Surface-bulk coupling in a Bi${}_2$Te${}_3$ nanoplate grown by van der Waals epitaxy

Abstract

We report on an experimental study of the effect of coherent surface-bulk electron scattering on quantum transport in a three-dimensional topological insulator Bi${}_2$Te${}_3$ nanoplate. The nanoplate is grown via van der Waals epitaxy on a mica substrate and a top-gated Hall-bar device is fabricated from the nanoplate directly on the growth substrate. Top-gate voltage dependent measurements of the sheet resistance of the device reveal that the transport carriers in the nanoplate are of n-type and that, with decreasing top gate voltage, the carrier density in the nanoplate is decreased. However, the mobility is increased with decreasing top-gate voltage. This mobility increase with decreasing carrier density in the nanoplate is demonstrated to arise from a decrease in bulk-to-surface electron scattering rate. Low-field magnetotransport measurements are performed at low temperatures. The measured magnetoconductivity of the nanoplate shows typical weak anti-localization (WAL) characteristics. We analyze the measurements by taking surface-bulk inter-channel electron scattering into account and extract dephasing times ${\tau }_{\varphi }$, diffusion coefficients $D$ of electrons at the top surface and in the bulk, and the surface-bulk scattering times ${\tau }_{SB}$ as a function of top-gate voltage and temperature. It is found that the dephasing in the nanoplate arises dominantly from electron-electron scattering with small energy transfers. It is also found that the ratio of ${\tau }_{\varphi }$/${\tau }_{SB}$ (a measure of the surface-bulk electron coherent coupling) is decreased with decreasing gate voltage or increasing temperature. We demonstrate that taking the surface-bulk coherent electron scattering in our Bi${}_2$Te${}_3$ nanoplate into account is essential to understand quantum transport measurements at low temperatures.

15 pages, 3 figures, Supplementary Materials

References in corpus (8)

• Superconducting proximity effect and Majorana fermions at the surface of a topological insulator
• Nonlocal edge state transport in the quantum spin Hall state
• Impurity effect on weak anti-localization in the topological insulator Bi2Te3
• Bulk Band Gap and Surface State Conduction Observed in Voltage-Tuned Crystals of the Topological Insulator Bi${}_2$Se${}_3$
• Tunable Surface Conductivity in Bi2Se3 Revealed in Diffusive Electron Transport
• Weak Localization and Antilocalization in Topological Insulator Thin Films with Coherent Bulk-Surface Coupling
• Enhanced electron dephasing in three-dimensional topological insulators
• Experimental evidence and control of the bulk-mediated intersurface coupling in topological insulator Bi2Te2Se nanoribbons