Study of the electronic properties of topological kagome metals YVSn and GdVSn
arXiv:2109.07394 · doi:10.1103/PhysRevB.104.235139
Abstract
The synthesis and characterization of vanadium-based kagome metals YVSn and GdVSn are presented. X-ray diffraction, magnetization, magnetotransport, and heat capacity measurements reveal an ideal kagome network of V-ions coordinated by Sn and separated by triangular lattice planes of rare-earth ions. The onset of low-temperature, likely noncollinear, magnetic order of Gd spins is detected in GdVSn, while V-ions in both compounds remain nonmagnetic. Density functional theory calculations are presented modeling the band structures of both compounds, which can be classified as topological metals in the paramagnetic state. Both compounds exhibit high mobility, multiband transport and present an interesting platform for controlling the interplay between magnetic order associated with the -site sublattice and nontrivial band topology associated with the V-based kagome network. Our results invite future exploration of other VSn (=rare earth) variants where this interplay can be tuned via -site substitution.
11 pages, 10 figures
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