable materials, especially with triangular lattice antiferromagnets. Here, we report that metallic triangular antiferromagnet Co1/3TaS2 exhibits a substantial anomalous Hall effect (AHE) related to its noncollinear magnetic order. Our first-principles calculations found that hourglass Weyl fermions from the non-symmorphic symmetry trigger AHE. We further show that AHE in Co1/3TaS2 can be characterized by the toroidal moment, a vortex-like multipole component that arises from a combination of chiral lattice and geometrical frustration. Finally, the unusual field-tunability of the toroidal moment puts Co1/3TaS2 as a rare example of a noncollinear metallic antiferromagnet filled with interesting magnetic and topological properties.

arXiv comment20 pages, 4 figures, Accepted for publication in npj Quantum Materials

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• Composition dependence of bulk properties in the Co-intercalated transition-metal dichalcogenide Co${}_{1/3}$TaS${}_2$
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• Double-$Q$ chiral stripe order in the anomalous Hall antiferromagnet CoNb${}_3$S${}_6$
• Correlation-driven origin of shallow electron pocket in Co${}_{1/3}$TaS${}_2$ revealed by ARPES and cluster perturbation theory
• Van der Waals Antiferromagnets: From Early Discoveries to Future Directions in the 2D Limit